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Optics Communications

The fluorescence spectrum of a three-level atom in two-photon resonance with the laser field

Božena Sobolewska

Published Mar 1, 1977• 7 citations
Publisher
DOI
10.1016/0030-4018(77)90208-5

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Two-photon resonance fluorescence in a three-level system

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OptSp•Dec 1, 1979•0 citations
We consider the possible physical processes that may arise in a three-level atom when only two of its levels interact with a strong electromagnetic field and when the atomic transition frequency is nearly equal to once and twice the frequency of the laser field, respectively. There have been found pronounced cooperative effects in the spectrum of the two-level system, which is in resonance with the laser field, arising from the presence of the third level. The excitation spectra describing the transitions from the first excited state into the second excited state and from that to the ground state consist, apart from the two central peaks, of two pairs of sidebands which are induced by the laser field of the neighbouring system. Detailed expressions of the spectral functions for the physical processes of one- and two-photon resonance fluorescence have been derived and discussed in the limit of high photon densities. The excitation spectrum of the low frequency modes has been considered and discussed in detail. It is found that quantum beats in spontaneous emission may appear in the spectra of the one- and two-photon resonance fluorescence arising from the interference between the two atomic transition frequencies and the frequency of the laser field. The importance of the low frequency modes that occur in the processes in question has been pointed out.
We theoretically investigate resonance fluorescence of a ladder- and a triangular-type three-level atomic system in the full quantization regime. By solving Heisenberg’s quantum kinetic equations of motion of an electron interacting with photons and two coherent laser fields, we obtain the firstorder electric field correlation function, which corresponds to photoluminescence spectrum. When the single electrons in both systems are resonantly excited by two strong cw-laser fields, in contrast to the ladder-type atomic systems emitting mainly incoherent photons, the triangular-type system shows that continuous coherent photons can be selectively generated from three optical transitions by trapping electronic population inversions and manipulated by changing the transition rates.