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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Toward the manipulation of a single spin in an AlGaAs/GaAs single-electron transistor

Sami Amasha, Kenneth MacLean, Dominik M. Zumbühl, Iuliana P. Radu, M. A. Kastner, Micah P. Hanson, Arthur C. Gossard

Published May 5, 2006• 6 citations
Publisher

Abstract

Single-electron transistors (SETs) are attractive candidates for spin qubits. An AlGaAs/GaAs SET consists of a confined two-dimensional droplet of electrons, called an artificial atom or quantum dot, coupled by tunnel barriers to two conducting leads. Controlling the voltages on the lithographic gates that define the quantum dot allows us to confine a single electron in the dot, as well as to adjust the tunnel barriers to the leads. By applying a magnetic field, we can split the spin-up and spin-down states of the electron by an energy |g|μBB; the goal is to utilize coherent superpositions of these spin states to construct a qubit. We will discuss our attempts to observe electron spin resonance (ESR) in this system by applying magnetic fields at microwave frequencies. Observation of ESR would demonstrate that we can manipulate a single spin and allow us to measure the decoherence time T2*.

DOI
10.1117/12.665548

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Single-electron transistors (SETs) are attractive candidates for spin qubits. An AlGaAs/GaAs SET consists of a confined two-dimensional droplet of electrons, called an artificial atom or quantum dot, coupled by tunnel barriers to two conducting leads. Controlling the voltages on the lithographic gates that define the quantum dot allows us to confine a single electron in the dot, as well as to adjust the tunnel barriers to the leads. By applying a magnetic field, we can split the spin-up and spin-down states of the electron by an energy |g|μBB; the goal is to utilize coherent superpositions of these spin states to construct a qubit. We will discuss our attempts to observe electron spin resonance (ESR) in this system by applying magnetic fields at microwave frequencies. Observation of ESR would demonstrate that we can manipulate a single spin and allow us to measure the decoherence time T2*.
By coupling a radio-frequency single-electron transistor (RF-SET) to a quantum dot (QD) in a GaAs/AlGaAs heterostructure, we have succeeded in detecting the tunneling of individual electrons on and off the QD on time scales as short as one microsecond. Using charge detection to probe the state of the QD allows us to nearly isolate the dot from its leads, thereby minimizing decoherence-inducing effects of the environment. We have extended these charge detection techniques to double quantum dots (DQDs) that can simultaneously be used to characterize the backaction of the RF-SET. The combined RF-SET/DQD system is well-suited to the development of charge- or spin-based quantum bits, and to investigation of the quantum measurement problem.
We report on our recent progress in applying semiconductor quantum dots for spin-based quantum computation, as proposed by Loss and DiVincenzo (1998 Phys. Rev. A 57 120). For the purpose of single-electron spin resonance, we study different types of single quantum dot devices that are designed for the generation of a local ac magnetic field in the vicinity of the dot. We observe photon-assisted tunnelling as well as pumping due to the ac voltage induced by the ac current driven through a wire in the vicinity of the dot, but no evidence for ESR so far. Analogue concepts for a double quantum dot and the hydrogen molecule are discussed in detail. Our experimental results in laterally coupled vertical double quantum dot device show that the Heitler–London model forms a good approximation of the two-electron wavefunction. The exchange coupling constant J is estimated. The relevance of this system for two-qubit gates, in particular the SWAP operation, is discussed. Density functional calculations reveal the importance of the gate electrode geometry in lateral quantum dots for the tunability of J in realistic two-qubit gates.
Connecting quantum processors over long distances using photon qubits would enable more complex quantum computing architectures and quantum networks. Recently a protocol to transfer a quantum state from a photonic qubit to a singlet-triplet spin qubit in GaAs/AlGaAs heterostructure has been theoretically demonstrated. In practice, the coherent transfer is facilitated by a hybrid device where a GaAs/AlGaAs gate-defined quantum dot (GDQD) is tunnel coupled to a self-assembled quantum dot (SAQD), in which a conversion between a photon state and a spin state takes place. This work addressed the three requirements of the optical-interface devices based on tunnel coupling between the GDQD and the SAQD: (i) a properly designed GaAs/AlGaAs heterostructure where the two-dimensional electron gas (2DEG) can be electrically tuned into resonance with the InAs SAQD; (ii) high-mobility 2DEG to form and operate a GDQD; (iii) precise alignment between the SAQD and the GDQD. It is proven that the InAs SAQD can be tuned to be charged, discharged, and resonant with the 2DEG by applying a local electric field.
