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Conference on Lasers and Electro-Optics

Cavity-enhanced spectroscopy using pump-probe differencing

Glenn de Vine, J. D. Close, David E. McClelland, M. Gray

Published Jan 1, 2005• 0 citations
Publisher

Abstract

We present a relatively simple experimental technique enabling mechanical-noise free, cavity-enhanced spectroscopic measurements of an atomic transition and its hyperfine structure. We demonstrate this technique at 532 nm with an iodine vapour cell.
DOI
10.1109/cleo.2005.202356

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We have shown earlier that hyperfine spectroscopy in a vapor cell using co-propagating pump-probe beams has many advantages over the usual technique of saturated-absorption spectroscopy using counter-propagating beams. The main advantages are the absence of crossover resonances, the appearance of the signal on a flat (Doppler-free) background, and the higher signal-to-noise ratio of the primary peaks. Interaction with non-zero-velocity atoms causes additional peaks, but only one of them appears within the primary spectrum. We first illustrate the advantages of this technique for high-resolution spectroscopy by studying the D2D_2D2​ line of Rb. We then use an acousto-optic modulator (AOM) for frequency calibration to make precise hyperfine-interval measurements in the first excited P3/2P_{3/2}P3/2​ state of 85,87^{85,87}85,87Rb and 133^{133}133Cs.
We present an experimental technique that permits mechanical-noise-free, cavity-enhanced frequency measurements of an atomic transition and its hyperfine structure. We employ the 532-nm frequency-doubled output from a Nd:YAG laser and an iodine vapor cell. The cell is placed in a folded ring cavity (FRC) with counterpropagating pump and probe beams. The FRC is locked with the Pound-Drever-Hall technique. Mechanical noise is rejected by differencing the pump and probe signals. In addition, this differenced error signal provides a sensitive measure of differential nonlinearity within the FRC.
Vapour-cell spectroscopy is widely used for the frequency stabilisation of diode lasers relative to specific atomic transitions - a technique essential in cold atom and ion trapping experiments. Two laser beams, tuned to different frequencies, can be overlapped on the same spatial path as an aid to compactness; this method also enhances the resulting spectroscopic signal via optical pumping effects, yielding an increase in the sensitivity of spectroscopically-generated laser stabilisation signals. Doppler-free locking features become visible over a frequency range several hundred MHz wider than for standard saturated absorption spectroscopy. Herein we present the measured Doppler-free spectroscopy signals from an atomic vapour cell as a function of both laser frequencies, showing experimental data that covers the full, 2D parameter space associated with dual-frequency spectroscopy. We consider how dual-frequency spectroscopy could be used for enhanced frequency-stabilisation of one laser, or alternatively to frequency-stabilise two lasers simultaneously, and analyse the likely performance of such stabilisation methods based on our experimental results. We discuss the underlying physical mechanism of the technique and show that a simple rate-equation model successfully predicts the key qualitative features of our results