Entanglement lies at the heart of quantum mechanics and challenged the intuition of physicists ever since it was discovered. At the same time, it is a powerful tool that serves as a key resource for quantum communication and quantum computation schemes. Many of these applications rely on multiparticle entanglement, whose description, generation and manipulation became therefore a very active field in theoretical and experimental quantum information science. The goals are here to classify and understand the different types of entanglement, to find new applications and to control and analyze the quantum states experimentally. In this thesis, the experimental observation and analysis of two different types of four-photon polarization entangled states is presented: The cluster state and the symmetric Dicke state with two excitations. For this purpose, experimental setups based on spontaneous parametric down conversion and linear optics with conditional detection were designed. They allowed to observe the cluster state with a fidelity of 74.1 % and the symmetric Dicke state with a fidelity of 84.4 %. The cluster state experiment included the development of a new instrument that is of interest for linear optics quantum logic in general: A probabilistic controlled phase gate that is, due to the simplification of a previous approach, highly stable and can actually be used in multiphoton experiments. The quality of the gate is evaluated by analyzing its entangling capability and by performing full process tomography. The achieved results demonstrate that this device is well suited for implementation in various multiphoton quantum information protocols. In order to study the observed quantum states, efficient analysis tools are introduced. It was possible to verify that essential properties of the ideal states are indeed reproduced in the experiment, among others, the presence of genuine four-partite entanglement. A particular focus is put on the behavior of the states under projective measurements and photon loss. Several new insights in their entanglement structure are revealed and verified experimentally. We further demonstrate properties that are characteristic for the entanglement classes of the states. These can be used to infer the applicability of the observed states for certain distributed quantum communication applications. The presented experiments are generic for the design of setups to observe cluster- and symmetric Dicke states with a higher number of photons. Furthermore, also the efficient non-tomographic methods for state analysis we employ can directly be generalized to experiments with higher qubit numbers, where the reduction of the experimental effort for state analysis is even more crucial.
Entanglement lies at the heart of quantum mechanics and challenged the intuition of physicists ever since it was discovered. At the same time, it is a powerful tool that serves as a key resource for quantum communication and quantum computation schemes. Many of these applications rely on multiparticle entanglement, whose description, generation and manipulation became therefore a very active field in theoretical and experimental quantum information science. The goals are here to classify and understand the different types of entanglement, to find new applications and to control and analyze the quantum states experimentally. In this thesis, the experimental observation and analysis of two different types of four-photon polarization entangled states is presented: The cluster state and the symmetric Dicke state with two excitations. For this purpose, experimental setups based on spontaneous parametric down conversion and linear optics with conditional detection were designed. They allowed to observe the cluster state with a fidelity of 74.1 % and the symmetric Dicke state with a fidelity of 84.4 %. The cluster state experiment included the development of a new instrument that is of interest for linear optics quantum logic in general: A probabilistic controlled phase gate that is, due to the simplification of a previous approach, highly stable and can actually be used in multiphoton experiments. The quality of the gate is evaluated by analyzing its entangling capability and by performing full process tomography. The achieved results demonstrate that this device is well suited for implementation in various multiphoton quantum information protocols. In order to study the observed quantum states, efficient analysis tools are introduced. It was possible to verify that essential properties of the ideal states are indeed reproduced in the experiment, among others, the presence of genuine four-partite entanglement. A particular focus is put on the behavior of the states under projective measurements and photon loss. Several new insights in their entanglement structure are revealed and verified experimentally. We further demonstrate properties that are characteristic for the entanglement classes of the states. These can be used to infer the applicability of the observed states for certain distributed quantum communication applications. The presented experiments are generic for the design of setups to observe cluster- and symmetric Dicke states with a higher number of photons. Furthermore, also the efficient non-tomographic methods for state analysis we employ can directly be generalized to experiments with higher qubit numbers, where the reduction of the experimental effort for state analysis is even more crucial.
