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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Collisionally induced quantum interference in resonance fluorescence of two-level atoms

Wojciech Gawlik, Bogdan Lobodzinski

Published Oct 21, 1998• 0 citations
Publisher

Abstract

In the experiment with barium vapor (close approximation of a two-level system) we found spectra of resonance fluorescence having the form of a pressure-broadened line with a narrow, not collisionally broadened, dip. They are interpreted as the result of collisionally-induced quantum interference among possible spontaneous emission channels of a dressed atom subjected to stochastic perturbation. Also, the analogy between these effects and the coherent population trapping in three-level systems is pointed out.

DOI
10.1117/12.328233

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In the experiment with barium vapor (close approximation of a two-level system) we found spectra of resonance fluorescence having the form of a pressure-broadened line with a narrow, not collisionally broadened, dip. They are interpreted as the result of collisionally-induced quantum interference among possible spontaneous emission channels of a dressed atom subjected to stochastic perturbation. Also, the analogy between these effects and the coherent population trapping in three-level systems is pointed out.
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Stochastic perturbation of two-level atoms strongly driven by a coherent light field is analyzed by the quantum-trajectory method. A method is developed for calculating the resonance fluorescence spectra from numerical simulations. It is shown that in the case of dominant incoherent perturbation, the stochastic noise can unexpectedly create phase correlation between the neighboring atomic dressed states. This phase correlation is responsible for quantum interference between the related transitions resulting in anomalous modifications of the resonance fluorescence spectra.
The resonance fluorescence from a four-level atom driven by two coherent fields is studied. If the dipole moments between the two upper levels and each of the two lower levels are parallel, the spontaneous emission paths from the upper levels to the lower levels will have strongly or even completely destructive quantum interference. We show that this quantum interference will result in a complete inhibition of the fluorescence when one of the driving fields is tuned at the middle point of the upper levels. The quantum interference will lead to the dependence of atomic populations at steady state on the initial condition, when both of the driving fields are tuned to the middle point of the upper levels. When the dipole moments are close to but not exactly parallel, or none of the driving fields is tuned at the middle point of the upper levels and there is a small difference between detunings of the two driving fields to the uppermost level, ultranarrow lines at the spectral center appear because of the destructive quantum interference.
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The effect of collisions on the resonance fluorescence spectrum of two-level atoms excited by monochromatic resonance radiation is studied. Analysis is performed for systems where the Doppler broadening is small compared to the collision frequency (high buffer gas pressures) and for the general case where collisions arbitrarily change the phase of the radiation-induced dipole moment (from completely interrupted to completely unaffected phase of the dipole moment). Both at a relatively low and at a high excitation radiation intensity, the resonance fluorescence spectrum is shown to depend on whether the two-level system is closed or open. This is especially true for the narrow unshifted Rayleigh scattering line. It is shown that, although the absorption line is homogeneously broadened, the resonance fluorescence spectrum exhibits a clearly pronounced anisotropy. In a direction close to the direction of propagation of the excitation radiation, the Rayleigh scattering line is maximally narrowed. Under certain conditions (that can easily be created in experiments), the width of this line is proportional to the diffusion coefficient of atoms interacting with the radiation.
The effect of the laser linewidth on the resonance fluorescence spectrum of a two-level atom is revisited. The novel spectral features, such as hole-burning and dispersive profiles at line centre of the fluorescence spectrum are predicted when the laser linewidth is much greater than its intensity. The unique features result from quantum interference between different dressed-state transition channels. c # 1999 Elsevier Science B.V. PACS : 42.50.Hz; 32.80.-t Keywords: Resonance fluorescence; Laser linewidth; Quantum interference The study of resonance fluorescence spectra has provided much fundamental insight into the subject of atom1light interactions. It is well known that for weak laser field excitation, the spectrum exhibits a Lorentzian lineshape, whereas it develops into the Mollow triplet for strong field excitation [1]. The latter is a direct signature of stimulated emissions and absorptions of the atom during the time interval for one spontaneous decay. Recently, considera...