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Physical Review Letters

Doppler-Free Superradiance Experiments with Rb Atoms: Polarization Characteristics

A. Crubellier, Sylvain Liberman, P. Pillet

Published Oct 30, 1978• 55 citations
Publisher

Abstract

In order to check theoretical results obtained recently in the treatment of the superradiant emission of atoms when taking the level degeneracy into account explicitly, an experiment has been performed using a special "multiple beam" of Rb atoms. A careful study of the polarization characteristics of the emitted light has shown us several features which appear to be quite different in the superradiant emission and in the ordinary spontaneous one. An analysis is given for the few typical cases which have been observed and reported.

DOI
10.1103/physrevlett.41.1237

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Up to now, the problem of the influence of level degeneracy on superradiance has been neglected. We describe here a first approach to this problem, in the frame of "small system" quantum model, generalized to the case of a collection of atoms with two degenerate levels of angular momenta $j$ and ${j}^{\ensuremath{'}}$ connected by an electric or magnetic dipole transition. The differences between this case and the well-known case of two (nondegenerate) level atoms are of two types. The first type is due to the competition between different transitions sharing a common state: superradiant emission on a transition inhibits or initiates superradiance on transitions with smaller transition probability, depending upon which state, upper or lower, is the common one. This effect does not come from the equality of the different wavelengths and would also appear with the same states even if the degeneracy were removed; its qualitative influence on the features of the superradiant pulse can be easily estimated. The second type of differences is quite specific to level degeneracy and consists in interferences between the transitions of the collective system having the same frequency and polarization. In analogy with the description of collections of two-level atoms as spin-\textonehalf{} systems, a group-theoretical description of the considered collection of atoms is found suitable; the problem of the determination of a basis of collective states and its group-theoretical implications are discussed; in particular, it is found that the isotropic character of spontaneous emission allows us to use tensorial formalism and simplifies the formal description of the problem.

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Journal of the Physical Society of Japan•Jan 1, 1981•5 citations
In order to check theoretical results obtained recently in the treatment of the superradiant emission of atoms when taking the level degeneracy into account explicitly, an experiment has been performed using a special "multiple beam" of Rb atoms. A careful study of the polarization characteristics of the emitted light has shown us several features which appear to be quite different in the superradiant emission and in the ordinary spontaneous one. An analysis is given for the few typical cases which have been observed and reported.
Up to now, the problem of the influence of level degeneracy on superradiance has been neglected. We describe here a first approach to this problem, in the frame of "small system" quantum model, generalized to the case of a collection of atoms with two degenerate levels of angular momenta jjj and ${j}^{\ensuremath{'}}$ connected by an electric or magnetic dipole transition. The differences between this case and the well-known case of two (nondegenerate) level atoms are of two types. The first type is due to the competition between different transitions sharing a common state: superradiant emission on a transition inhibits or initiates superradiance on transitions with smaller transition probability, depending upon which state, upper or lower, is the common one. This effect does not come from the equality of the different wavelengths and would also appear with the same states even if the degeneracy were removed; its qualitative influence on the features of the superradiant pulse can be easily estimated. The second type of differences is quite specific to level degeneracy and consists in interferences between the transitions of the collective system having the same frequency and polarization. In analogy with the description of collections of two-level atoms as spin-\textonehalf{} systems, a group-theoretical description of the considered collection of atoms is found suitable; the problem of the determination of a basis of collective states and its group-theoretical implications are discussed; in particular, it is found that the isotropic character of spontaneous emission allows us to use tensorial formalism and simplifies the formal description of the problem.
In the theoretical stuqy of superradiance, the atoms or molecules are generally considered as two-level systems. However in many experimental situations, this simple assumption is not valid. It is the case, for example, in all experiments exhibiting superradiant beats [1-3]. Moreover, these beats are sometimes due to a specific property of superradiance : the existence of interferences between different atoms. Other examples of multilevel superradiance are encountered each time one observes several superradiant transitions sharing a common level [3,4]. In addition, superradiance is generally observed between degenerate levels, and it has been alreaqy shown experimentally that the level-degeneracy influences the properties of the superradiant light, in particular its polarization characteristics [5].
For pt.I see ibid., vol.18, p.3811 (1985). This paper is the second of a theoretical study of subradiance, i.e. of the cooperative inhibition of spontaneous emission by a destructive interatomic interference, a phenomenon which has recently been observed. It is devoted to the particular case of atomic systems with degenerate transitions, i.e. with several transitions of the same frequency and the same polarisation. The interatomic interference which then occurs between the different transitions is responsible, when destructive, for a new sort of subradiance. The phenomenon is studied for a few typical level configurations, using both quantum mechanical and semiclassical models. The first example concerns a four-level configuration with two transitions of the same frequency and polarisation. The other examples concern three-level configurations with a degenerate transition; in the case of the 'degenerate' cascade, new superradiant beats and subradiance effects are predicted.
For pt.II see ibid., vol.19, p.2109 (1986). This paper is the third in a theoretical study of subradiance, i.e. the cooperative inhibition of spontaneous emission by a destructive interatomic interference, a phenomenon which has recently been observed. The paper is devoted to the problem of the cooperative spontaneous emission of atomic samples with linear dimensions much smaller than the wavelength of the emitted light. The treatment, which is based on a fully quantum mechanical description of the problem, corroborates the results obtained in a semiclassical treatment by Friedberg and Hartmann (1974). Starting from a master equation describing both the cooperative spontaneous emission and the dipole-dipole interaction, a statistical treatment of the latter is introduced and the corresponding symmetry relaxation is studied. The evolution of the atoms is described in three typical cases that correspond to different sample geometries and/or atomic distributions. In one of these cases, in particular, the symmetry is first conserved and the atoms follow Dicke's predictions for a time. A 'retarded' symmetry breaking then occurs suddenly, near the zero value of the collective energy, as in Friedberg and Hartmann's calculations for a small sphere. With regard to the further evolution of the atoms in this case, which cannot be studied in a semiclassical model, it is shown that the decay rate quickly becomes much smaller than the incoherent decay rate. An unquestionable subradiance phenomenon is thus predicted in this case.
Macroscopic fluctuation of superradiance most sensitively appears as the fluctuation of the polarized photon number. This fluctuation is not much affected by unexpected variation of the exciting pulse area. In the superradiance limit the relative fiuctuation of the polarized photon number is equal to 1/3\sqrt{1/3}1/3​, and it decreases rapidly as the atomic number density is reduced below a threshold density. Such a characteristic change is attributed to a transition from the superradiant emission to the amplified spontaneous emission.