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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Raman-excited spin coherences in N-V diamond

Philip Hemmer, Alexey V. Turukhin, J. A. Musser, M. S. Shahriar

Published Jan 29, 2002• 0 citations
Publisher

Abstract

Raman excited spin coherences were experimentally observed in nitrogen-vacancy (N-V) diamond color centers via nondegenerate four-wave mixing (NDFWM) and electromagnetically induced transparency (EIT). The maximal EIT-induced absorption suppression was found to be 17%, which corresponds to 70% of what is possible given the four possible geometric orientations of the N-V center in diamond. The properties of these coherences are discussed in the context of potential applications to solid-state quantum computing and high-temperature spectral hole burning memories.

DOI
10.1117/12.454042

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Raman excited spin coherences were experimentally observed in nitrogen-vacancy (N-V) diamond color centers via nondegenerate four-wave mixing (NDFWM) and electromagnetically induced transparency (EIT). The maximal EIT-induced absorption suppression was found to be 17%, which corresponds to 70% of what is possible given the four possible geometric orientations of the N-V center in diamond. The properties of these coherences are discussed in the context of potential applications to solid-state quantum computing and high-temperature spectral hole burning memories.
Raman excited spin coherences were experimentally observed in N-V diamond color centers via nondegenerate four-wave mixing (NDFWM) and electromagnetically induced transparency (EIT). The maximal absorption suppression was found to be 17%, which corresponds to 70% of what is possible given the random geometric orientation of the N-V center in diamond. In the context of quantum computing in solids, this level of transparency represents the efficient preparation of quantum bits (qubits), as well as ability to perform arbitrary single qubit rotations.
Raman-excited spin coherences were experimentally observed in nitrogen-vacancy (N-V) diamond color centers by means of nondegenerate four-wave mixing and electromagnetically induced transparency. The maximal absorption suppression was found to be 17%, which corresponds to 70% of what is possible given the random geometric orientation of the N-V center in diamond. In the context of quantum computing in solids, this level of transparency represents efficient preparation of quantum bits, as well as the ability to perform arbitrary single-quantum-bit rotations.
Summary form only given. The use of optical Raman interactions to excite spin coherences in solids has numerous potential applications, ranging from low-power nonlinear optics to high-temperature spectral hole burning memories to solid-state quantum computing. The interest in Raman excitation lies in the fact that the spin coherences can be efficiently excited and manipulated using optical laser fields yet are weakly coupled to the environment and hence have the long coherence lifetimes needed for optical memories and quantum computing. The interest in nitrogen-vacancy (N-V) color centers in diamond is its large optical oscillator strength. For memory, a large oscillator strength is important for high temperature operation. For quantum computing, the high optical transition rate enables the higher gate speed and the larger number of quantum logic operations that can be performed within the spin coherence lifetime.
Summary form only given.Optical spectral hole-burning has demonstrated the ability to achieve high-capacity, high-speed data storage. Unfortunately, widespread application of this technique has been limited by the requirement for low temperature operation. To circumvent this problem, we have been investigating the possibility of using Raman-excited spin coherences to store and recall optical data. The motivation is that optical Raman excitation allows storage densities and response times characteristic of optical hole-burning memories, but because it is based on long-lived spin coherences, it can maintain these characteristics at much higher operating temperatures. For the initial experiments we chose to use N-V color centers in diamond as the Raman hole-burning material because it is comparatively well studied.
We use electromagnetically induced transparency (EIT) to probe the narrow electron-spin resonance of nitrogen-vacancy centers in diamond. Working with a multipass diamond chip at temperatures 6--30 K, the zero-phonon absorption line (637 nm) exhibits an optical depth of 6 and inhomogeneous linewidth of $\ensuremath{\sim}30\text{ }\text{ }\mathrm{GHz}$ FWHM. Simultaneous optical excitation at two frequencies separated by the ground-state zero-field splitting (2.88 GHz) reveals EIT resonances with a contrast exceeding 6% and FWHM down to 0.4 MHz. The resonances provide an all-optical probe of external electric and magnetic fields with a projected photon-shot-noise-limited sensitivity of 0.2  V/cm/Hz0.2\text{ }\text{ }\mathrm{V}/\mathrm{cm}/\sqrt{\mathrm{Hz}}0.2  V/cm/Hz​ and 0.1  nT/Hz0.1\text{ }\text{ }\mathrm{nT}/\sqrt{\mathrm{Hz}}0.1  nT/Hz​, respectively. Operation of a prototype diamond-EIT magnetometer measures a noise floor of $\ensuremath{\lesssim}1\text{ }\text{ }\mathrm{nT}/\sqrt{\mathrm{Hz}}$ for frequencies above 10 Hz and Allan deviation of $1.3\ifmmode\pm\else\textpm\fi{}1.1\text{ }\text{ }\mathrm{nT}$ for 100 s intervals. The results demonstrate the potential of diamond-EIT devices for applications ranging from quantum-optical memory to precision measurement and tests of fundamental physics.
The nitrogen-vacancy center in diamond exhibits a zero-phonon transition art 637 nm that has been assigned as an A→E transition at a site with trigonal symmetry.1 Paramagnetic resonance studies revealed a triplet feature that was originally assigned to an excited state.2 More recently, it was argued that the triplet signal actually arose from the ground state,3,4We employ a new method of ultra-high-resolution nearly degenerate four-wave-mixing (NDFWM) spectroscopy, as well as persistent hole burning and electron paramagnetic resonance, to measure the metastable spin singlet excited-state lifetime and the g round-state spin-lattice relaxation time and also to prove that the ground state is indeed a triplet.