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Physical Review A

Level-degeneracy effects in superradiance theory

A. Crubellier

Published Jun 1, 1977• 22 citations
Publisher

Abstract

Up to now, the problem of the influence of level degeneracy on superradiance has been neglected. We describe here a first approach to this problem, in the frame of "small system" quantum model, generalized to the case of a collection of atoms with two degenerate levels of angular momenta $j$ and ${j}^{\ensuremath{'}}$ connected by an electric or magnetic dipole transition. The differences between this case and the well-known case of two (nondegenerate) level atoms are of two types. The first type is due to the competition between different transitions sharing a common state: superradiant emission on a transition inhibits or initiates superradiance on transitions with smaller transition probability, depending upon which state, upper or lower, is the common one. This effect does not come from the equality of the different wavelengths and would also appear with the same states even if the degeneracy were removed; its qualitative influence on the features of the superradiant pulse can be easily estimated. The second type of differences is quite specific to level degeneracy and consists in interferences between the transitions of the collective system having the same frequency and polarization. In analogy with the description of collections of two-level atoms as spin-\textonehalf{} systems, a group-theoretical description of the considered collection of atoms is found suitable; the problem of the determination of a basis of collective states and its group-theoretical implications are discussed; in particular, it is found that the isotropic character of spontaneous emission allows us to use tensorial formalism and simplifies the formal description of the problem.

DOI
10.1103/physreva.15.2430

Related papers

Level-degeneracy effects in super-radiance theory. Calculations for j=12 to j′=12 dipole transition

A. Crubellier, Marie-Gabrielle Schweighofer

We study here level-degeneracy effects in super-radiance, using the quantum "small-system" model whose interest and limitations are discussed. First, we show that this model allows one to understand the physical origin of these effects and to describe their qualitative influence on the properties of the emitted light. We also present and analyze numerical results obtained for the case of a dipole transition between two degenerate levels of angular momenta \textonehalf{}. We show that in this particular case one can define a basis of collective states which is well adapted to the invariance properties of the master equation. It is then possible to solve the master equation and to compute expectation values for the radiated field (intensity radiated with a given polarization, quantum fluctuations of this intensity) for various initial conditions and for small but already significant values of the number of individual systems. A detailed analysis of these results and a comparison with analogous calculations in the case where the degeneracy is supposed to be removed allows us to estimate the individual influence of the different types of effects (interference effects and the two sorts of competition effects, inhibition and initiation). We also compare the total intensity radiated to the intensity radiated by the same number of two (nondegenerate) level atoms. This comparison can be simply understood if one studies the partition of the population of the collective energy levels between the different states of these levels, and it appears that the most populated states are these which are able to radiate the most. Finally, it is shown how level degeneracy affects the quantum fluctuations of the intensity.

Physical Review A•Nov 1, 1978•24 citations

Superradiance and subradiance. II. Atomic systems with degenerate transitions

A. Crubellier, D Pavolini

For pt.I see ibid., vol.18, p.3811 (1985). This paper is the second of a theoretical study of subradiance, i.e. of the cooperative inhibition of spontaneous emission by a destructive interatomic interference, a phenomenon which has recently been observed. It is devoted to the particular case of atomic systems with degenerate transitions, i.e. with several transitions of the same frequency and the same polarisation. The interatomic interference which then occurs between the different transitions is responsible, when destructive, for a new sort of subradiance. The phenomenon is studied for a few typical level configurations, using both quantum mechanical and semiclassical models. The first example concerns a four-level configuration with two transitions of the same frequency and polarisation. The other examples concern three-level configurations with a degenerate transition; in the case of the 'degenerate' cascade, new superradiant beats and subradiance effects are predicted.

Journal of Physics B Atomic and Molecular Physics•Jul 28, 1986•29 citations

Coupled 'Ihmsitions in Superradiance

A. Crubellier, Catherine Bréchignac, Ph. Cahuzac +1 more

In the theoretical stuqy of superradiance, the atoms or molecules are generally considered as two-level systems. However in many experimental situations, this simple assumption is not valid. It is the case, for example, in all experiments exhibiting superradiant beats [1-3]. Moreover, these beats are sometimes due to a specific property of superradiance : the existence of interferences between different atoms. Other examples of multilevel superradiance are encountered each time one observes several superradiant transitions sharing a common level [3,4]. In addition, superradiance is generally observed between degenerate levels, and it has been alreaqy shown experimentally that the level-degeneracy influences the properties of the superradiant light, in particular its polarization characteristics [5].

