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Conference on Lasers and Electro-Optics

Quantum-state-preserving optical pulse reshaping and multiplexing by four-wave mixing in a fiber

Colin J. McKinstrie, Lasse Mejling, M. G. Raymer, Karsten K. Rottwitt

Published Jan 1, 2012• 0 citations
Publisher

Abstract

Nondegenerate four-wave mixing driven by two pulsed pumps transfers the quantum state of an input signal pulse to an output idler pulse, which is a frequency-translated and reshaped version of the signal. By varying the pump shapes appropriately, one can connect signal and idler pulses with arbitrary durations and shapes. This process enables a variety of functions required by quantum information networks.

DOI
10.1364/cleo_at.2012.jw4a.117

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Nondegenerate four-wave mixing driven by two pulsed pumps transfers the quantum state of an input signal pulse to an output idler pulse, which is a frequency-converted and reshaped version of the signal. By varying the pump shapes appropriately, one can connect signal and idler pulses with arbitrary durations and shapes. This process enables a variety of functions required by quantum information networks.

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It must be pointed out here that in a conventional wavelength-divisionmultiplexed classical optical communication line, one strives to suppress the fourphoton or four-wave mixing process, which otherwise causes cross talk between the wavelength channels and sets limits on the total data capacity of the communication line. In our experiment, the four-photon mixing takes place in a nonlinear-fiber Sagnac interferometer (NFSI), which we previously used to generate quantum-correlated twin beams in the fiber.5 The pump is a mode-locked train of ~3-ps-long pulses. The pulsed operation serves two important purposes: the NFSI amplifier can be operated at low average powers and the production of the signal/ idler fluorescence photons is confined to well-defined temporal windows, allowing use of a gated detection scheme to increase the signal-to-noise ratio. To measure the nonclassical (i.e., quantum) correlations between the signal and the idler photons, one must effectively suppress the pump photons from reaching the detectors. Since a typical pump pulse contains ~108 photons and we are interested in detecting ~0.01 signal (idler) photons/pulse, a pump-to-signal (idler) rejection ratio in excess of 100 dB is required. We achieved this specification by sending the fluorescence photons through a free-space double-grating spectral filter that separates the signal and idler photons from each other and from the pump photons not rejected by the NFSI. To demonstrate the quantum nature of the four-photon scattering at the single photon level, we assembled a photonFigure 1.C oincidence rates as a function of the single-photon rates in two different cases: signalidler fluorescence produced by a pump pulse (diamonds) and signal-idler fluorescence produced by two consecutive pump pulses (triangles). 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Nondegenerate four-wave mixing driven by two pulsed pumps transfers the quantum state of an input signal pulse to an output idler pulse, which is a frequency-translated and reshaped version of the signal. By varying the pump shapes appropriately, one can connect signal and idler pulses with arbitrary durations and shapes. This process enables a variety of functions required by quantum information networks.
Q uantum entanglement refers to the nonclassical dependency of physically separated quantum systems. It is an essential resource that must be freely available for implementing many of the novel functions of quantum information processing, such as database searching, clock synchronization, teleportation, computing and cryptography.1 The efficient generation and transmission of quantum entanglement is therefore of prime importance. With the ubiquitous standard optical fiber serving as the transmission medium and the widespread availability of efficient active and passive fiber devices, technological synergy between the generation and propagation components of the overall quantum network can be achieved by deploying sources of entanglement that rely on the nonlinearity of the fiber itself. Such fiber-based sources of quantum entanglement would also have the advantage of modal purity over their crystal counterparts,2,3 which is very important for realizing complex networks that involve many quantum operations. In our quest to develop fiber-based devices for quantum information processing, we have recently demonstrated an allfiber source of quantum-correlated photon pairs.4 The operating physical mechanism in this source is nondegenerate fourphoton mixing, wherein two pump photons scatter through the Kerr nonlinearity of the fiber to create simultaneous signal and idler photons. Our experiment is conducted near the zero-dispersion wavelength of standard dispersion-shifted fiber, where such scattering is enhanced owing to phase matching of the photon wave functions. It must be pointed out here that in a conventional wavelength-divisionmultiplexed classical optical communication line, one strives to suppress the fourphoton or four-wave mixing process, which otherwise causes cross talk between the wavelength channels and sets limits on the total data capacity of the communication line. In our experiment, the four-photon mixing takes place in a nonlinear-fiber Sagnac interferometer (NFSI), which we previously used to generate quantum-correlated twin beams in