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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Ultrafast phenomena in an active microcavity

Paolo Mataloni, Ottavia Jedrkiewicz, F. De Martini

Published Jul 14, 1998• 0 citations
Publisher

Abstract

Some ultrafast phenomena occurring in an active microcavity have been investigated. This device can behave as an efficient source of non-classical light, when a small number of molecules inside are excited by a femtosecond laser.In this way single photon n > states are generated with anon-classical sub-Poissonian distribution. Multiple excitations of a larger number of molecules can give rise to collective phenomena because of the strong super-radiant ultrafast coupling within the transverse region of the microcavity electromagnetic field. This process has been experimentally studied by means of a high efficiency, single photon, femtosecond non-linear optical gate.

DOI
10.1117/12.316576

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Some ultrafast phenomena occurring in an active microcavity have been investigated. This device can behave as an efficient source of non-classical light, when a small number of molecules inside are excited by a femtosecond laser.In this way single photon n > states are generated with anon-classical sub-Poissonian distribution. Multiple excitations of a larger number of molecules can give rise to collective phenomena because of the strong super-radiant ultrafast coupling within the transverse region of the microcavity electromagnetic field. This process has been experimentally studied by means of a high efficiency, single photon, femtosecond non-linear optical gate.
The process of generation of non-classical radiation in an active Fabry-Perot dye microcavity, under femtosecond excitation, has been investigated. Single photon states, with a non-classical sub-Poissonian distribution have been generated after the excitation of a small number of active molecules, located between the two mirrors. By multiple excitation of the active medium, collective emission phenomena are expected because of the strong superradiant coupling occurring within the transverse coherence area of the microcavity. In particular, we have experimentally verified the principle of relativistic causality within the process of two-dipole superradiance by transverse interaction, in condition of strong microcavity confinement.
The active microcavity is adopted as an efficient source of nonclassical light. Using this device, excited with a mode-locked laser at a rate of 100 MHz, single photons are generated over a single field mode with a nonclassical sub-Poissonian distribution. Adiabatic recycling within a multistep Franck-Condon molecular optical-pumping mechanism, characterized by quantum efficiency close to 1, implies a pump self-regularization process leading to a striking nnn-squeezing effect. Replicating the basic single-atom excitation process a beam of quantum photon ∣n〉|n〉∣n〉 states (Fock states) can be created. This represents a significant advance in the fields of basic quantum-mechanical investigation, quantum communication, and quantum cryptography.
The active microcavity is adopted as an efficient source of non-classical light. By this device, excited by a mode-locked laser at a rate of 100 MHz, single photons are generated over a single field mode with a non-classical sub-Poissonian distribution. The process of adiabatic recycling within a multistep Franck–Condon molecular optical-pumping mechanism, characterized in our case by a quantum efficiency close to one, implies a pump self-regularization process leading to a striking n-squeezing effect. Moreover, the microactivity has been adopted as active beam splitter in a novel Hanbury-Brown–Twiss configuration for the radiation taking place over the two output mirrors. By a replication of the basic single-atom excitation process a beam of quantum photon |n〉 states (Fock states) can be created. The new process may represent a significant advance in the modern fields of basic quantum-mechanical investigation, quantum communication and quantum cryptography.
The active microcavity is adopted as an efficient source of non-classical light. By this device, excited by a mode-locked laser at a rate of 100 MHz, single-photons are generated over a single field mode with a nonclassical sub-poissonian distribution. The process of adiabatic recycling within a multi-step Franck-Condon molecular optical-pumping mechanism, characterized in our case by a quantum efficiency very close to one, implies a pump self-regularization process leading to a striking n-squeezing effect. By a replication of the basic single-atom excitation process a beam of quantum photon (Fock states) can be created. The new process represents a significant advance in the modern fields of basic quantum-mechanical investigation, quantum communication and quantum cryptography.
The use of molecules in quantum optical applications has been hampered by incoherent internal vibrations and other phononic interactions with their environment. Here we show that an organic molecule placed into an optical microcavity behaves as a coherent two-level quantum system. This allows the observation of 99% extinction of a laser beam by a single molecule, saturation with less than 0.5 photons and non-classical generation of few-photons super-bunched light. Furthermore, we demonstrate efficient interaction of the molecule–microcavity system with single photons generated by a second molecule in a distant laboratory. Our achievements represent an important step towards linear and nonlinear quantum photonic circuits based on organic platforms.
Semiconductor microcavities are widely used to study collective interactions of cavity exciton-polaritons leading to their condensation phenomenon. Exciton-light interaction is highly enhanced in such structures due to the resonance enhancement of the electromagnetic field inside the high quality cavity. Considerably lower interest is concerned to exciton states non-resonant with the cavity mode for which the exciton-photon interaction is strongly reduced due to the existence of the cavity. We point out here that these states are responsible for non-classical light generation in semiconductor microcavities.