•Jan 1, 1979•0 citations

Superradiance and subradiance. I. Interatomic interference and symmetry properties in three-level systems

A. Crubellier, Sylvain Liberman, D Pavolini +1 more

This paper is the first of a sequence of four papers devoted to the theoretical study of subradiance, i.e. of the cooperative inhibition of spontaneous emission, a phenomenon which has been recently observed. It is shown, in the typical example of a pencil-shaped sample of three-level atoms in the 'V' configuration (two transitions sharing a common lower level), that the system can spontaneously reach a state in which the emission in the so-called 'end-fire' superradiant field modes is cooperatively inhibited; this occurs for initially uncorrelated atoms when the initial state is a statistical mixing of the two upper states. The whole study is centered on the concept of destructive interatomic interference and it is therefore based on the symmetry properties of the collective atomic state with respect to the permutations of locally indistinguishable atoms. Semiclassical and fully quantum-mechanical models are used in turn. The obstacles to the interatomic interference and thus to subradiance are finally discussed.

Journal of Physics B Atomic and Molecular Physics•Sep 28, 1985•67 citations

Superradiance and subradiance. IV. Atomic cascades between degenerate levels

A. Crubellier, D Pavolini

For pt.III see ibid., vol.20, p.971 (1987). This paper is the fourth in a series devoted to the theoretical study of subradiance, i.e. of the cooperative inhibition of spontaneous emission. It first describes how the main results of the first paper have been developed in the general case of j to j' transitions between degenerate levels. In particular, the link between statistical mixing and symmetry properties is now derived in the general case of n-level atoms. The authors also explain how these results have allowed them to conceive the experiment which has recently provided the first evidence for the subradiance phenomenon, in the case of the 3 / 2 to 1 / 2 to 1 / 2 cascade of atomic gallium. The specific influence of the degenerate transitions which are associated with the Zeeman transitions of same polarisation is then discussed in a simplified example. Numerical simulations corresponding to the case of the experiment and to similar cases are finally presented and analysed.

Journal of Physics B Atomic and Molecular Physics•Apr 14, 1987•21 citations

Superradiance and subradiance. III. Small samples

A. Crubellier

For pt.II see ibid., vol.19, p.2109 (1986). This paper is the third in a theoretical study of subradiance, i.e. the cooperative inhibition of spontaneous emission by a destructive interatomic interference, a phenomenon which has recently been observed. The paper is devoted to the problem of the cooperative spontaneous emission of atomic samples with linear dimensions much smaller than the wavelength of the emitted light. The treatment, which is based on a fully quantum mechanical description of the problem, corroborates the results obtained in a semiclassical treatment by Friedberg and Hartmann (1974). Starting from a master equation describing both the cooperative spontaneous emission and the dipole-dipole interaction, a statistical treatment of the latter is introduced and the corresponding symmetry relaxation is studied. The evolution of the atoms is described in three typical cases that correspond to different sample geometries and/or atomic distributions. In one of these cases, in particular, the symmetry is first conserved and the atoms follow Dicke's predictions for a time. A 'retarded' symmetry breaking then occurs suddenly, near the zero value of the collective energy, as in Friedberg and Hartmann's calculations for a small sphere. With regard to the further evolution of the atoms in this case, which cannot be studied in a semiclassical model, it is shown that the decay rate quickly becomes much smaller than the incoherent decay rate. An unquestionable subradiance phenomenon is thus predicted in this case.

