The present work develops further the idea of using an atomic scale object as a lens in corpuscular optics which was introduced previously and developed for electrons. A possible atomic lens in the form of a nanohole for atomic and molecular optics is considered and studied.
The most efficient method for controlling the motion of material particles in experimental physics is the use of interaction potentials with electromagnetic fields. The static magnetic and electric interaction potentials are used in the optics of charged particles. In the optics of neutral atoms, the various interaction potentials of atoms with laser and electromagnetic fields are used in addition to the static fields. The effective methods of diffraction, interference, mirror reflection of atoms are implemented in atom optics. The most difficult problem in atom optics is the problem of high-resolution focusing of neutral atoms, which is promising for the nondestructive method for probing the surface at the atomic level, as well as for the creation of nanostructures on the surface. Although there are many proposals for focusing of atomic beams, this problem is experimentally unsolved. The main difficulty is the creation of the interaction potential of the atom with the electromagnetic field that is close to an ideal lens for atoms.In this paper, we experimentally implement another approach to the problem of focusing and construction of an image in atom optics, which is based on a well known idea of optical pinhole camera. The pinhole camera in optics is a camera without lens. Light forming an image passes through a small hole. In our experiment with the atom pinhole camera the Cr atomic beam passes through a set of holes in a metal mask and thereby forms, by analogy with optics, a glowing object of a given geometry. The atoms pass through the holes in the mask, propagate in vacuum along rectilinear trajectories, similar to light rays, and are incident on a thin film (thickness 5 mum) placed at a distance of 90 mm from the mask with a large number (n =107-108/cm2) of nanoholes (50 nm diameter). Each hole of the film is a pinhole camera for atoms, which forms its individual image of the object on the substrate surface placed at a distance of l = 5mum behind the film.
In the field of atom optics, there has been much interests in developing components such as lenses, mirrors, beam splitters and waveguides to manipulate neutral atoms. Especially many clever methods to focus neutral atoms have been developed. The lenses have been constructed using the static electrical and magnetic fields, Fresnel zone plates, and radiation pressure forces. Before the laser cooling and trapping techniques were invented, the electrostatic fields could not be used for manipulating neutral atoms because of its weak interaction energy with atoms. After the cold atoms were available, it has been possible to manipulate atoms with weak electrostatic interaction energy. We developed an atom lens system using electrostatic fields.
A nitrogen vacancy (NV) center in diamond is known as a solid-state spin quantum bit (qubit) at room temperature. The fabrication of scalable quantum registers based on NV centers is a long-standing issue. In 2005, spin-spin interaction between NV-N pairs, which were fabricated by N2 ion implantation, was reported. An entanglement between two electron-spin qubits becomes an excellent quantum information processing component, as accomplished by an NV-NV pair with a nanometer-scale distance in 2010 and 2013. More recently,strongly dipolar coupled NV-NV pairs were realized by 14N 30 keV implantationvia nanoholes in PMMA resist mask. The creation yields of NV-NV pairs dramatically improved, and the nanohole implantation had been thought to be the most promising technique to integrate NV centers. However, the problem of the technique is the finite size of nanoholes. The distribution of nitrogen atoms is determined by both ion straggling and nanohole diameter. The scaling of NV centers is stagnant up to two for several years. To overcome the barrier of triple NV centers, our previous research gave a ground-breaking idea of a highly populated NV center complex by introducing a molecular ion implantation technique in 2019. Since the molecular ion is regarded as an idea point source, the distribution of nitrogen atoms is determined by only ion straggling. Therefore, our proposed method is more effective than other implantation techniques including nanohole implantation. Instead of a pure nitrogen cluster which is commonly unstable, the stable organic molecular ions (adenine; C5N5H5) were utilized as the ion source. We successfully implanted C5N4Hn ions into single crystalline diamonds. Three NV centers were integrated, and the dipolar interactions among them were successfully observed. In 2022, we succeeded in creating more than 5 NV centers by phthalocyanine (C32H18N8) ion implantation. The next challenge is the implantation of isotopically enriched molecular ions. The isotopically enriched ion contains 13C and 15N. The implantation of isotopically enriched molecular ions is able to create 15NV-13C hybrid quantum registers. In this presentation, we will show the development of the isotopically enriched molecular ion beam and the characterization of created NV centers by laboratory-built confocal microscopy (CFM) and optically detected magnetic resonance (ODMR).