Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Optics Express

Cold atom Raman spectrography using velocity-selective resonances

Fredrik K. Fatemi, Matthew L. Terraciano, Mark Bashkansky, Zachary Dutton

Published Jul 14, 2009• 4 citations
Publisher

Abstract

We have studied velocity-selective resonances in the presence of a uniform magnetic field and shown how they can be used for rapid, single-shot assessment of the ground state magnetic sublevel spectrum in a cold atomic vapor. Cold atoms are released from a magneto-optical trap in the presence of a small bias magnetic field ( approximately 300 mG) and exposed to a laser field comprised of two phase-locked counterpropagating beams connecting the two ground state hyperfine manifolds. An image of the expanded cloud shows the velocity-selected resonances as distinct features, each corresponding to specific magnetic sublevel, in a direct, intuitive manner. We demonstrate the technique with both 87Rb and 85Rb, and show the utility of the technique by optically pumping into particular magnetic sublevels. The results are shown to agree with a theoretical model, and are compared to traditional Raman spectroscopy.

DOI
10.1364/oe.17.012971

Related papers

Imaging velocity selective resonances in a magnetic field

Fredrik K. Fatemi, Matthew L. Terraciano, Zachary Dutton +1 more

We demonstrate techniques for imaging both magnetic fields and magnetic sublevel distributions using velocity-selective Raman transitions in cold 87Rb and 85Rb ensembles. When an expanding atom cloud is exposed to counterpropagating laser beams, resonant atom trajectories undergoing Raman transitions are perturbed and result in distinctive features in images of the expanded cloud. If the counterpropagating laser fields couple magnetic sublevels in different hyperfine manifolds, the images provide a spectrograph of sublevel occupation. The techniques are simple to implement and provide a useful, rapid diagnostic tool for cold atom experiments.

Journal of Modern Optics•Sep 14, 2009•0 citations

A single-shot imaging magnetometer using cold atoms

Matthew L. Terraciano, Mark Bashkansky, Fredrik K. Fatemi

We demonstrate a technique for imaging magnetic fields using velocity-selective two-photon resonances in a cold atom cloud. Freely expanding (85)Rb atoms released from a magneto-optical trap are exposed to a brief (approximately 1 ms), off-resonant, retro-reflected laser pulse in a lin-perp-lin configuration. Two-photon resonance between magnetic sublevels occurs only for atoms in narrow velocity classes dependent on the magnetic field strength. The momentum of resonant atoms is altered by the pulse, and this two-photon momentum change is easily visible after further ballistic expansion. When the momentum pulse is applied to an atom cloud with finite size, magnetic field variations across the sample result in position-dependent features in images of the expanded cloud. We demonstrate the technique by imaging magnetic field variations over approximately 5 mm with approximately 250 microm spatial resolution.

Optics Express•Aug 11, 2008•17 citations

Magnetically controlled velocity selection in a cold-atom sample using stimulated Raman transitions

Matthew L. Terraciano, Spencer E. Olson, Mark Bashkansky +2 more

We observe velocity-selective two-photon resonances in a cold atom cloud in the presence of a magnetic field. We use these resonances to demonstrate a simple magnetometer with sub-mG resolution. The technique is particularly useful for zeroing the magnetic field and does not require any additional laser frequencies than are already used for standard magneto-optical traps. We verify the effects using Faraday rotation spectroscopy.

arXiv:0801.0577•Physical Review A•Nov 29, 2007•5 citations

Pump-probe spectroscopy and velocimetry of cold atoms in a slow beam

G. Domenico, G. Mileti, P. Thomann

In this paper we report on the first purely ``pump-probe'' nonlinear laser spectroscopy results in a slow atomic beam. We have observed Raman, Rayleigh, and recoil-induced resonances (RIR) in a continuous beam of slow and cold cesium atoms extracted from a two-dimensional (2D) magneto-optical-trap (MOT) with the moving molasses technique. The RIR enabled us to measure the velocity distribution, therefore the average speed (0.6--4 m/s) and temperature (50--500 \ensuremath{\mu}K) of the atomic beam. Compared to time of flight, this technique has the advantage of being local, more sensitive in the low-velocity regime $(v<1 \mathrm{m}/\mathrm{s}),$ and it gives access to transverse velocities and temperatures. Moreover, it may be extended to measure atomic velocities in the 2D MOT source of the atomic beam.

