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Optics Letters

Walsh modes and radial quantum correlations of spatially entangled photons

Daniël Geelen, W. Löffler

Published Oct 8, 2013• 11 citations
Publisher

Abstract

Orthogonal sets of 2D transverse modes are key to controlling the spatial degree of freedom of light in a classical or quantum context. In contrast to the azimuthal part, which is easily accessible using orbital angular momentum modes, control of the radial part is more difficult. We show here that simple sets of orthogonal binary sequences, the Walsh functions, provide a workable solution for exploration of the radial space with phase-only spatial light modulation. We demonstrate this by measuring "sequency" quantum correlations between different radial Walsh modes of spatially entangled photon pairs and for numerically optimized versions thereof.

DOI
10.1364/ol.38.004108

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Orthogonal sets of 2D transverse modes are key to controlling the spatial degree of freedom of light in a classical or quantum context. In contrast to the azimuthal part, which is easily accessible using orbital angular momentum modes, control of the radial part is more difficult. We show here that simple sets of orthogonal binary sequences, the Walsh functions, provide a workable solution for exploration of the radial space with phase-only spatial light modulation. We demonstrate this by measuring "sequency" quantum correlations between different radial Walsh modes of spatially entangled photon pairs and for numerically optimized versions thereof.
Spatially entangled twin photons allow the study of high-dimensional entanglement, and the Laguerre-Gauss modes are the most commonly used basis to discretize the single-photon mode spaces. In this basis, to date only the azimuthal degree of freedom has been investigated experimentally due to its fundamental and experimental simplicity. We show that the full spatial entanglement is indeed accessible experimentally; i.e., we have found practicable radial detection modes with negligible cross correlations. This allows us to demonstrate hybrid azimuthal-radial quantum correlations in a Hilbert space with more than 100 dimensions per photon.
With the emergence of the field of quantum communications, the appropriate choice of photonic degrees of freedom used for encoding information is of paramount importance. Highly precise techniques for measuring the polarisation, frequency, and arrival time of a photon have been developed. However, the transverse spatial degree of freedom still lacks a measurement scheme that allows the reconstruction of its full transverse structure with a simple implementation and a high level of accuracy. Here we show a method to measure the azimuthal and radial modes of Laguerre-Gaussian beams with a greater than 99 % accuracy, using a single phase screen. We compare our technique with previous commonly used methods and demonstrate the significant improvements it presents for quantum key distribution and state tomography of high-dimensional quantum states of light. Moreover, our technique can be readily extended to any arbitrary family of spatial modes, such as mutually unbiased bases, Hermite-Gauss, and Ince-Gauss. Our scheme will significantly enhance existing quantum and classical communication protocols that use the spatial structure of light, as well as enable fundamental experiments on spatial-mode entanglement to reach their full potential.
The Bell inequalities for azimuthal quantum number, i.e., orbital angular momentum, have been extensively reported to show quantum correlations between the spatial degree of freedom of entangled photon pairs. Here we investigate instead the Bell inequalities for radial quantum number. We demonstrate, both theoretically and experimentally, the violation of a suitable Clauser-Horne-Shimony-Holt Bell inequality for the radial index ppp of the Laguerre-Gaussian mode, thus manifesting the entanglement in the radial structure of two-photon wave functions.
Abstract It is well known that photons can carry a spatial structure akin to a ‘twisted’ or ‘rippled’ wavefront. Such structured light fields have sparked significant interest in both classical and quantum physics, with applications ranging from dense communications to light–matter interaction. Harnessing the full advantage of transverse spatial photonic encoding using the Laguerre–Gaussian (LG) basis in the quantum domain requires control over both the azimuthal (twisted) and radial (rippled) components of photons. However, precise measurement of the radial photonic degree-of-freedom has proven to be experimentally challenging primarily due to its transverse amplitude structure. Here we demonstrate the generation and certification of full-field LG entanglement between photons pairs generated by spontaneous parametric down conversion in the telecom regime. By precisely tuning the optical system parameters for state generation and collection, and adopting recently developed techniques for precise spatial mode measurement, we are able to certify fidelities up to 85% and entanglement dimensionalities up to 26 in a 43-dimensional radial and azimuthal LG mode space. Furthermore, we study two-photon quantum correlations between nine LG mode groups, demonstrating a correlation structure related to mode group order and inter-modal cross-talk. In addition, we show how the noise-robustness of high-dimensional entanglement certification can be significantly increased by using measurements in multiple LG mutually unbiased bases. Our work demonstrates the potential offered by the full spatial structure of the two-photon field for enhancing technologies for quantum information processing and communication.