Since the awareness of entanglement was raised by Einstein, Podolski, Rosen and Schrödinger in the beginning of the last century, it took almost 55 years until entanglement entered the laboratories as a new resource. Meanwhile, entangled states of various quantum systems have been investigated. Sofar, their biggest variety was observed in photonic qubit systems. Thereby, the setups of today's experiments on multi-photon entanglement can all be structured in the following way: They consist of a photon source, a linear optics network by which the photons are processed and the conditional detection of the photons at the output of the network. In this thesis, two new linear optics networks are introduced and their application for several quantum information tasks is presented. The workhorse of multi-photon quantum information, spontaneous parametric down conversion, is used in different configurations to provide the input states for the networks. The first network is a new design of a controlled phase gate which is particularly interesting for applications in multi-photon experiments as it constitutes an improvement of former realizations with respect to stability and reliability. This is explicitly demonstrated by employing the gate in four-photon experiments. In this context, a teleportation and entanglement swapping protocol is performed in which all four Bell states are distinguished by means of the phase gate. A similar type of measurement applied to the subsystem parts of two copies of a quantum state, allows further the direct estimation of the state's entanglement in terms of its concurrence. Finally, starting from two Bell states, the controlled phase gate is applied for the observation of a four photon cluster state. The analysis of the results focuses on measurement based quantum computation, the main usage of cluster states. The second network, fed with the second order emission of non-collinear type II spontaneous parametric down conversion, constitutes a tunable source of a whole family of states. Up to now the observation of one particular state required one individually tailored setup. With the network introduced here many different states can be obtained within the same arrangement by tuning a single, easily accessible experimental parameter. These states exhibit many useful properties and play a central role in several applications of quantum information. Here, they are used for the solution of a four-player quantum Minority game. It is shown that, by employing four-qubit entanglement, the quantum version of the game clearly outperforms its classical counterpart. Experimental data obtained with both networks are utilized to demonstrate a new method for the experimental discrimination of different multi-partite entangled states. Although theoretical classifications of four-qubit entangled states exist, sofar there was no experimental tool to easily assign an observed state to the one or the other class. The new tool presented here is based on operators which are formed by the correlations between local measurement settings that are typical for the respective quantum state.
Major efforts in quantum information science are devoted to the development of methods that are superior to the one of classical information processing, for example the quantum computer or quantum simulations. For these purposes, superposition and entangled states are considered a decisive resource. Furthermore, since the early days of quantum mechanics, entanglement has revealed the discrepancy between the quantum mechanical and the everyday life perception of the physical world. This combination of fundamental science and application-oriented research makes the realization, characterization, and application of entanglement a challenge pursued by many researchers. In this work, the observation of entangled states of polarization encoded photonic qubits is pushed forward in two directions: flexibility in state observation and increase in photon rate. To achieve flexibility two different schemes are developed: setup-based and entanglement-based observation of inequivalent multi-photon states. The setup-based scheme relies on multi-photon interference at a polarizing beam splitter with prior polarization manipulations. It allows the observation of a family of important four-photon entangled states. The entanglement-based scheme exploits the rich properties of Dicke states under particle projections or loss in order to obtain inequivalent multi-photon entangled states. The observed states are characterized using the fidelity and entanglement witnesses. An increase in photon rate is crucial to achieve entanglement of higher photon numbers. This holds especially, when photon sources are utilized that emit photons spontaneously. To this end, a new photon source is presented based on a femtosecond ultraviolet enhancement cavity and applied to the observation of the six-photon Dicke state with three excitations. The implemented schemes not only allow the observation of inequivalent types of entanglement, but also the realization of various quantum information tasks. In this work, the four-photon GHZ state has been used in a quantum simulation of a minimal instance of the toric code. This code enables the demonstration of basic properties of anyons, which are quasiparticles distinct from bosons and fermions. Further, the six-photon Dicke state has been applied for quantum metrology: It allows one to estimate a phase shift with a higher precision than by using only classical resources. Altogether, a whole series of experiments for observing inequivalent multi-photon entangled states can now be substituted by a single experimental setup based on the designs developed in this work. In addition to this new approach of photon processing, a novel photon source has been implemented, paving the way to realizations of applications requiring higher photon numbers.
