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Physical Review A

Angle-dependent postcollisional interaction and interference effects in resonant double photoionization of neon

Bruno Rouvellou, Stéphane Rioual, L. Avaldi, R. Camilloni, Giovanni Stefani, Giorgio Turri

Published Jan 23, 2003• 9 citations
Publisher

Abstract

The resonant double photoionization of Ne has been studied via an electron-electron coincidence experiment. A complete set of measurements was performed at different mutual angles when the photoelectron and Auger-electron pairs have nearly equal energy. The overall experimental energy resolution, narrower than the natural linewidth of the intermediate state, has allowed us to observe interference effects due to the indistinguishability of the two electrons. The observed energy and angular distribution exhibit a strong interplay of postcollisional interaction and interference effects. Calculations based on the model developed by Sheinerman and Schmidt [J. Phys. B 30, 1677 (1997)] describe the main trend of the experimental observations.

DOI
10.1103/physreva.67.012706

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The resonant double photoionization of Ne has been studied via an electron-electron coincidence experiment. A complete set of measurements was performed at different mutual angles when the photoelectron and Auger-electron pairs have nearly equal energy. The overall experimental energy resolution, narrower than the natural linewidth of the intermediate state, has allowed us to observe interference effects due to the indistinguishability of the two electrons. The observed energy and angular distribution exhibit a strong interplay of postcollisional interaction and interference effects. Calculations based on the model developed by Sheinerman and Schmidt [J. Phys. B 30, 1677 (1997)] describe the main trend of the experimental observations.
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Wave-particle duality is an inherent peculiarity of the quantum world. The double-slit experiment has been frequently used for understanding different aspects of this fundamental concept. The occurrence of interference rests on the lack of which-way information and on the absence of decoherence mechanisms, which could scramble the wave fronts. Here, we report on the observation of two-center interference in the molecular-frame photoelectron momentum distribution upon ionization of the neon dimer by a strong laser field. Postselection of ions, which are measured in coincidence with electrons, allows choosing the symmetry of the residual ion, leading to observation of both, gerade and ungerade, types of interference.
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In this paper, we shed new light on the molecular photoionization of a diatomic molecule. We will elaborate the differences and analogy between a quantum optical and light–matter interaction approach in a study of K-shell photoionization of N 2 in which the photoelectron and the subsequently emitted Auger electron are both measured in coincidence in the body fixed frame of the molecule. The two electrons form an entangled state inside a double slit. By changing the photon energy we create different types of interference in the photoelectron and the Auger electron wave.
The authors present experimental data on the autoionisation of neon and argon excited by electron impact. The energy of the incident electrons is chosen such that the two outgoing electrons in the final state have comparable energies. In this energy region state-state coherences and post-collision interactions (PCI) between the two electrons may be observed. Examples of observations of state-state interferences are presented and the effect of PCI in these experiments is discussed. A detailed analysis of the measurements is complicated due to the presence of overlapping neighbouring states.