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arXiv:2104.04506 · Journal of Optics

Entangled ripples and twists of light: radial and azimuthal Laguerre–Gaussian mode entanglement

Natalia Herrera Valencia, Vatshal Srivastav, Saroch Leedumrongwatthanakun, Will McCutcheon, Mehul Malik

Published Aug 25, 2021• 23 citations
arXivHTMLPDF

Abstract

Abstract It is well known that photons can carry a spatial structure akin to a ‘twisted’ or ‘rippled’ wavefront. Such structured light fields have sparked significant interest in both classical and quantum physics, with applications ranging from dense communications to light–matter interaction. Harnessing the full advantage of transverse spatial photonic encoding using the Laguerre–Gaussian (LG) basis in the quantum domain requires control over both the azimuthal (twisted) and radial (rippled) components of photons. However, precise measurement of the radial photonic degree-of-freedom has proven to be experimentally challenging primarily due to its transverse amplitude structure. Here we demonstrate the generation and certification of full-field LG entanglement between photons pairs generated by spontaneous parametric down conversion in the telecom regime. By precisely tuning the optical system parameters for state generation and collection, and adopting recently developed techniques for precise spatial mode measurement, we are able to certify fidelities up to 85% and entanglement dimensionalities up to 26 in a 43-dimensional radial and azimuthal LG mode space. Furthermore, we study two-photon quantum correlations between nine LG mode groups, demonstrating a correlation structure related to mode group order and inter-modal cross-talk. In addition, we show how the noise-robustness of high-dimensional entanglement certification can be significantly increased by using measurements in multiple LG mutually unbiased bases. Our work demonstrates the potential offered by the full spatial structure of the two-photon field for enhancing technologies for quantum information processing and communication.

