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Review of Scientific Instruments

Cascaded two-photon spectroscopy of Yb atoms with a transportable effusive atomic beam apparatus

Minsoo Song, Tai Hyun Yoon

Published Feb 1, 2013• 0 citations
Publisher

Abstract

We present a transportable effusive atomic beam apparatus for cascaded two-photon spectroscopy of the dipole-forbidden transition (6s(2)(1)S0↔ 6s7s (1)S0) of Yb atoms. An ohmic-heating effusive oven is designed to have a reservoir volume of 1.6 cm(3) and a high degree of atomic beam collimation angle of 30 mrad. The new atomic beam apparatus allows us to detect the spontaneously cascaded two-photons from the 6s7s(1)S0 state via the intercombination 6s6p(3)P1 state with a high signal-to-noise ratio even at the temperature of 340 °C. This is made possible in our apparatus because of the enhanced atomic beam flux and superior detection solid angle.

DOI
10.1063/1.4790849

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Magneto-optical trapping of Yb atoms using an intercombination transition

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We report the magneto-optical trapping of ytterbium atoms using the 6s2 1S0-6s6p 3P1 intercombination transition. The magneto-optical trap is continuously loaded from an atomic beam decelerated by a Zeeman-tuned atomic-beam slower operated at the 6s2 1S0-6s6p 1P1 transition. Among seven stable isotopes of ytterbium, six isotopes of 170Yb, 171Yb, 172Yb, 173Yb, 174Yb, and 176Yb are successfully trapped. The number and density of the trapped atoms are about 108 and 1011 cm-3, respectively. The temperature of atoms is estimated to be about 20 μK from the time-of-flight measurement. The decay time of the trapped atoms after stopping the loading of atoms is about 3 s.

