Some new experiments leading to observation of multi-photon entanglement will be presented. They utilize multi-pair emissions in a down-conversion crystal. In configurations that avoid interferometric overlaps this leads to a high visibility multi-photon interference. General theoretical results concerning the influence of photon statistics and distinguishability on the interference effects in such experiments is be given. Methods of detection of entanglement in multi-qubit systems, via Bell's theorem and a non-linear generalization of entanglement witnesses, will be presented. Finally it will be shown that multi-photon entanglement can be applied to reduce of communication complexity of some computational tasks.
Some new experiments leading to observation of multi-photon entanglement will be presented. They utilize multi-pair emissions in a down-conversion crystal. In configurations that avoid interferometric overlaps this leads to a high visibility multi-photon interference. General theoretical results concerning the influence of photon statistics and distinguishability on the interference effects in such experiments is be given. Methods of detection of entanglement in multi-qubit systems, via Bell's theorem and a non-linear generalization of entanglement witnesses, will be presented. Finally it will be shown that multi-photon entanglement can be applied to reduce of communication complexity of some computational tasks.
A number of recent interference experiments involving multiple photons are reviewed. These experiments include generalized photon bunching effects, generalized Hong-Ou-Mandel interference effects and multi-photon interferometry for demonstrations of multi-photon de Broglie wavelength. The multi-photon states used in these experiments are from two pairs of photons in parametric down-conversion. We find that the size of the interference effect in these experiments, characterized by the visibility of the interference pattern, is governed by the degree of distinguishability among different pairs of photons. Based on this discovery, we generalize the concept of multi-photon temporal distinguishability and relate it to a number of multi-photon interference effects. Finally, we make an attempt to interpret the coherence theory by multi-photon interference via the concept of temporal distinguishability of photons.
Entangled photons are at the heart of experimental quantum physics. They were used for the first fundamental tests of quantum theory, and became a basic building block for many novel quantum protocols, such as quantum cryptography, dense coding or teleportation. Therefore, the efficient generation of entangled photons, as well as their distribution and accurate analysis are of paramount importance, particularly with regard to the practicability of many applications of quantum communication. This thesis deals largely with the problem of efficient generation of photonic entanglement with the principal aim of developing a bright source of polarization-entangled photon pairs, which meets the requirements for reliable and economic operation of quantum communication prototypes and demonstrators. Our approach uses a correlated photon-pair emission in nonlinear process of spontaneous parametric down-conversion pumped by light coming from a compact and cheap blue laser diode. Two alternative source configurations are examined within the thesis. The first makes use of a well established concept of degenerate non-collinear emission from a single type-II nonlinear crystal and the second relies on a novel method where the emissions from two adjacent type-I phase-matched nonlinear crystals operated in collinear non-degenerate regime are coherently overlapped. The latter approach showed to be more effective, yielding a total detected rate of almost 10^6 pairs/s at >98 % quantum interference visibility of polarization correlations. This performance, together with the almost free of alignment operation of the system, suggest that it is an especially promising candidate for many future practical applications, including quantum cryptography, detector calibration or use in undergraduate lab courses. The second issue addressed within the thesis is the simplification and practical implementation of quantum-assisted solutions to multiparty communication tasks. While the recent rapid progress in the development of bright entangled photon-pair sources has been followed with ample experimental reports on two-party quantum communication tasks, the practical implementations of tasks for more than two parties have been held back, so far. This is mainly due to the requirement of multiparty entangled states, which are very difficult to be produced with current methods and moreover suffer from a high noise. We show that entanglement is not the only non-classical resource endowing the quantum multiparty information processing its power. Instead, only the sequential communication and transformation of a single qubit can be sufficient to accomplish certain tasks. This we prove for two distinct communication tasks, secret sharing and communication complexity. Whereas the goal of the first is to split a cryptographic key among several parties in a way that its reconstruction requires their collaboration, the latter aims at reducing the amount of communication during distributed computational tasks. Importantly, our qubit-assisted solutions to the problems are feasible with state-of-the-art technology. This we clearly demonstrate in the laboratory implementation for 6 and 5 parties, respectively, which is to the best of our knowledge the highest number of actively performing parties in a quantum protocol ever implemented. Thus, by successfully solving and implementing a cryptographic task as well as a task originating in computer science, we clearly illustrate the potential to introduce multiparty communication problems into real life.