Journal of Physics B Atomic and Molecular Physics•Mar 14, 1987•17 citations
Up to now, the problem of the influence of level degeneracy on superradiance has been neglected. We describe here a first approach to this problem, in the frame of "small system" quantum model, generalized to the case of a collection of atoms with two degenerate levels of angular momenta jjj and j\ensuremath′{j}^{\ensuremath{'}}j\ensuremath′ connected by an electric or magnetic dipole transition. The differences between this case and the well-known case of two (nondegenerate) level atoms are of two types. The first type is due to the competition between different transitions sharing a common state: superradiant emission on a transition inhibits or initiates superradiance on transitions with smaller transition probability, depending upon which state, upper or lower, is the common one. This effect does not come from the equality of the different wavelengths and would also appear with the same states even if the degeneracy were removed; its qualitative influence on the features of the superradiant pulse can be easily estimated. The second type of differences is quite specific to level degeneracy and consists in interferences between the transitions of the collective system having the same frequency and polarization. In analogy with the description of collections of two-level atoms as spin-\textonehalf{} systems, a group-theoretical description of the considered collection of atoms is found suitable; the problem of the determination of a basis of collective states and its group-theoretical implications are discussed; in particular, it is found that the isotropic character of spontaneous emission allows us to use tensorial formalism and simplifies the formal description of the problem.
We study here level-degeneracy effects in super-radiance, using the quantum "small-system" model whose interest and limitations are discussed. First, we show that this model allows one to understand the physical origin of these effects and to describe their qualitative influence on the properties of the emitted light. We also present and analyze numerical results obtained for the case of a dipole transition between two degenerate levels of angular momenta \textonehalf{}. We show that in this particular case one can define a basis of collective states which is well adapted to the invariance properties of the master equation. It is then possible to solve the master equation and to compute expectation values for the radiated field (intensity radiated with a given polarization, quantum fluctuations of this intensity) for various initial conditions and for small but already significant values of the number of individual systems. A detailed analysis of these results and a comparison with analogous calculations in the case where the degeneracy is supposed to be removed allows us to estimate the individual influence of the different types of effects (interference effects and the two sorts of competition effects, inhibition and initiation). We also compare the total intensity radiated to the intensity radiated by the same number of two (nondegenerate) level atoms. This comparison can be simply understood if one studies the partition of the population of the collective energy levels between the different states of these levels, and it appears that the most populated states are these which are able to radiate the most. Finally, it is shown how level degeneracy affects the quantum fluctuations of the intensity.
For pt.I see ibid., vol.18, p.3811 (1985). This paper is the second of a theoretical study of subradiance, i.e. of the cooperative inhibition of spontaneous emission by a destructive interatomic interference, a phenomenon which has recently been observed. It is devoted to the particular case of atomic systems with degenerate transitions, i.e. with several transitions of the same frequency and the same polarisation. The interatomic interference which then occurs between the different transitions is responsible, when destructive, for a new sort of subradiance. The phenomenon is studied for a few typical level configurations, using both quantum mechanical and semiclassical models. The first example concerns a four-level configuration with two transitions of the same frequency and polarisation. The other examples concern three-level configurations with a degenerate transition; in the case of the 'degenerate' cascade, new superradiant beats and subradiance effects are predicted.
In the theoretical stuqy of superradiance, the atoms or molecules are generally considered as two-level systems. However in many experimental situations, this simple assumption is not valid. It is the case, for example, in all experiments exhibiting superradiant beats [1-3]. Moreover, these beats are sometimes due to a specific property of superradiance : the existence of interferences between different atoms. Other examples of multilevel superradiance are encountered each time one observes several superradiant transitions sharing a common level [3,4]. In addition, superradiance is generally observed between degenerate levels, and it has been alreaqy shown experimentally that the level-degeneracy influences the properties of the superradiant light, in particular its polarization characteristics [5].
This paper is the first of a sequence of four papers devoted to the theoretical study of subradiance, i.e. of the cooperative inhibition of spontaneous emission, a phenomenon which has been recently observed. It is shown, in the typical example of a pencil-shaped sample of three-level atoms in the 'V' configuration (two transitions sharing a common lower level), that the system can spontaneously reach a state in which the emission in the so-called 'end-fire' superradiant field modes is cooperatively inhibited; this occurs for initially uncorrelated atoms when the initial state is a statistical mixing of the two upper states. The whole study is centered on the concept of destructive interatomic interference and it is therefore based on the symmetry properties of the collective atomic state with respect to the permutations of locally indistinguishable atoms. Semiclassical and fully quantum-mechanical models are used in turn. The obstacles to the interatomic interference and thus to subradiance are finally discussed.
For pt.III see ibid., vol.20, p.971 (1987). This paper is the fourth in a series devoted to the theoretical study of subradiance, i.e. of the cooperative inhibition of spontaneous emission. It first describes how the main results of the first paper have been developed in the general case of j to j' transitions between degenerate levels. In particular, the link between statistical mixing and symmetry properties is now derived in the general case of n-level atoms. The authors also explain how these results have allowed them to conceive the experiment which has recently provided the first evidence for the subradiance phenomenon, in the case of the 3 / 2 to 1 / 2 to 1 / 2 cascade of atomic gallium. The specific influence of the degenerate transitions which are associated with the Zeeman transitions of same polarisation is then discussed in a simplified example. Numerical simulations corresponding to the case of the experiment and to similar cases are finally presented and analysed.
For pt.II see ibid., vol.19, p.2109 (1986). This paper is the third in a theoretical study of subradiance, i.e. the cooperative inhibition of spontaneous emission by a destructive interatomic interference, a phenomenon which has recently been observed. The paper is devoted to the problem of the cooperative spontaneous emission of atomic samples with linear dimensions much smaller than the wavelength of the emitted light. The treatment, which is based on a fully quantum mechanical description of the problem, corroborates the results obtained in a semiclassical treatment by Friedberg and Hartmann (1974). Starting from a master equation describing both the cooperative spontaneous emission and the dipole-dipole interaction, a statistical treatment of the latter is introduced and the corresponding symmetry relaxation is studied. The evolution of the atoms is described in three typical cases that correspond to different sample geometries and/or atomic distributions. In one of these cases, in particular, the symmetry is first conserved and the atoms follow Dicke's predictions for a time. A 'retarded' symmetry breaking then occurs suddenly, near the zero value of the collective energy, as in Friedberg and Hartmann's calculations for a small sphere. With regard to the further evolution of the atoms in this case, which cannot be studied in a semiclassical model, it is shown that the decay rate quickly becomes much smaller than the incoherent decay rate. An unquestionable subradiance phenomenon is thus predicted in this case.