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Optics Express

Quantum frequency translation by four-wave mixing in a fiber: low-conversion regime

Lasse Mejling, Colin J. McKinstrie, Michael G. Raymer, Karsten K. Rottwitt

Published Mar 26, 2012• 28 citations
Publisher

Abstract

In this paper we consider frequency translation enabled by Bragg scattering, a four-wave mixing process. First we introduce the theoretical background of the Green function formalism and the Schmidt decomposition. Next the Green functions for the low-conversion regime are derived perturbatively in the frequency domain, using the methods developed for three-wave mixing, then transformed to the time domain. These results are also derived and verified using an alternative time-domain method, the results of which are more general. For the first time we include the effects of convecting pumps, a more realistic assumption, and show that separability and arbitrary reshaping is possible. This is confirmed numerically for Gaussian pumps as well as higher-order Hermite-Gaussian pumps.

DOI
10.1364/oe.20.008367

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In this paper we consider frequency translation enabled by Bragg scattering, a four-wave mixing process. First we introduce the theoretical background of the Green function formalism and the Schmidt decomposition. Next the Green functions for the low-conversion regime are derived perturbatively in the frequency domain, using the methods developed for three-wave mixing, then transformed to the time domain. These results are also derived and verified using an alternative time-domain method, the results of which are more general. For the first time we include the effects of convecting pumps, a more realistic assumption, and show that separability and arbitrary reshaping is possible. This is confirmed numerically for Gaussian pumps as well as higher-order Hermite-Gaussian pumps.
We study quantum frequency translation and two-color photon interference enabled by the Bragg scattering four-wave mixing process in optical fiber. Using realistic model parameters, we computationally and analytically determine the Green function and Schmidt modes for cases with various pump-pulse lengths. These cases can be categorized as either "non-discriminatory" or "discriminatory" in regards to their propensity to exhibit high-efficiency translation or high-visibility two-photon interference for many different shapes of input wave packets or for only a few input wave packets, respectively. Also, for a particular case, the Schmidt mode set was found to be nearly equal to a Hermite-Gaussian function set. The methods and results also apply with little modification to frequency conversion by sum-frequency conversion in optical crystals.
In this paper, we consider the effects of nonlinear phase modulation on frequency conversion by four-wave mixing (Bragg scattering) in the low-conversion regime. We derive the Green functions for this process using the time-domain collision method, for partial collisions, in which the four fields interact at the beginning or the end of the fiber, and complete collisions, in which the four fields interact at the midpoint of the fiber. If the Green function is separable, there is only one output Schmidt mode, which is free from temporal entanglement. We find that nonlinear phase modulation always chirps the input and output Schmidt modes and renders the Green function formally nonseparable. However, by pre-chirping the pumps, one can reduce the chirps of the Schmidt modes and enable approximate separability. Thus, even in the presence of nonlinear phase modulation, frequency conversion with arbitrary pulse reshaping is possible, as predicted previously [Opt. Express 20, 8367-8396 (2012)].
We present a quantum-mechanical model that describes fiber-based frequency conversion by four-wave-mixing Bragg scattering in the presence of Raman interactions. In the case of continuous-wave pumps, we find closed-form expressions for the conversion efficiency and photon statistics characterized by the second-order correlation function. For pulsed pumps, we derive a highly general model based on Green functions and provide a numerical solution method using a split-step scheme. In both cases, we find that noise from spontaneous Raman scattering can pose a serious challenge to this type of frequency conversion if the pumps are less than 30 THz from the quantum fields. However, this impact can be mitigated with cross-polarized pumps and, on the anti-Stokes side, through fiber cooling.
Recently, we solved the coupled-mode equations for Bragg scattering (BS) in the low- and high-conversion regimes, but without the effects of nonlinear phase modulation (NPM). We now present solutions and Green functions in the low-conversion regime that include NPM. We find that NPM does not change the lowest-order conversion efficiency, but prevents complete separability (freedom from temporal entanglement). This problem is overcome to some degree by pre-chirping the pumps, which mitigates the effects of NPM. We conclude that arbitrary reshaping of the output modes and nearly complete separability are still possible, even when the effects of NPM are included. Finally, the effects of using different input signals are considered, and we conclude that using the natural input modes of the system drastically increases the efficiency.
The authors consider, experimentally and theoretically, the quantum frequency translation (i.e., noiseless conversion) of quantum states of light, including single-photon states. This process is useful for allowing quantum optical systems (atoms, ions, cavities, fibers, detectors) operating at different wavelengths to communicate with each other. The authors recently developed the process of frequency translation in optical fiber through use of the Bragg scattering four-wave mixing process. The high nonlinearity and the ability to control dispersion in photonic crystal fiber (PCF) enable efficient translation between nearby photon channels within the visible to-near-infrared spectral range, useful in quantum networks. This offers an important advantage compared with frequency translation using second-order nonlinear optical crystals, which limits the translation process to widely separated frequencies only.
We experimentally demonstrate frequency translation of a non-classical optical field by Bragg-scattering four-wave mixing, driven by orthogonally polarized pump pulses in a birefringent optical fiber. Heralded single photons are up- and down-translated by 6.8 THz between bands at 688.1 nm and 678.2 nm, each with efficiency > 97%. The input and output spectral shape and bandwidth show negligible modulation. Second-order auto-correlation measurements of the 678.2 nm and 688.1 nm fields at maximum conversion yield values of 0.0302 ± 0.0005 and 0.028 ± 0.001, respectively, compared with the input second-order correlation of 0.026 ± 0.001; this indicates that the frequency translation process preserves the non-classical nature of the field. The high efficiency, broad bandwidth, and low noise render this scheme useful for quantum networks and sources.