We consider a single electron in a 1D quantum dot with a static slanting Zeeman field. By combining the spin and orbital degrees of freedom of the electron, an effective quantum two-level (qubit) system is defined. This pseudospin can be coherently manipulated by the voltage applied to the gate electrodes, without the need for an external time-dependent magnetic field or spin-orbit coupling. Single-qubit rotations and the controlled-NOT operation can be realized. We estimated the relaxation (T1) and coherence (T2) times and the (tunable) quality factor. This scheme implies important experimental advantages for single electron spin control.
A two-level quantum system is the building block of a quantum computer. This pair of quantum states defines the computational unit of a quantum computer, and it is called a quantum bit or qubit in analogy to the bit that is the binary unit of a classical computer. The spin of a single electron naturally defines such a two-level quantum system. A quantum dot can be tuned to the single-electron regime, and an array of singly occupied quantum dots provides a multi-qubit register. This thesis describes the multielectron encoding of a spin qubit using a pair or a trio of quantum dots, and it analyzes the coherence properties and manipulation protocols of this system. The singlet-triplet qubit, coded using the singlet state and the spinless triplet state of a pair of singly occupied quantum dots, can be controlled all electrically when applying voltages to gates close to the quantum dot structure. Rapid, subnanosecond modifications of the double quantum dot's charge configuration have been realized successfully. A small magnetic field gradient across the double quantum dot enables universal qubit control. Two modifications of the normal singlet-triplet encoding are introduced. (1) The six-electron configuration of a double quantum dot encodes a singlet-triplet qubit in the same way as for the two-electron double quantum dot. Two electrons at each quantum dot are irrelevant for the qubit manipulations because they are paired in a singlet state; the remaining two electrons encode the qubit. The qubit's wave function is immune to charge noise at moderate out-of-plane magnetic fields. (2) A singlet-triplet qubit encoded using two quantum dots of different sizes has an orbital state degeneracy of the singlet state and the spinless triplet state at finite out-of-plane magnetic fields. Spin-orbit interactions lift this state degeneracy, while the magnitude of the state coupling is determined by the size difference of the QDs. This setup enables the manipulations of singlet-triplet qubits without the need for magnetic field gradients. Finally, two-qubit gates between singlet-triplet qubits are proposed that use mediated exchange interactions via one quantum state. These operations are well controlled and highly noise insensitive. Orbital interactions alone can control spin qubits coded in a three electron Hilbert space. For example, the exchange-only qubit is encoded using three singly occupied quantum dots. The exchange interactions of two quantum dot pairs need to be modified to manipulate this qubit. The noise sensitivity of the exchange-only qubit is discussed. Alternatively, a three-electron qubit at a double quantum dot can be operated when single electrons are transferred between the quantum dots. Fast, subnanosecond manipulations of the double quantum dot's charge configuration are required to realize single-qubit gates. A novel two-qubit pulse gate for the three-electron double quantum dot qubit is proposed.
The spin states of electrons and holes confined in InAs quantum dot molecules have recently come to fore as a promising system for the storage or manipulation of quantum information. We describe here a feasible scheme for complete quantum optical control of two electron spin qubits in two vertically-stacked singly-charged InAs quantum dots coupled by coherent electron tunneling. With an applied magnetic field transverse to the growth direction, we construct a universal set of gates that corresponds to the possible Raman transitions between the spin states. We detail the procedure to decompose a given two-qubit unitary operation, so as to realize it with a successive application of up to 8 of these gates. We give the pulse shapes for the laser pulses used to implement this universal set of gates and demonstrate the realization of the two-qubit quantum Fourier transform with fidelity of 0.881 and duration of 414 ps. Our proposal therefore offers an accessible path to universal computation in quantum dot molecules and points to the advantages of using pulse shaping incoherent manipulation of optically active quantum dots to mitigate the negative effects of unintended dynamics and spontaneous emission.