Physical Review A•Sep 1, 2001•16 citations

Real-time local density probe for cold atoms utilizing Raman driven spin noise spectroscopy

Sayari Majumder, Bhagyashri Bidwai, Bernadette Varsha +1 more

We demonstrate a minimally perturbative detection method—Raman driven spin noise spectroscopy (RDSNS)—to directly probe the local density of a cloud of cold 39K atoms in real time. The technique relies on detecting the polarization fluctuations of a far-off resonant focused probe light passing through the atoms, driven by two coherent Raman lasers connecting adjacent Zeeman spin states. This is an easily implementable scheme with a wide-ranging applicability in detecting cold atoms. Unlike traditional fluorescence and absorption imaging techniques, this approach does not require stochastic photon scattering from trapped atoms, thereby leaving the cold cloud unperturbed. The data can be collected in MHz refresh rate, allowing for near real-time detection. We validated this technique by monitoring the strength of the RDSNS signal by varying the key parameters of the three-dimensional magneto-optical trap (MOT) and the cold atom source (two-dimensional MOT). We performed experiments to probe local densities across the cold atom cloud using our technique and compared it with the inverse Abel-transformed density profiles extracted from the fluorescence of a spherically symmetric atomic cloud and found excellent agreement. This detection protocol is particularly advantageous for probing systems that lack inherent symmetry, where the Abel transformation is inapplicable. Moreover, RDSNS imaging is suitable for extracting the dynamical properties of systems in real time.

Applied Physics Letters•Jul 28, 2025•0 citations

Technique for magnetic moment reconstruction of laser-cooled atoms using direct imaging and prospects for measuring magnetic sublevel distributions

Gehrig Carlse, Alexander Pouliot, Thomas Vacheresse +4 more

We describe a simple time-of-flight technique for measuring the magnetic moment of an optically pumped magneto-optical trap. The technique relies on free-expansion imaging of a cold atom cloud in a small magnetic field gradient without the need to detect spatial separation between magnetic sublevels. We find that the effective acceleration of the cloud can be used to characterize extreme state optical pumping. In the general case, we show that the integrated displacement of the falling cloud can be accurately modeled using rate equation simulations of magnetic sublevel populations, and knowledge of local magnetic fields, field gradients, and light intensities. The agreement between the model and the data allows the reconstruction of magnetic moments and suggests that this technique may be suitable for the measurement of population distributions over a range of optical pumping conditions.

