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Journal of Experimental and Theoretical Physics

Characteristics of the coherent excitation of an impurity atom in a photonic crystal

Ashat M. Basharov

Published Dec 1, 1999• 3 citations
Publisher

Abstract

It is shown that when an optically allowed transition is coherently excited in an impurity atom in a photonic crystal under conditions where one of the normal relaxation channels is suppressed by the spectral characteristics of the photonic crystal, new relaxation mechanisms are activated involving a coherent field quantum. These mechanisms substantially alter the dynamics of the atomic system, leading to filling of levels of the impurity atom which do not belong to the coherently excited atomic transition. Under certain conditions this leads to population inversion as a result of an optically allowed transition which does not interact with the coherent pump and at a frequency where no photonic band gaps can exist.

DOI
10.1134/1.559053

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It is shown that when an optically allowed transition is coherently excited in an impurity atom in a photonic crystal under conditions where one of the normal relaxation channels is suppressed by the spectral characteristics of the photonic crystal, new relaxation mechanisms are activated involving a coherent field quantum. These mechanisms substantially alter the dynamics of the atomic system, leading to filling of levels of the impurity atom which do not belong to the coherently excited atomic transition. Under certain conditions this leads to population inversion as a result of an optically allowed transition which does not interact with the coherent pump and at a frequency where no photonic band gaps can exist.
It is shown that resonant interaction of a coherent wave with impurity atoms leads to filling of levels of an impurity atom that lie in the gap in the photon density of states and do not belong to resonant transitions, while the interaction of impurity atoms with a nonresonant coherent wave results in effective deactivation of the indicated levels. The main mechanism determining the pumping and decay of an impurity level in a gap are two-photon radiative relaxation processes previously investigated by the present author (Zh. Éksp. Teor. Fiz. 102 , 1126 (1992) [Sov. Phys. JETP 75 , 611 (1992)]).
Two-quantum relaxation transitions in an impurity atom that are activated by its resonance interaction with a monochromatic wave lead to hole burning in the distribution of atoms populating the lower energy level over detunings from the resonance. In this case, the levels of an impurity atom lying within the gap or the pseudogap in the density of photon states of a photonic crystal act as a trap. The impurity atoms change to these levels in the process of interaction of a monochromatic wave with the atomic transition that is not influenced by specific spectral features of a photonic crystal.
On the base of the concept of radiative interaction between atoms of two different species, a novel electric-dipole mechanism of spontaneous radiating relaxation of an impurity atom in a medium with a gap in the photonic density of states about the transition frequency has been suggested. A kinetic equation for an impurity atom has been derived, and polarizations of the photonic band-gap crystal and an induced electromagnetic wave at the spontaneous transition frequency due to the suggested mechanism have been investigated. The parameters of the induced wave are determined by those of the suggested mechanism, and this dependence can be used in experimental investigations of these parameters.
We investigate quantum interference and classical interference effects when a three-level system interacts with both a cavity field mode and an external driving field mode, within the confines of a photonic crystal material. In freespace, we found that under certain circumstances the cavity field evolves to be equal in magnitude to, but 180° out-of- phase with the external pump field when the pump field frequency equals the cavity frequency. The better the cavity, the quicker this build-up occurs. When the cavity field reaches this out-of-phase condition, the resonance fluorescence from the atom in the cavity goes to zero. This is a purely classical interference effect between the two out-of-phase fields, with the resonance fluorescence going to zero at the same time as the two excited state populations go to zero. This is quite different from the quantum interference that occurs under the right circumstances, when the state populations are coherently driven into a linear combination that is decoupled from any applied field - and population is trapped in the excited states, thus allowing for a population inversion and an amplification of incoming optical signals. In this paper, we investigate the additional effects due to the presence of the altered photon density of states in a photonic crystal.
A quantum dot interacting with the radiation field of a photonic crystal is considered. An analytical description of the dynamics and the coherence between the two states of the quantum dot is provided. Besides the well-known trapping, a fractional nature of the dynamics appears via relaxations of the Mittag–Leffler type. Furthermore, coherence exhibits a transition from the decay to if the transition frequency of the quantum dot is exactly in the middle of the band gap. Similarly, the population of the excited level undergoes a transition from the relaxation to . These resonances and transitions belong also to the context of matter-wave emissions in optical lattices.
Summary form only given. Unlike semiconductors which facilitate the coherent propagation of electrons, photonic band gap (PBG) materials execute their novel functions through the coherent localization of photons. When a PBG material is doped with impurity atoms which have an electronic transition that lies within the gap, spontaneous emission of light from the atom is inhibited. Inside the gap, the photon forms a bound state to the atom. Outside the gap, radiative dynamics in the colored vacuum is highly nonMarkovian. I discuss the influence of these memory effects on laser action. When spontaneous emission is absent, the next order radiative effect (resonance dipole-dipole interaction between atoms) must be incorporated, leading to anomalous nonlinear optical effects which occur at a much lower threshold than in ordinary vacuum. I describe the collective switching of two-level atoms near a photonic band edge, by external laser field, from a passive stare to one exhibiting population inversion. This effect is forbidden in ordinary vacuum. Finally, I discuss the prospects for a phase sensitive, single (3-level) atom quantum memory device, onto which information may be written by an external laser pulse. By scattering polarized photons (flying qubit) this system may execute certain quantum logic operations.