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Physical Review B

Zigzag carbon nanotubes with generic electron-electron interactions

Judith E. Bunder, James Murray Hill

Published Oct 6, 2009• 5 citations
Publisher

Abstract

A Hamiltonian is derived for a zigzag carbon nanotube with an arbitrary number of weak electron-electron charge and spin interactions, which become significant in ultraclean systems. The renormalization group and bosonization are used to determine the ground-state phase diagram. Our phase diagram contains some exotic phases which have not previously been predicted in carbon nanotubes with physically possible interaction profiles. Phases of the undoped case include Mott insulators and a variety of density wave states. In the doped case a Tomanaga-Luttinger liquid is possible.

DOI
10.1103/physrevb.80.153406

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•Jan 1, 2001•6 citations
A Hamiltonian is derived for a zigzag carbon nanotube with an arbitrary number of weak electron-electron charge and spin interactions, which become significant in ultraclean systems. The renormalization group and bosonization are used to determine the ground-state phase diagram. Our phase diagram contains some exotic phases which have not previously been predicted in carbon nanotubes with physically possible interaction profiles. Phases of the undoped case include Mott insulators and a variety of density wave states. In the doped case a Tomanaga-Luttinger liquid is possible.
We investigate a metallic zigzag carbon nanotube by means of a Hubbard model, which includes both on-site and nearest-neighbor interactions. Assuming weak interactions, a renormalization group analysis of the equivalent two-leg ladder followed by bosonization and refermionization results in a Gross-Neveu model with an enlarged symmetry relative to the original Hamiltonian. For the undoped case the symmetry of the Gross-Neveu model is SO(8), but for the doped case the particle-hole symmetry is broken and the symmetry reduces to SO(6). Four ground-state phases are found in the undoped carbon nanotube with repulsive interactions, a ddd-wave Mott insulator, an sss-wave Mott insulator, a ppp-density wave, and a charge density wave. The doped case has two ground-state phases, a ddd-wave superconductor and a phase where a ppp density wave and a charge density wave coexist. We also explore the global phase diagram with a general interaction profile and find several additional states, including a chiral current phase where current flows around the nanotube along the zigzag bonds.
A $\ensuremath{\pi}$-electron network in nanographite systems with zigzag edges exhibits strongly localized edge states, which are expected to have peculiar properties. We study effects of electron-electron interactions on ground-state properties of zigzag nanographite ribbons and open-ended zigzag nanotubes by means of the weak-coupling renormalization group and the density-matrix renormalization-group method. It is shown that the ground state is a spin-singlet Mott insulator with finite charge and spin gaps. We also find that the edge states are robust against the electronic correlations, resulting in edge-effective spins that can flip almost freely. The schematic picture for the low-energy physics of the systems is discussed.
We derive a Hamiltonian for a two-leg ladder which includes an arbitrary number of charge and spin interactions which must be weak but are otherwise of arbitrary strength. To illustrate this Hamiltonian we consider two examples and use a renormalization-group technique to evaluate the ground-state phases. The first example is a two-leg ladder with zigzagged legs. We find that increasing the number of interactions in such a two-leg ladder may result in a richer phase diagram, particularly at half-filling where a few exotic phases are possible when the number of interactions are large and the angle of the zigzag is small. In the second example we determine under which conditions a two-leg ladder at quarter-filling is able to support a Tomanaga-Luttinger liquid phase. We show that this is only possible when the spin interactions across the rungs are ferromagnetic. In both examples we focus on lithium purple bronze, a two-leg ladder with zigzagged legs which is thought to support a Tomanaga-Luttinger liquid phase.
We derive a low-energy effective model of metallic zigzag carbon nanotubes at half filling. We show that there are three important features characterizing the low-energy properties of these systems: the long-range Coulomb interaction, umklapp scattering, and an explicit dimerization generated by interactions. The ratio of the dimerization induced gap and the Mott gap induced by the umklapp interactions is dependent on the radius of the nanotube and can drive the system upon increasing dimerization strength from a Haldane spin-liquid phase through a quantum phase transition with SU(2)1\mathrm{SU}{(2)}_{1}SU(2)1​ quantum symmetry to a dimerized phase. We consider the physical properties of the phases on either side of this transition, which should be relevant for realistic nanotubes.
The Luttinger model of the one-dimensional Fermi gas is the cornerstone of modern understanding of interacting electrons in one dimension. In fact, the enormous class of systems whose universal behavior is adiabatically connected to it are now deemed Luttinger liquids. Recently, it has been shown that metallic single-walled carbon nanotubes are almost perfectly described by the Luttinger Hamiltonian. Indeed, strongly non-Fermi liquid behavior has been observed in a variety of DC transport experiments, in very good agreement with theoretical predictions. Here, we describe how fractional quasiparticle charge, a fundamental property of Luttinger liquids, can be observed in impurity-induced shot noise.
We calculate the correlation functions and the dc conductivity of Luttinger liquid superlattices, modelled by a repeated pattern of interacting and free Luttinger liquids. In a specific realization, where the interacting subsystem is a Hubbard chain, the system exhibits a rich phase diagram with four different phases: two metals and two compressible insulators. In general, we find that the effective low-energy description amalgamates features of both types of liquids in proportion to their spatial extent, suggesting the interesting possibility of `engineered' Luttinger liquids. In recent years, new experimental techniques have made it possible to grow nanostructures which are topologically one-dimensional, such as quantum wires and Carbon nanotubes. However, care must be taken when invoking existing models to discuss their electronic properties, since inhomogeneities must be taken into account in a fundamental way. Consider, for instance, the Luttinger liquid (LL), which is the standard model for low-energy phenomena involving interacting electrons in one dimension [1]. The absence of conductance renormalization in long high-mobility GaAs wires [2] has been explained in terms of a usual LL (representing the wire) in contact with a non-interacting LL at each of its ends (representing the Fermi liquid leads); that is, overall, the system can be thought of as an inhomogeneous Luttinger Liquid (ILL). LLs with different inhomogeneity profiles have also been used in the context of the fractional quantum Hall effect (FQHE), to describe transitions between edge states at different fillings [3, 4], or between an edge state connected to a Fermi liquid [5]. A different class of inhomogeneous systems is represented by superlattices (SLs) and multilayers. By varying the relative th...