•Aug 1, 1999•0 citations
We present a transportable effusive atomic beam apparatus for cascaded two-photon spectroscopy of the dipole-forbidden transition (6s(2)(1)S0↔ 6s7s (1)S0) of Yb atoms. An ohmic-heating effusive oven is designed to have a reservoir volume of 1.6 cm(3) and a high degree of atomic beam collimation angle of 30 mrad. The new atomic beam apparatus allows us to detect the spontaneously cascaded two-photons from the 6s7s(1)S0 state via the intercombination 6s6p(3)P1 state with a high signal-to-noise ratio even at the temperature of 340 °C. This is made possible in our apparatus because of the enhanced atomic beam flux and superior detection solid angle.
We report on the generation of narrow-bandwidth and frequency-modulated cascaded emission of two photons from a collimated Yb atomic beam. Efficient population transfer from the ground state (6s26{s}^{2}6s2 1S0{}^{1}{S}_{0}1S0​) to upper state (6s7s6s7s6s7s 1S0{}^{1}{S}_{0}1S0​), of which direct transition at 291.1 nm is dipole forbidden, is achieved through a resonant two-photon excitation enhanced by the electromagnetically induced transparency mediated by the intermediate state (6s6p6s6p6s6p 1P1{}^{1}{P}_{1}1P1​). Then cascaded emission of two photons with a bandwidth of 54 MHz at 611.3 nm (idler) and 555.8 nm (signal) occurs in sequence from the upper state via the spin triplet state (6s26{s}^{2}6s2 3P1{}^{3}{P}_{1}3P1​). Numerical calculations of the density matrix equations taking into account the residual Doppler effect and strong driving fields successfully explain the experimental results for the idler and signal beam intensities depending on the various parameters of the driving fields. Synchronized optical switching and frequency-modulation characteristics of the idler and signal beams are also reported.
We calculate and measure the magic wavelengths for the $6{s}^{2}^{1}S_{0}\ensuremath{-}6s6p\phantom{\rule{0.16em}{0ex}}^{3}P_{1}$ intercombination transition of the neutral ytterbium atom. The calculation is performed with the ab initio configuration interaction +++ all-order method. The measurement is done with laser spectroscopy on cold atoms in an optical dipole trap. The magic wavelengths are determined to be 1035.68(4) nm for the $\ensuremath{\pi}$ transition $(\mathrm{\ensuremath{\Delta}}m=0)$ and 1036.12(3) nm for the $\ensuremath{\sigma}$ transitions $(|\mathrm{\ensuremath{\Delta}}m|=1)$ in agreement with the calculated values. Laser cooling on the narrow intercombination transition could achieve better results for atoms in an optical dipole trap when the trap wavelength is tuned to near the magic wavelength.
We report the magneto-optical trapping of ytterbium atoms using the ${6s}^{2}{}^{1}{S}_{0}\ensuremath{-}6s6p{}^{3}{P}_{1}$ intercombination transition. The magneto-optical trap is continuously loaded from an atomic beam decelerated by a Zeeman-tuned atomic-beam slower operated at the ${6s}^{2}{}^{1}{S}_{0}\ensuremath{-}6s6p{}^{1}{P}_{1}$ transition. Among seven stable isotopes of ytterbium, six isotopes of170Yb,\mathrm{of}{ }^{170}\mathrm{Y}\mathrm{b},of170Yb, 171Yb,{}^{171}\mathrm{Yb},171Yb, 172Yb,{}^{172}\mathrm{Yb},172Yb, 173Yb,{}^{173}\mathrm{Yb},173Yb, 174Yb,{}^{174}\mathrm{Yb},174Yb, and 176Yb{}^{176}\mathrm{Yb}176Yb are successfully trapped. The number and density of the trapped atoms are about 108{10}^{8}108 and ${10}^{11} {\mathrm{cm}}^{\ensuremath{-}3},$ respectively. The temperature of atoms is estimated to be about $20 \ensuremath{\mu}\mathrm{K}$ from the time-of-flight measurement. The decay time of the trapped atoms after stopping the loading of atoms is about 3 s.
We demonstrate launching of laser-cooled Yb atoms in a cold atomic fountain. Atoms in a collimated thermal beam are first cooled and captured in a magneto-optical trap (MOT) operating on the strongly allowed ${{}^{1}S}_{0}\ensuremath{\rightarrow}{{}^{1}P}_{1}$ transition at 399 nm (blue line). They are then transferred to a MOT on the weakly allowed ${{}^{1}S}_{0}\ensuremath{\rightarrow}{{}^{3}P}_{1}$ transition at 556 nm (green line). Cold atoms from the green MOT are launched against gravity at a velocity of around 2.5 m/s using a pair of green beams. We trap more than 107{10}^{7}107 atoms in the blue MOT and transfer up to 7070%70 into the green MOT. The temperature for the odd isotope 171Yb^{171}\mathrm{Yb}171Yb is  1mK~1 \mathrm{mK} 1mK in the blue MOT, and reduces by a factor of 40 in the green MOT.
Two-photon Doppler-free spectroscopy of the 6s2  1S0→6s23s  1S06s^2\;^1S_0 \rightarrow 6s23s\;^1S_06s21S0​→6s23s1S0​ Rydberg transition for quantum sensing in ytterbium
Here we report atomic structure calculations and experimental observations of the two-photon 6s2  1S0→6s23s  1S06s^2\;^1S_0 \rightarrow 6s23s\;^1S_06s21S0​→6s23s1S0​ transition in Yb. The unique level structure of Yb places the 6s6p  1P16s6p\;^1P_16s6p1P1​ state's energy at ≈ ⁣49.7%\approx\!49.7\%≈49.7% of the ionization energy, which facilitates two-photon Doppler-free excitation of the 6s23s  1S06s23s\;^1S_06s23s1S0​ Rydberg state from the 6s2  1S06s^2\;^1S_06s21S0​ ground state at a relatively low optical intensity. This J=0→J=0J= 0 \rightarrow J=0J=0→J=0 transition is immune to first-order Zeeman and electric quadrupole shifts, has reduced sensitivity to higher-order Zeeman shifts, and is further predicted to have relatively low sensitivity to density shifts. Using configuration interaction theory, we compute relevant properties of the 6s23s  1S06s23s\;^1S_06s23s1S0​ Rydberg state for sensing, including the C6C_6C6​ coefficient, dc polarizability, blackbody radiation (BBR) shift, and BBR depopulation rate. As a first experimental step, we demonstrate two-photon Doppler-free spectroscopy of the 6s2  1S0→6s23s  1S06s^2\;^1S_0 \rightarrow 6s23s\;^1S_06s21S0​→6s23s1S0​ transition. From our experimental spectra, we estimate the natural linewidth (lifetime) of the 6s23s  1S06s23s\;^1S_06s23s1S0​ state to be 90 kHz (1.8 μμμs). We believe this transition, or other 6s2  1S0→6sns  1S06s^2\;^1S_0 \rightarrow 6sns\;^1S_06s21S0​→6sns1S0​ transitions in Yb with n≈23n\approx23n≈23, may find use in a variety of sensing applications, potentially including a two-photon clock, electrometer, or BBR thermometer.
We report the magneto-optical trapping of ytterbium atoms using the 6s2 1S0-6s6p 3P1 intercombination transition. The magneto-optical trap is continuously loaded from an atomic beam decelerated by a Zeeman-tuned atomic-beam slower operated at the 6s2 1S0-6s6p 1P1 transition. Among seven stable isotopes of ytterbium, six isotopes of 170Yb, 171Yb, 172Yb, 173Yb, 174Yb, and 176Yb are successfully trapped. The number and density of the trapped atoms are about 108 and 1011 cm-3, respectively. The temperature of atoms is estimated to be about 20 μK from the time-of-flight measurement. The decay time of the trapped atoms after stopping the loading of atoms is about 3 s.