Multi-particle entangled states are becoming more and more interesting for different applications in quantum information, such as quantum multi-particle teleportation, entangled based cryptography and quantum communication schemes based on multi-particle states, but also for fundamental reasons such as testing local realism by means of the Greenberger-Horne-Zeilinger states (GHZ) arguments . The advantage of multiparticle entanglement versus the most common two particle one lies in the fact that the greater the number of particles involved in the entangled state, the more clearly the quantum effects are exhibited. Our final goal is to exploit the multi-photon entangled states for quantum metrology. By the interaction of those states with nanostructures (mostly nanoholes, but in a future also nanospheres), we expect to reach sub-wavelength sensitivity phase measurements beating the Standard Quantum Limit as well as to detect plasmonic effects. In this thesis we present our work consisting on designing and building an experimental setup for the generation of states of 4-photon entangled in the transverse linear momentum. In the first part we explain some basics in the form of a technical introduction. We then adapt a general theoretical model to our particular case, explaining the physics of the process of generation of entangled states of photons. We proceed explaining the details of our setup, as well as the procedure of measurement. We then present the results of our tests in a "standard" 2-photon regime to show the correct functioning of the setup itself. Some more sophisticated measurements using structured light in the form of a first-order Hermite-Gaussian mode has been performed to generate entanglement in higher spatial modes are also presented. We conclude with theoretical and experimental details regarding the 4-photon experiments feasible with our setup. Our source is based on Spontaneous Parametric Down-Conversion (SPDC). In the last two decades it has been extensively studied for the generation of two-photon entangled states, since Kwiat et al. published in 1995 the new scheme based on polarization entangled photons. Most of the studies regarding entangled states involving more than two photons are indeed based on quantum correlations in the polarization or in the path of the down converted beams. The great advantage of entangling a spatial degree of freedom (as we do) is related to the dimensionality of the Hilbert space in which the state is defined. In the particular case of linear momentum, which is a continuous variable, we are dealing with infinite dimensions. Since in each dimension of the state one quanta of information can be encoded, the advantage of having multidimension entanglement for the field of quantum communication and computing is clear. The specs of our setup include a periodically-poled KTP crystals offering high conversion efficiency and cut for type-0 SPDC. The photons generated are well known to be inherently entangled in different degrees of freedom such as polarization, energy-time, linear momentum, and orbital angular momentum. Since each single SPDC event generates one photon pair, in order to reach four photon we entangle two consecutive SPDC events per each state. Furthermore, it is possible to manipulate (to enhance) the dimensionality of the entanglement by properly tailoring the pump spatial profile. The key point for the generation of four-photon entangled states is that, under some conditions, two consecutive pairs generated via SPDC cannot be described as two independent pairs but necessarily as a four-photon state showing genuine entanglement. This can happen when using a pulsed laser to generate the entangled photons; in particular, in the regime in which the coherence time of the down-converted photons τc is (much) longer than the temporal length of the pumping pulse Δt. In this condition the emission of a second pair is stimulated by the presence of the first one. That effect can be ultimately seen as a constructive multi-particle interference effect, the deep origin of which has to be sought in the boson statistic of photons.
Entanglement is the crucial resource in the field of quantum information processing and consequently a better understanding of its properties is very desirable. While for bipartite entangled qubit states many tools for characterization exist and also the experimental implementation of the tools is feasible, the situation for multipartite entangled states is different: The available tools have to be suited for a much greater diversity of entanglement properties, e.g. to analyze all the different entanglement classes [1]. A full experimental characterization via state tomography is increasingly difficult as the number of necessary measurement settings grows exponentially with the number of particles. In this contribution we focus on efficient, non-tomographic methods to characterize experimentally observed, multipartite entangled states. First steps towards this goal were demonstrated recently, for instance, for the proof of genuine multipartite entanglement [2] or for the analysis of the persistency of entanglement under loss [3]. Such methods can be further optimized by tailoring them to particular properties of states. We show how three important characteristic quantities, the fidelity, the non-separability and the permutation symmetry, can be evaluated with a significantly lower number of measurement settings than required for a complete tomography. Although the determination of these particular properties provides less information than the reconstruction of the complete density matrix, it allows to judge how well state characteristics are reproduced experimentally. This might be important with respect to an experimental application of states in quantum information. Exemplarily we apply the analysis tools to two genuinely four-qubit entangled states: the Dicke state with two excitations |D 4 〉 [4] and the cluster state |C4 〉 [5, 6]. These states are relevant for particular tasks: The state |D 4 〉 is a resource for telecloning [7], cluster states find an application in one-way quantum computation [6, 8] and are a subgroup of graph states, which play an important role for quantum error correction.