Journal of the Optical Society of America B•Mar 18, 2020•10 citations
We have studied velocity-selective resonances in the presence of a uniform magnetic field and shown how they can be used for rapid, single-shot assessment of the ground state magnetic sublevel spectrum in a cold atomic vapor. Cold atoms are released from a magneto-optical trap in the presence of a small bias magnetic field ( approximately 300 mG) and exposed to a laser field comprised of two phase-locked counterpropagating beams connecting the two ground state hyperfine manifolds. An image of the expanded cloud shows the velocity-selected resonances as distinct features, each corresponding to specific magnetic sublevel, in a direct, intuitive manner. We demonstrate the technique with both 87Rb and 85Rb, and show the utility of the technique by optically pumping into particular magnetic sublevels. The results are shown to agree with a theoretical model, and are compared to traditional Raman spectroscopy.
We demonstrate techniques for imaging both magnetic fields and magnetic sublevel distributions using velocity-selective Raman transitions in cold 87Rb and 85Rb ensembles. When an expanding atom cloud is exposed to counterpropagating laser beams, resonant atom trajectories undergoing Raman transitions are perturbed and result in distinctive features in images of the expanded cloud. If the counterpropagating laser fields couple magnetic sublevels in different hyperfine manifolds, the images provide a spectrograph of sublevel occupation. The techniques are simple to implement and provide a useful, rapid diagnostic tool for cold atom experiments.
We demonstrate a technique for imaging magnetic fields using velocity-selective two-photon resonances in a cold atom cloud. Freely expanding (85)Rb atoms released from a magneto-optical trap are exposed to a brief (approximately 1 ms), off-resonant, retro-reflected laser pulse in a lin-perp-lin configuration. Two-photon resonance between magnetic sublevels occurs only for atoms in narrow velocity classes dependent on the magnetic field strength. The momentum of resonant atoms is altered by the pulse, and this two-photon momentum change is easily visible after further ballistic expansion. When the momentum pulse is applied to an atom cloud with finite size, magnetic field variations across the sample result in position-dependent features in images of the expanded cloud. We demonstrate the technique by imaging magnetic field variations over approximately 5 mm with approximately 250 microm spatial resolution.
In this paper we report on the first purely ``pump-probe'' nonlinear laser spectroscopy results in a slow atomic beam. We have observed Raman, Rayleigh, and recoil-induced resonances (RIR) in a continuous beam of slow and cold cesium atoms extracted from a two-dimensional (2D) magneto-optical-trap (MOT) with the moving molasses technique. The RIR enabled us to measure the velocity distribution, therefore the average speed (0.6--4 m/s) and temperature (50--500 \ensuremath{\mu}K) of the atomic beam. Compared to time of flight, this technique has the advantage of being local, more sensitive in the low-velocity regime (v<1m/s),(v<1 \mathrm{m}/\mathrm{s}),(v<1m/s), and it gives access to transverse velocities and temperatures. Moreover, it may be extended to measure atomic velocities in the 2D MOT source of the atomic beam.
We demonstrate a minimally perturbative detection method—Raman driven spin noise spectroscopy (RDSNS)—to directly probe the local density of a cloud of cold 39K atoms in real time. The technique relies on detecting the polarization fluctuations of a far-off resonant focused probe light passing through the atoms, driven by two coherent Raman lasers connecting adjacent Zeeman spin states. This is an easily implementable scheme with a wide-ranging applicability in detecting cold atoms. Unlike traditional fluorescence and absorption imaging techniques, this approach does not require stochastic photon scattering from trapped atoms, thereby leaving the cold cloud unperturbed. The data can be collected in MHz refresh rate, allowing for near real-time detection. We validated this technique by monitoring the strength of the RDSNS signal by varying the key parameters of the three-dimensional magneto-optical trap (MOT) and the cold atom source (two-dimensional MOT). We performed experiments to probe local densities across the cold atom cloud using our technique and compared it with the inverse Abel-transformed density profiles extracted from the fluorescence of a spherically symmetric atomic cloud and found excellent agreement. This detection protocol is particularly advantageous for probing systems that lack inherent symmetry, where the Abel transformation is inapplicable. Moreover, RDSNS imaging is suitable for extracting the dynamical properties of systems in real time.
We describe a simple time-of-flight technique for measuring the magnetic moment of an optically pumped magneto-optical trap. The technique relies on free-expansion imaging of a cold atom cloud in a small magnetic field gradient without the need to detect spatial separation between magnetic sublevels. We find that the effective acceleration of the cloud can be used to characterize extreme state optical pumping. In the general case, we show that the integrated displacement of the falling cloud can be accurately modeled using rate equation simulations of magnetic sublevel populations, and knowledge of local magnetic fields, field gradients, and light intensities. The agreement between the model and the data allows the reconstruction of magnetic moments and suggests that this technique may be suitable for the measurement of population distributions over a range of optical pumping conditions.