DOI
10.1088/2040-8986/ac213c

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Abstract It is well known that photons can carry a spatial structure akin to a ‘twisted’ or ‘rippled’ wavefront. Such structured light fields have sparked significant interest in both classical and quantum physics, with applications ranging from dense communications to light–matter interaction. Harnessing the full advantage of transverse spatial photonic encoding using the Laguerre–Gaussian (LG) basis in the quantum domain requires control over both the azimuthal (twisted) and radial (rippled) components of photons. However, precise measurement of the radial photonic degree-of-freedom has proven to be experimentally challenging primarily due to its transverse amplitude structure. Here we demonstrate the generation and certification of full-field LG entanglement between photons pairs generated by spontaneous parametric down conversion in the telecom regime. By precisely tuning the optical system parameters for state generation and collection, and adopting recently developed techniques for precise spatial mode measurement, we are able to certify fidelities up to 85% and entanglement dimensionalities up to 26 in a 43-dimensional radial and azimuthal LG mode space. Furthermore, we study two-photon quantum correlations between nine LG mode groups, demonstrating a correlation structure related to mode group order and inter-modal cross-talk. In addition, we show how the noise-robustness of high-dimensional entanglement certification can be significantly increased by using measurements in multiple LG mutually unbiased bases. Our work demonstrates the potential offered by the full spatial structure of the two-photon field for enhancing technologies for quantum information processing and communication.
With the emergence of the field of quantum communications, the appropriate choice of photonic degrees of freedom used for encoding information is of paramount importance. Highly precise techniques for measuring the polarisation, frequency, and arrival time of a photon have been developed. However, the transverse spatial degree of freedom still lacks a measurement scheme that allows the reconstruction of its full transverse structure with a simple implementation and a high level of accuracy. Here we show a method to measure the azimuthal and radial modes of Laguerre-Gaussian beams with a greater than 99 % accuracy, using a single phase screen. We compare our technique with previous commonly used methods and demonstrate the significant improvements it presents for quantum key distribution and state tomography of high-dimensional quantum states of light. Moreover, our technique can be readily extended to any arbitrary family of spatial modes, such as mutually unbiased bases, Hermite-Gauss, and Ince-Gauss. Our scheme will significantly enhance existing quantum and classical communication protocols that use the spatial structure of light, as well as enable fundamental experiments on spatial-mode entanglement to reach their full potential.
We demonstrate the generation of unbalanced two-photon entanglement in the Laguerre–Gaussian (LG) transverse-spatial degree-of-freedom, where one photon carries a fundamental (Gauss) mode and the other a higher-order LG mode with a non-zero azimuthal (ℓ) or radial (p) component. Taking a cue from the N00N state nomenclature, we call these types of states ℓ00ℓ-entangled. They are generated by shifting one photon in the LG mode space and combining it with a second (initially uncorrelated) photon at a beamsplitter, followed by coincidence detection. In order to verify two-photon coherence, we demonstrate a two-photon “twisted” quantum eraser, where Hong–Ou–Mandel interference is recovered between two distinguishable photons by projecting them into a rotated LG superposition basis. Using an entanglement witness, we find that our generated states have fidelities of 95.31% and 89.80% to their respective ideal maximally entangled states. In addition to being of fundamental interest, this type of entanglement will likely have a significant impact on tickling the average quantum physicist's funny bone.
Abstract High-dimensional spatially entangled two-photon states generated by the spontaneous parametric down-conversion process (SPDC) have become a promising resource for several quantum information science applications. In order to harness high-dimensional entanglement advantages, detection capability in the Schmidt basis is a necessity. Spatial entanglement has been explored in several modal bases, such as pixel, azimuthal, and radial modes. Among them, pixel and azimuthal entanglement have been widely utilized due to efficient access to their Schmidt modes, while radial-mode entanglement remains underexploited. This is due to radial coordinates not having a Schmidt-decomposed form for the SPDC photons or a technique for measuring high-dimensional radial Schmidt modes, which is a major roadblock in harnessing radial mode advantages. In this work, we first theoretically show that azimuthal averaging of SPDC two-photon states yields a radial Schmidt-decomposed form under typical experimental situations. We then demonstrate an innovative approach for extracting the radial Schmidt modes and their spectrum by characterizing the density matrix in the radial basis of one of the SPDC photons. Finally, we report the first-ever measurement of the radial Schmidt spectrum of up to 50 radial Schmidt modes with about 98% fidelity.
High-dimensional spatially entangled two-photon state generated by spontaneous parametric down-conversion process (SPDC) has become a promising resource for several quantum information science applications. For harnessing high-dimensional entanglement advantages, detection capability in the Schmidt basis is a necessity. Spatial entanglement has been explored in several modal bases, such as pixel, azimuthal, and radial modes. Among them, pixel and azimuthal entanglement have been widely utilized due to efficient access to their Schmidt modes, while radial-mode entanglement remains underexploited. This is because for radial coordinates, there is neither a Schmidt-decomposed form for the SPDC photons nor is there a technique for measuring high-dimensional radial Schmidt modes, which is a major roadblock in harnessing radial mode advantages. In this work, we first theoretically show that the azimuthal averaging of SPDC two-photon state yields a radial Schmidt-decomposed form under typical experimental situations. We then demonstrate an innovative approach for extracting the radial Schmidt modes and their spectrum by characterizing the density matrix in the radial basis of one of the SPDC photons. Finally, we report the first-ever measurement of radial Schmidt spectrum of upto 50 radial Schmidt modes with about 98\% fidelity.
High-dimensional spatial entanglement generated via spontaneous parametric down-conversion (SPDC) provides a powerful resource for quantum information processing, yet its mode structure becomes increasingly complex when the pump occupies a higher-order Laguerre--Gaussian (LG) mode. Here, we develop an algebraic framework for characterizing biphoton spatial-mode entanglement by factorizing LG-pumped SPDC into a spatial-mode beam-splitter transformation followed by spatial two-mode squeezing. By choosing the biphoton LG basis radius as the geometric mean of the pump-beam radius and the crystal-induced correlation width, we obtain a natural modal basis in which the two operations can be treated separately. When the pump-beam radius matches the correlation width, spatial squeezing vanishes, and the two circular-mode components of the pump are independently conserved across the signal and idler photons, leading to conservation of both orbital angular momentum and the total spatial mode number. We further derive an analytical expression for the Schmidt number for arbitrary LG pump modes and squeezing strengths, revealing how the radial and azimuthal pump indices govern the dimensionality of the spatial entanglement. This algebraic characterization provides a unified description of the mode structure, conservation laws, and entanglement dimensionality of higher-order-LG-pumped SPDC.
Laguerre–Gaussian (LG) modes are characterized by two integer parameters, p and l , which correspond to the radial and azimuthal modes of photons. Both degrees of freedom are discrete and high-dimensional, and each can be used to construct a high-dimensional Hilbert space. Here, we use the radial-azimuthal modes of a single photon to construct two-dimensional and four-dimensional Bell states and experimentally realize full single-photon Bell-state characterization, thereby verifying the orthogonality and completeness of the Bell states. Subsequently, we measure the magnitude and phase of a four-dimensional superposition state in a 16-dimensional Hilbert space, obtaining results in good agreement with theoretical predictions, which further confirms the completeness of the four-dimensional Bell basis. Our experiment demonstrates that the radial and azimuthal modes of a single photon play equally important roles. Multiplexing these two degrees of freedom enables the construction of higher-dimensional Hilbert spaces and significantly enhances the information-carrying capacity of a single photon. Our results hold potential applications in the development of quantum communication protocols with high channel capacity.