Since the awareness of entanglement was raised by Einstein, Podolski, Rosen and Schrödinger in the beginning of the last century, it took almost 55 years until entanglement entered the laboratories as a new resource. Meanwhile, entangled states of various quantum systems have been investigated. Sofar, their biggest variety was observed in photonic qubit systems. Thereby, the setups of today's experiments on multi-photon entanglement can all be structured in the following way: They consist of a photon source, a linear optics network by which the photons are processed and the conditional detection of the photons at the output of the network. In this thesis, two new linear optics networks are introduced and their application for several quantum information tasks is presented. The workhorse of multi-photon quantum information, spontaneous parametric down conversion, is used in different configurations to provide the input states for the networks. The first network is a new design of a controlled phase gate which is particularly interesting for applications in multi-photon experiments as it constitutes an improvement of former realizations with respect to stability and reliability. This is explicitly demonstrated by employing the gate in four-photon experiments. In this context, a teleportation and entanglement swapping protocol is performed in which all four Bell states are distinguished by means of the phase gate. A similar type of measurement applied to the subsystem parts of two copies of a quantum state, allows further the direct estimation of the state's entanglement in terms of its concurrence. Finally, starting from two Bell states, the controlled phase gate is applied for the observation of a four photon cluster state. The analysis of the results focuses on measurement based quantum computation, the main usage of cluster states. The second network, fed with the second order emission of non-collinear type II spontaneous parametric down conversion, constitutes a tunable source of a whole family of states. Up to now the observation of one particular state required one individually tailored setup. With the network introduced here many different states can be obtained within the same arrangement by tuning a single, easily accessible experimental parameter. These states exhibit many useful properties and play a central role in several applications of quantum information. Here, they are used for the solution of a four-player quantum Minority game. It is shown that, by employing four-qubit entanglement, the quantum version of the game clearly outperforms its classical counterpart. Experimental data obtained with both networks are utilized to demonstrate a new method for the experimental discrimination of different multi-partite entangled states. Although theoretical classifications of four-qubit entangled states exist, sofar there was no experimental tool to easily assign an observed state to the one or the other class. The new tool presented here is based on operators which are formed by the correlations between local measurement settings that are typical for the respective quantum state.
Progress in multiphoton interferometry allows us now to observe even six-photon interference of a very high contrast. Also, it is possible to observe interference of two photons originating from truly independent sources. Non-classical effects may violate Bell inequalities, or reveal quantum non-separability. Methods of producing non-classical states of few photons, and the detection of entanglement via Bell inequalities, or via nor-separability criteria will be presented. Implications of violations of Bell inequalities will be discussed, with a special stress on over-interpretations of this fact.
Entanglement lies at the heart of quantum mechanics and challenged the intuition of physicists ever since it was discovered. At the same time, it is a powerful tool that serves as a key resource for quantum communication and quantum computation schemes. Many of these applications rely on multiparticle entanglement, whose description, generation and manipulation became therefore a very active field in theoretical and experimental quantum information science. The goals are here to classify and understand the different types of entanglement, to find new applications and to control and analyze the quantum states experimentally. In this thesis, the experimental observation and analysis of two different types of four-photon polarization entangled states is presented: The cluster state and the symmetric Dicke state with two excitations. For this purpose, experimental setups based on spontaneous parametric down conversion and linear optics with conditional detection were designed. They allowed to observe the cluster state with a fidelity of 74.1 % and the symmetric Dicke state with a fidelity of 84.4 %. The cluster state experiment included the development of a new instrument that is of interest for linear optics quantum logic in general: A probabilistic controlled phase gate that is, due to the simplification of a previous approach, highly stable and can actually be used in multiphoton experiments. The quality of the gate is evaluated by analyzing its entangling capability and by performing full process tomography. The achieved results demonstrate that this device is well suited for implementation in various multiphoton quantum information protocols. In order to study the observed quantum states, efficient analysis tools are introduced. It was possible to verify that essential properties of the ideal states are indeed reproduced in the experiment, among others, the presence of genuine four-partite entanglement. A particular focus is put on the behavior of the states under projective measurements and photon loss. Several new insights in their entanglement structure are revealed and verified experimentally. We further demonstrate properties that are characteristic for the entanglement classes of the states. These can be used to infer the applicability of the observed states for certain distributed quantum communication applications. The presented experiments are generic for the design of setups to observe cluster- and symmetric Dicke states with a higher number of photons. Furthermore, also the efficient non-tomographic methods for state analysis we employ can directly be generalized to experiments with higher qubit numbers, where the reduction of the experimental effort for state analysis is even more crucial.