In this thesis, I present experimental and theoretical work which assesses and develops a range of tools that are required for performing quantum information processing, particularly in photonic systems. I investigate the three degrees of freedom of a single photon—its polarisation, spatialmomentum and time-frequency distributions. For polarisation, I show that using wave plates to implement arbitrary, single-qubit rotations is more complicated than is commonly appreciated. In the spatial-momentum and time-frequency domains, I develop ways to perform tomographic analysis of quantum states, and I report the first demonstrations of these techniques. In the time-frequency domain, the tomography technique utilises entanglement in the photon polarisation as a resource to store and provide access to the time-frequency information. In my first two experiments, I use spontaneous parametric down-conversion to produce entanglement between pairs of single photons in all three degrees of freedom. I demonstrate the first characterisation of entanglement in spatial modes and the time-frequency domain, the first quantitative measurement of entangled qutrit states, and the highest quality entangled states yet measured in both polarisation and spatial modes. I also report the first realisation of complete hyperentanglement, and a full, black-box tomography of a 36-dimensional two-photon state—the largest system to be characterised in this way to date. In my final experiment, I model and implement a new architecture for a controlled-Z gate which is much simpler to align than previous implementations. This gate requires only one non-classical interference condition, the visibility of which is the main limitation to its performance. I show that the gate operates effectively as a means of both creating entanglement and discriminating between the four elements in a basis of maximally entangled, Bell-type states. Indeed, its observed performance as a Bell analyser would be sufficient to build a quantum state teleporter which would guarantee that the recipient would be left with a better copy of an unknown input state than any eavesdropper. In a series of numerical simulations, I investigate some of the practicalities that arise when using tomographic reconstruction techniques, including how to estimate errors, which measurements to make and what is actually the optimal reconstruction. In particular, I show that tomographies perform better when based on the results from over-complete sets of measurements. Finally, I discuss the important issue of how to compare two processes, particularly when trying to assess the quality of a measured process by comparing it to some expected ideal. Judging possible candidate measures against a set of experimentally and theoretically motivated
This thesis describes a linear-optical device for performing generalized quantum measurements \non quantum bits (qubits) encoded in photon polarization, the implementation \nof said device, and its use in two diff erent but related experiments. The device works by \ncoupling the polarization degree of freedom of a single photon to a `mode' or `path' degree \nof freedom, and performing a projective measurement in this enlarged state space in order \nto implement a tunable four-outcome positive operator-valued measure (POVM) on the \ninitial quantum bit. In both experiments, this POVM is performed on one photon from a \ntwo-photon entangled state created through spontaneous parametric down-conversion. \nIn the fi rst experiment, this entangled state is viewed as a two-qubit photonic cluster \nstate, and the POVM as a means of increasing the computational power of a given resource \nstate in the cluster-state model of quantum computing. This model traditionally \nachieves deterministic outputs to quantum computations via successive projective measurements, \nalong with classical feedforward to choose measurement bases, on qubits in a highly entangled \nresource called a cluster state; we show that `virtual qubits' can be appended to a \ngiven cluster by replacing some projective measurements with POVMs. Our experimental \ndemonstration fully realizes an arbitrary three-qubit cluster computation by implementing \nthe POVM, as well as fast active feed-forward, on our two-qubit photonic cluster state. \nOver 206 diff erent computations, the average output delity is 0.9832 +/- 0.0002; furthermore \nthe error contribution from our POVM device and feedforward is only of order 10^-3, less \nthan some recent thresholds for fault-tolerant cluster computing. \nIn the second experiment, the POVM device is used to implement a deterministic \nprotocol for remote state preparation (RSP) of arbitrary photon polarization qubits. RSP \nis the act of preparing a quantum state at a remote location without actually transmitting \nthe state itself. We are able to remotely prepare 178 diff erent pure and mixed qubit \nstates with an average delity of 0.995. Furthermore, we study the the fidelity achievable \nby RSP protocols permitting only classical communication, without shared entanglement, \nand compare the resulting benchmarks for average fidelity against our experimental results. \nOur experimentally-achieved average fi delities surpass the classical thresholds whenever \nclassical communication alone does not trivially allow for perfect RSP.