the fiber.5 The pump is a mode-locked train of ~3-ps-long pulses. The pulsed operation serves two important purposes: the NFSI amplifier can be operated at low average powers and the production of the signal/ idler fluorescence photons is confined to well-defined temporal windows, allowing use of a gated detection scheme to increase the signal-to-noise ratio. To measure the nonclassical (i.e., quantum) correlations between the signal and the idler photons, one must effectively suppress the pump photons from reaching the detectors. Since a typical pump pulse contains ~108 photons and we are interested in detecting ~0.01 signal (idler) photons/pulse, a pump-to-signal (idler) rejection ratio in excess of 100 dB is required. We achieved this specification by sending the fluorescence photons through a free-space double-grating spectral filter that separates the signal and idler photons from each other and from the pump photons not rejected by the NFSI. To demonstrate the quantum nature of the four-photon scattering at the single photon level, we assembled a photonFigure 1.C oincidence rates as a function of the single-photon rates in two different cases: signalidler fluorescence produced by a pump pulse (diamonds) and signal-idler fluorescence produced by two consecutive pump pulses (triangles). T he line represents the calculated accidental counts. T he inset shows a plot of the detected idler photons as a function of the injected pump photons (hollow circles). A second-order polynomial is shown to fit the experimental data. T he contributions of the dark counts, linear scattering and quadratic scattering are plotted separately as well. counting apparatus for detecting the signal and idler photons in coincidence. This apparatus is based on commercial InGaAs avalanche photodiodes operating in the gated Geiger mode.4 In the inset in Fig. 1, we show the number of scattered photons, NS, versus the number of pump photons, NP, injected into the NFSI. We fit the experimental data with a second-order polynomial fit, including the number of dark counts during the gate interval, ND. The fit clearly shows that the quadratic scattering ( ∝NP) in the fiber can dominate over the residual linear scattering ( ∝NP) of the pump, owing to imperfect filtering. The main body of Fig. 1 shows the coincidence-counting results. The diamonds represent the rate of coincidence counts versus the rate of the signal (idler) photons generated during the same pump pulse. The triangles represent the measured coincidence rate versus the signalphoton count rate when the signal is delayed with respect to the idler by one pulse period. For two independent photon sources, each with a count rate RS <<1, the accidental coincidence rate RC is given by RC = RS 2, regardless of the photon statistics of the sources. This quadratic relation is plotted as the solid line in Fig. 1, which fits the delayed-coincidence data (triangles) very well. These measurements show that while the fluorescence photons produced by the adjacent pump pulses are independent, those coming from the same pump pulse show a strong correlation, which is a signature of their non-classical behavior. This work was supported by the Department of Defense Multidisciplinary University Research Initiative program administered by the Army Research Office under Grants DAAD19-00-1-0177 and DAAD19-00-1-0469, and by the U.S. Office of Naval Research under Grant N00014-91-J-1268.
This thesis deals with applications of nonlinear four-wave mixing in the context of optical quantum information science. By enabling diverse functionalities such as single-photon generation, temporal shaping, and frequency conversion, four-wave mixing is a highly versatile tool for processing optical quantum information. The first part addresses the use of spontaneous four-wave mixing for generating entangled photon pairs with the particular property that the photons are uncorrelated in time and frequency. Two schemes are proposed to achieve this. The first proposal relies on a gradually varying interaction between two orthogonally polarized pump pulses in a birefringent waveguide. It is shown that, if the two pump pulses undergo a complete walk-through, the two generated photons emerge in orthogonal polarizations with uncorrelated- and tailorable time-frequency distributions. The second proposal deals with photon-pair generation in a microring resonator. In this setting, it is shown that a dual-pulse configuration can be used to excite- and subsequently de-excite the resonator on a sub-lifetime timescale. This turns out to strongly diminish time-frequency correlations. The second part considers the four-wave-mixing process Bragg scattering, which is known to enable noise-free frequency conversion. The Bragg-scattering process treated here, which occurs in a birefringent waveguide, is shown to allow for shape-preserving and strongly uni-directional conversion with a large acceptance bandwidth.
Photon pair states and multiple-photon squeezed states have many applications in quantum information science. In this paper, Green functions are derived for spontaneous four-wave mixing in the low- and high-gain regimes. Nondegenerate four-wave mixing in a strongly-birefringent medium generates signal and idler photons that are associated with only one pair of temporal (Schmidt) modes, for a wide range of pump powers and arbitrary pump shapes. The Schmidt coefficients (expected photon numbers) depend sensitively on the pump powers, and the Schmidt functions (shapes of the photon wavepackets) depend sensitively on the pump powers and shapes, which can be controlled.