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Physical Review A

Two-photon-state generation via four-wave mixing in optical fibers

Jun Chen, Xiaoying Li, Prem Kumar

Published Sep 2, 2005• 99 citations
Publisher

Abstract

A quantum theory of two-photon-state generation via four-wave mixing in optical fibers is studied, with emphasis on the case where the pump is a classical, narrow (picosecond-duration) pulse. One of the experiments performed in our lab is discussed and analyzed. Numerical predictions from the theory are shown to be in good agreement with the experimental results.

DOI
10.1103/physreva.72.033801

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A quantum theory of two-photon-state generation via four-wave mixing in optical fibers is studied, with emphasis on the case where the pump is a classical, narrow (picosecond-duration) pulse. One of the experiments performed in our lab is discussed and analyzed. Numerical predictions from the theory are shown to be in good agreement with the experimental results.
We present a quantum theory for generating two-photon states by means of four-wave mixing in optical fiber. We start with an interaction Hamiltonian that can correctly describe all nonlinear interactions among the four waves present in the fiber, namely, the frequency non-degenerate pumps, signal, and idler, including the terms responsible for self-phase modulation (SPM), cross-phase modulation (XPM), and four-photon scattering (FPS). The exact form of this Hamiltonian is obtained through comparison between the classical and quantum equations of motion. The two-photon state is then calculated by means of first-order perturbation theory. It turns out that only the FPM and the pump SPM terms contribute to the formation of the two-photon state. The entangled nature of this state is verified in a coincidence counting experiment. The results of the theoretical calculation agree well with experimental data.
We develop a theoretical analysis of four-wave mixing used to generate photon pairs useful for quantum information processing. The analysis applies to a single mode microstructured fibre pumped by an ultra-short coherent pulse in the normal dispersion region. Given the values of the optical propagation constant inside the fibre, we can estimate the created number of photon pairs per pulse, their central wavelength and their respective bandwidth. We use the experimental results from a picosecond source of correlated photon pairs using a micro-structured fibre to validate the model. The fibre is pumped in the normal dispersion regime at 708 nm and phase matching is satisfied for widely spaced parametric wavelengths of 586 and 894 nm. We measure the number of photons per pulse using a loss-independent coincidence scheme and compare the results with the theoretical expectation. We show a good agreement between the theoretical expectations and the experimental results for various fibre lengths and pump powers.
Four-wave mixing in optical fibers has been proven to have many applications within processing of classical optical signals. In addition, recent developments in multimode fibers have made it possible to achieve the necessary phase-matching for efficient four-wave mixing over a very wide bandwidth. Thus, the combination of multimode fiber optics and four-wave mixing is very attractive for various applications. This is especially the case for applications in quantum communication, for example in photon-pair generation. This is the subject of this work, where we discuss the impact of fluctuations in core radius on the quality of the heralded single-photon states and demonstrate experimental results of intermodal spontaneous four-wave mixing for photon-pair generation.
We study both experimentally and theoretically the generation of photon pairs by spontaneous four-wave mixing (SFWM) in standard birefringent optical fibers. The ability to produce a range of two-photon spectral states, from highly correlated (entangled) to completely factorable, by means of cross-polarized birefringent phase matching, is explored. A simple model is developed to predict the spectral state of the photon pair which shows how this can be adjusted by choosing the appropriate pump bandwidth, fiber length and birefringence. Spontaneous Raman scattering is modeled to determine the tradeoff between SFWM and background Raman noise, and the predicted results are shown to agree with experimental data.
Spectral correlation of photon pairs generated in dispersion shifted fiber by a pulsed pump is theoretically analyzed and experimentally investigated. We first calculate the spectral function of photon pairs according to the deduced two-photon state generated by spontaneous four wave mixing under the assumptions close to the real experimental conditions. We then experimentally study the spectral property of the signal and idler photon pairs generated in optical fiber by photon correlation measurements, and the experimental results agree with the calculation. The investigation is useful for developing fiber-based sources of entangled photon pairs and for studying multi-photon quantum interference with multiple photon pairs.
We present a general quantum theory capable of describing photon statistics under the combined effects of four-wave mixing and Raman scattering inside optical fibers. Our theory is vectorial in nature and includes all polarization effects. Our analysis shows that spontaneous Raman scattering degrades the pair correlation in all cases but the extent of degradation depends on the pumping configuration employed. In a single-pump configuration, photon pairs can be created with polarization either parallel or orthogonal to the pump. Our results show that the orthogonal configuration can improve the extent of quantum correlation considerably over a broad bandwidth. In the case of a dual-pump configuration, we show that imbalance of two pump powers can be used to improve the quality of photon pairs. We show that orthogonally polarized pumps can generate photon pairs automatically in a polarization-entangled state. In particular, orthogonal pumping with circular polarizations produces such an entangled state with relatively high quality. We also quantify the quality of polarization entanglement as well as energy-time entanglement constructed using correlated photon pairs.