Multi-particle entangled states are becoming more and more interesting for different applications in quantum information, such as quantum multi-particle teleportation, entangled based cryptography and quantum communication schemes based on multi-particle states, but also for fundamental reasons such as testing local realism by means of the Greenberger-Horne-Zeilinger states (GHZ) arguments . The advantage of multiparticle entanglement versus the most common two particle one lies in the fact that the greater the number of particles involved in the entangled state, the more clearly the quantum effects are exhibited. Our final goal is to exploit the multi-photon entangled states for quantum metrology. By the interaction of those states with nanostructures (mostly nanoholes, but in a future also nanospheres), we expect to reach sub-wavelength sensitivity phase measurements beating the Standard Quantum Limit as well as to detect plasmonic effects. In this thesis we present our work consisting on designing and building an experimental setup for the generation of states of 4-photon entangled in the transverse linear momentum. In the first part we explain some basics in the form of a technical introduction. We then adapt a general theoretical model to our particular case, explaining the physics of the process of generation of entangled states of photons. We proceed explaining the details of our setup, as well as the procedure of measurement. We then present the results of our tests in a "standard" 2-photon regime to show the correct functioning of the setup itself. Some more sophisticated measurements using structured light in the form of a first-order Hermite-Gaussian mode has been performed to generate entanglement in higher spatial modes are also presented. We conclude with theoretical and experimental details regarding the 4-photon experiments feasible with our setup. Our source is based on Spontaneous Parametric Down-Conversion (SPDC). In the last two decades it has been extensively studied for the generation of two-photon entangled states, since Kwiat et al. published in 1995 the new scheme based on polarization entangled photons. Most of the studies regarding entangled states involving more than two photons are indeed based on quantum correlations in the polarization or in the path of the down converted beams. The great advantage of entangling a spatial degree of freedom (as we do) is related to the dimensionality of the Hilbert space in which the state is defined. In the particular case of linear momentum, which is a continuous variable, we are dealing with infinite dimensions. Since in each dimension of the state one quanta of information can be encoded, the advantage of having multidimension entanglement for the field of quantum communication and computing is clear. The specs of our setup include a periodically-poled KTP crystals offering high conversion efficiency and cut for type-0 SPDC. The photons generated are well known to be inherently entangled in different degrees of freedom such as polarization, energy-time, linear momentum, and orbital angular momentum. Since each single SPDC event generates one photon pair, in order to reach four photon we entangle two consecutive SPDC events per each state. Furthermore, it is possible to manipulate (to enhance) the dimensionality of the entanglement by properly tailoring the pump spatial profile. The key point for the generation of four-photon entangled states is that, under some conditions, two consecutive pairs generated via SPDC cannot be described as two independent pairs but necessarily as a four-photon state showing genuine entanglement. This can happen when using a pulsed laser to generate the entangled photons; in particular, in the regime in which the coherence time of the down-converted photons τc is (much) longer than the temporal length of the pumping pulse Δt. In this condition the emission of a second pair is stimulated by the presence of the first one. That effect can be ultimately seen as a constructive multi-particle interference effect, the deep origin of which has to be sought in the boson statistic of photons.