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Physical Review Letters

High Frequency Atomic Magnetometer by Use of Electromagnetically Induced Transparency

George E. Katsoprinakis, David Petrosyan, Iannis K. Kominis

Published Dec 6, 2006• 26 citations
Publisher

Abstract

Atomic magnetometers have achieved magnetic sensitivities in the subfemtotesla regime. Their bandwidth is determined by the transverse spin relaxation rate, 1/T2, which also determines the magnetic sensitivity. It is theoretically demonstrated that by using an electromagnetically induced transparent probe beam in a pump-probe atomic magnetometer, it is possible to operate the latter at frequencies much higher than its bandwidth, maintaining a high signal-to-noise ratio.

DOI
10.1103/physrevlett.97.230801

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Atomic magnetometers have achieved magnetic sensitivities in the subfemtotesla regime. Their bandwidth is determined by the transverse spin relaxation rate, 1/T2, which also determines the magnetic sensitivity. It is theoretically demonstrated that by using an electromagnetically induced transparent probe beam in a pump-probe atomic magnetometer, it is possible to operate the latter at frequencies much higher than its bandwidth, maintaining a high signal-to-noise ratio.
A high-sensitivity optically pumped atomic magnetometer working in the geomagnetic range utilizing the light-narrowing effect and in-phase excitation is described. The setup is based on a simple pump–probe arrangement built around a Cs vapor cell whose active volume is 64 mm3. The transverse oscillating field is applied parallel to the probe beam to drive Zeeman resonance, and the in-phase component of the resonance signal is measured to determine the field. The sensitivity of the magnetometer is improved by pumping most atoms into the stretched state. Consequently, spin-exchange relaxation is suppressed, and a sensitivity of 0.1 pT/Hz1/2 in the range of 10 μT is achieved. This magnetometer has the advantages of large dynamic range, high performance of low-frequency stabilization, high response speed, and compact size. It can be used for many cutting-edge applications such as detection of magnetic anomalies.
An atomic magnetometer is a sensor which is used to measure a magnetic field through its interaction with the atomic sample. Significant research into atomic magnetometry has led to the development of very sensitive atomic sensors capable of matching the sensitivity of the most sensitive magnetometers, superconducting quantum interference devices (SQUIDs). Because SQUIDS require cryogenics to operate, atomic magnetometers provide a sensitive, yet low-cost alternative. They have found use in many areas such as medicine, security, explosives detection and fundamental physics research. One of the primary factors influencing sensitivity is the detuning of the probe beam from the resonant transitions of the atomic ground state. A caesium room temperature radio-frequency (rf) magnetometer is constructed and used to investigate the influence of the probe beam detuning on the magnetometer signal of the F = 3 and F = 4 ground states. The results of probing near and far from resonance revealed an off-resonant regime and two absorptive regimes. In the off-resonant regime, the atomic spins are unperturbed by the probe beam; it is a quantum non-demolition (QND) interaction. The two absorptive regimes, found when the probe beam is in the vicinity of either the 62S1 2 F = 3 → 6 2P3 2 F 0 = 2,3,4 or the 62S1 2 F = 4 → 6 2P3 2 F 0 = 3,4,5 transitions, is characterised as a non-QND interaction in which the probe beam influences the measurement. The sensitivity of the rf magnetometer is determined to be ≈ 1.98 fT/ √ Hz. In addition, the exploration of the relationship between the signal to noise ratio (SNR) and probe beam detuning revealed that the SNR is constant with detuning but the larger the detuning, the higher the probe beam power needs to be to reach the optimum SNR.
Optically pumped radio frequency (RF) atomic magnetometers have been shown to have an improved sensitivity over standard tuned coils for frequencies less than 50 MHz, making these RF magnetometers attractive for the detection of nuclear quadrupole resonance (NQR) and low-field nuclear magnetic resonance (NMR) signals. In an atomic magnetometer a linearly polarized probe beam measures, through Faraday rotation, the transverse atomic magnetization induced by the resonant RF signal. The resonance, or Larmor, frequency of the magnetometer is easily tuned with a small magnetic field. We construct an atomic magnetometer based on a potassium vapor cell with a measured sensitivity of 0.22 ± 0.02 fT/ √ Hz and a detection bandwidth of 334 ± 11 Hz when tuned to 423 kHz, giving