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Journal of Physics A Mathematical and General

Dissipative quantum dynamics: solution of the generalized von Neumann equation for the damped harmonic oscillator

Martin Hensel, H. J. Korsch

Published Apr 7, 1992• 14 citations
Publisher

Abstract

A recently proposed generalized von Neumann equation describing dissipative time evolution of quantum systems is applied to a damped and driven harmonic oscillator. Utilizing Lie algebraic methods the nonlinear operator equation is solved and from this solution the behaviour of the mean value (x) is extracted, including both amplitude and phaseshift relative to the driving force. A differential equation for (x) is derived and the damping constant is identified.

DOI
10.1088/0305-4470/25/7/040

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A recently proposed generalized von Neumann equation describing dissipative time evolution of quantum systems is applied to a damped and driven harmonic oscillator. Utilizing Lie algebraic methods the nonlinear operator equation is solved and from this solution the behaviour of the mean value (x) is extracted, including both amplitude and phaseshift relative to the driving force. A differential equation for (x) is derived and the damping constant is identified.
The need for a quantum-mechanical formalism for systems with dissipation which is applicable to the radiation field of a cavity is discussed. Two methods that have been used in this connection are described. The first, which starts with the classical Newtonian equation of motion for a damped oscillator and applies the conventional formal quantization techniques, leads to an exact solution; but subsequent discussion shows that this method is invalid, the results being unacceptable from a quantum-mechanical viewpoint. The second method, which considers the interaction of two systems, the lossless oscillator and the loss mechanism, is adopted in the present article. No special model is used for the loss mechanism, but this mechanism is assumed to have a large number of densely-spaced energy states.The approximations with respect to the loss mechanism that underlie the concept of dissipation are discussed. These approximations are then applied to the analysis, and a differential equation for a coordinate operator of the harmonic oscillator is obtained which has the formal appearance of the Newtonian equation of motion for a driven damped harmonic oscillator, the driving term being an operator referring to the loss mechanism. The presence of the driving term is responsible for the difference between the present theory and that of the first method mentioned above. A solution of the differential equation for the coordinate operator is given explicitly. An examination of the physical significance of the solution shows that the driving term is responsible not only for the thermal fluctuations which are due to the loss mechanism, but also for the proper commutation relationship of the conjugate coordinates of the oscillator and for its zero-point fluctuations.A generalization of the solution to provide for a classical driving force and coupled atomic systems is given. The results are then restated in a form that refers to the loss mechanism only through the two parameters by which it is usually described---the dissipation constant and the temperature.
In this paper we use the algebraic and the invariant method to study the time-dependent damped harmonic oscillator from classical and quantum points of view. The solution of the classical equation of motion and the wavefunction solving the time-dependent Schrödinger equation are found explicitly. We show that the original time-dependent quantum-mechanical problem is completely related to the well known time-independent harmonic oscillator. In addition, we elucidate the intimate connection between the damped harmonic oscillator (DHO) and the generalized harmonic oscillator (GHO). More importantly, the evolution of the states of the DHO cannot be cyclic, in contradistinction with the states of the GHO. Explicit expressions for both the dynamical and the geometric angles and phases are deduced in the adiabatic limit. The coherent states describing the invariant-angle variables of the classical DHO are constructed; they allow us to recover the classical evolution and invariant from the quantum evolution.
We have studied quantum-mechanical behavior of a driven Morse oscillator coupled to a bath of harmonic oscillators. The purpose is to compare the quantum behavior of such a system with the classical solutions of a driven damped Morse oscillator. We start with the quantum Liouville equation, in which the Hamiltonian of the Morse oscillator is expressed in terms of generators of an su(2) Lie algebra. This algebra and the Markovian approximation allow us to derive the generalized master equation (for the reduced density matrix of the Morse oscillator), which contains level-dependent energy and phase relaxation terms. We have numerically integrated the differential equations of the matrix elements to obtain the time evolution of the reduced density matrix and the energy of the Morse oscillator. We show that the energy of the Morse oscillator in general varies with time and eventually reaches an asymptotic oscillatory state. The mean energy value of the asymptotic oscillatory state is studied as a function of the relaxation rates and laser frequency and amplitude. Vibrational distributions have also been found as functions of laser frequency and amplitude. The shape of the distribution changes gradually as laser amplitude increases; it first peaks at the ground state at a small field amplitude, then it peaks at some excited state at a large field amplitude, and for an amplitude in between it can have two maxima. This bimodal vibrational distribution reflects the bistability observed in the classical and semiclassical models. Thus bistability exists in quantum results, not as a hysteresis loop, but as a bimodal distribution. Finally, we show that as laser intensity increases, the time series of the oscillator energy evolves from regular to quasiperiodic behavior, and eventually a chaotic-looking series appears.
We obtain analytic solutions to various models of dissipation of the quantum harmonic oscillator, employing a simple method in the Wigner function Fourier transform description of the system; and study as an exemplification, the driven open quantum harmonic oscillator. The environmental models we use are based on optical master equations for the zero and finite temperature bath and whose open dynamics are described by a Lindblad master equation, and also we use the Caldeira-Leggett model for the high temperature limit, in the the under damped an the over damped case. Under the Wigner Fourier transform or chord function as it has been called, it becomes particularly simple to solve the dynamics of the open oscillator in the sense that the dynamics of the system are reduced to the application of an evolution matrix related to the damped motion of the oscillator.