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Physical review. B, Condensed matter

Transition from quantum to classical dissipation in the problem of escape from a metastable well: Application to Josephson junctions

Kenneth S. Chow, Vinay Ambegaokar

Published Dec 1, 1988• 9 citations
Publisher

Abstract

For a dissipative quantum system in the low-damping regime, we show that the master-equation description of the reduced density matrix reduces, in the semiclassical limit, to the energy-diffusion version of the Fokker-Planck equation. This result can be generalized to include non-Ohmic damping and an external harmonic perturbation. Results of calculations based on the master equation show good agreement with experiments on the resistanceless-to-resistive transition in Josephson junctions in the classical regime and with results of purely classical calculations.

DOI
10.1103/physrevb.38.11168

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For a dissipative quantum system in the low-damping regime, we show that the master-equation description of the reduced density matrix reduces, in the semiclassical limit, to the energy-diffusion version of the Fokker-Planck equation. This result can be generalized to include non-Ohmic damping and an external harmonic perturbation. Results of calculations based on the master equation show good agreement with experiments on the resistanceless-to-resistive transition in Josephson junctions in the classical regime and with results of purely classical calculations.
We analyze the behavior of a damped quantum harmonic oscillator immersed in a heat bath with a nonlinear coupling. For this purpose, we construct a generalized master equation (GME) for the reduced density of the oscillator. We specialize the results for a quadratic coupling in the presence of a bosonic reservoir and an Ohmic dissipation model, analyzing the evolution equation for the mean value of the oscillator coordinate. In the asymptotic case we obtain a gain-loss master equation whose transition rates are polynomials in the number of quanta. No explicit solutions other than the equilibrium one can be written, since the standard methods do not apply. The equilibrium solution is investigated and the eigenvalues of the corresponding spectral problem are numerically computed to study the effect of the nonlinearity on the evolution of the system. By means of the Wigner transformation of the GME, we extract a third-order partial derivative equation that represents the semiclassical evolution of the damped oscillator. In the classical limit this is a nonlinear Fokker-Planck equation.
Using the quantum effective action in the Schwinger-Keldysh formalism, we derive quantum-thermal corrections to the semiclassical dynamics of a dissipative system described by a macroscopic degree of freedom. We discuss the connection with the Ehrenfest theorem and, within the local potential approximation, obtain the corrections in closed form for arbitrary temperature and damping, showing that as the temperature increases, they cross over from purely quantum to purely thermal. In the low-temperature and weak-damping regime, corrections are set by the zero-point energy of fluctuations evaluated at the classical underdamped frequency, closely paralleling the conservative case, which allows us to go to higher order in the derivative expansion. We apply these general results to the resistively and capacitively shunted superconducting Josephson junction and to an elongated bosonic junction, where corrections can reach the percent level under realistic conditions.
Abstract We consider a particle trapped by a generic external potential and under the influence of a quantum-thermal Ohmic bath. Starting from the Langevin equation, we derive the corresponding Schwinger-Keldysh action. Then, within the path-integral formalism, we obtain both the semiclassical Fokker-Planck equation and the quantum Fokker-Planck equation for this out-of-equilibrium system. In the case of an external harmonic potential and in the underdamped regime, we find that our Fokker-Planck equations contain an effective temperature TeffT_{\text {eff}}Teff​ T eff , which crucially depends on the interplay between quantum and thermal fluctuations in contrast to the classical Fokker-Planck equation. In the regime of high temperatures, one recovers the classical Fokker-Planck equation. As an application of our result, we also provide the stationary solution of the semiclassical Fokker-Planck equations for a superconducting Josephson circuit and for a Bose Josephson junction, which are experimentally accessible.
Thermal escape out of a metastable well is considered in the weak friction regime, where the bottleneck for decay is energy diffusion, and at lower temperatures, where quantum tunneling becomes relevant. Within a systematic semiclassical formalism an extension of the classical diffusion equation is derived starting from a quantum mechanical master equation. In contrast to previous approaches finite barrier transmission also affects transition probabilities. The decay rate is obtained from the stationary nonequilibrium solution and captures the intimate interplay between thermal and quantum fluctuations above the crossover to the deep quantum regime.
Recent progress in our understanding of quantum effects on the Brownian motion in an external potential is reviewed. This problem is ubiquitous in physics and chemistry, particularly in the context of decay of metastable states, for example, the reversal of the magnetization of a single domain ferromagnetic particle, kinetics of a superconducting tunnelling junction, etc. Emphasis is laid on the establishment of master equations describing the diffusion process in phase space analogous to the classical Fokker-Planck equation. In particular, it is shown how Wigner's [E. P. Wigner, Phys. Rev., 1932, 40, 749] method of obtaining quantum corrections to the classical equilibrium Maxwell-Boltzmann distribution may be extended to the dissipative non-equilibrium dynamics governing the quantum Brownian motion in an external potential V(x), yielding a master equation for the Wigner distribution function W(x,p,t) in phase space (x,p). The explicit form of the master equation so obtained contains quantum correction terms up to o(h(4)) and in the classical limit, h --> 0, reduces to the classical Klein-Kramers equation. For a quantum oscillator, the method yields an evolution equation coinciding in all respects with that of Agarwal [G. S. Agarwal, Phys. Rev. A, 1971, 4, 739]. In the high dissipation limit, the master equation reduces to a semi-classical Smoluchowski equation describing non-inertial quantum diffusion in configuration space. The Wigner function formulation of quantum Brownian motion is further illustrated by finding quantum corrections to the Kramers escape rate, which, in appropriate limits, reduce to those yielded via quantum generalizations of reaction rate theory.