a Q of over 1200. While high Q magnetometers are sensitive to weak magnetic fields, they are also sensitive to magnetic transients, such as those associated with the excitation pulses needed for magnetic resonance. The ringing created by such transients can obscure the signal of interest. This is particularly detrimental for magnetic resonance signals that decay faster than the transverse relaxation rate. We demonstrate that by feeding back part of the optical signal to orthogonal electromagnetic coils, this unwanted ringing can be quickly damped out leaving the magnetometer ready for the detection of the signal. This negative feedback as applied to the K spins is called spin-damping and can be used to relax the K atoms faster by more than two orders of magnitude. Using spin-damping we reduce the dead-time before data acquisition from 0.8 to 0.2 ms in the detection of NQR signals from ammonium nitrate, one of the so-called fertilizer bomb explosives with an NQR frequency of 423 kHz. Furthermore, we discover that spin-damping can not only be used to suppress signals, it can also be used to suppress noise. We show that it can be used to suppress both environmental noise and more fundamental quantum noise, such as photon shot and spin projection noise. The latter suppression opens the door for its use in quantum control to initialize spin systems before measurements. For phase-sensitive detection, as is often used in magnetic resonance, spin-damping suppresses signal and noise in such a way as to increase the sensitivity bandwidth of the magnetometer. We prove, both theoretically and experimentally, that it is possible to increase the magnetometer detection bandwidth by a factor of 3 or more without significant loss in sensitivity. Such gains in bandwidth for a high Q magnetometer translate into savings in detection time, particularly for substance detection where the frequency of the signal of interest may not be completely known.
Here we demonstrate an atomic magnetometer that has a bandwidth of more than 100 kHz and a sensitivity of $180\phantom{\rule{0.2em}{0ex}}\mathrm{fT/}\ensuremath{\surd}\mathrm{Hz}$ at a Fourier frequency of 8 Hz, and $0.7\phantom{\rule{0.2em}{0ex}}\mathrm{nT/}\ensuremath{\surd}\mathrm{Hz}$ at 100 kHz. These sensitivity measurements are achieved at geophysically useful magnetic field magnitudes (approximately $50\phantom{\rule{0.2em}{0ex}}\ensuremath{\mu}\mathrm{T}$ inside a three-layer $\ensuremath{\mu}$-metal shield) and are limited by the photon shot noise for frequencies above 8 Hz. This device is based on a nonlinear magneto-optical rotation sensor that is operated with an active feedback to the pump modulation frequency. We present a theoretical description of the response functions of the components in the magnetometer. We show that the range of operation of atomic magnetometers can thus be expanded beyond the conventional high-sensitivity, low-bandwidth domain, to provide a high-linearity, high-bandwidth, and high-sensitivity sensor.
An optically pumped atomic magnetometer using a hybrid cell of potassium and rubidium atoms was demonstrated to yield high sensitivity to magnetic fields. We operated the magnetometer with the four possible combinations of optically pumped and optically probed atoms and found that the combination of optically pumped potassium and optically probed rubidium showed the highest sensitivity among the four combinations because the rubidium atoms were denser than those of potassium. Furthermore, we investigated the dependence of the sensitivity on the power densities of the pump and probe beams and the wavelength of the probe beam. The magnetometer using the hybrid cell required higher pump-beam power and had narrower magnetic linewidth than those of the single alkali-metal cell. However, the magnetic linewidth was larger than the theoretical value, ignoring the spin relaxation caused by the spin-exchange collisions. By adjusting the laser conditions, the highest sensitivity approached 30 fTrms/Hz1/2.
We demonstrate experimentally an atomic magnetometer based on optical pumping theory, a magnetic resonance that is induced by a radio frequency field and dependent on the magnetic field strength. Compared with the conventional method using one radiation field, which is used not only as the probe beam but also as a pump beam, the additional re-pump beam can increase remarkably the amplitude of the signal. It is shown that the amplitude of the magnetic field resonance signal can increase more than 55% by using an additional re-pump beam, which makes the sensitivity of the magnetometer higher. Finally, we investigate the relation between amplitude of the signal and re-pump laser power, and calculate the atomic population in the trapping states with rate equations.