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Physical Review A

Theory of four-wave mixing with matter waves without the undepleted pump approximation

Ying Wu, Xiaoxue Yang, C. P. Sun, Xiaoji Zhou, Y. Q. Wang

Published Mar 8, 2000• 51 citations
Publisher

Abstract

Starting from the Gross-Pitaevskii nonlinear Schr"odinger equation, we derive a set of nonlinear coupled equations describing four-wave mixing with matter waves and solve them analytically without utilizing the undepleted pump approximation.
DOI
10.1103/physreva.61.043604

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A recent experiment [Deng et al., Nature (London) 398, 218 (1999)] demonstrated four-wave mixing of matter wave packets created from a Bose-Einstein condensate. The experiment utilized light pulses to create two high-momentum wave packets via Bragg diffraction from a stationary Bose-Einstein condensate. The high-momentum components and the initial low-momentum condensate interact to form a new momentum component due to the nonlinear self-interaction of the bosonic atoms. We develop a three-dimensional quantum- mechanical description, based on the slowly-varying-envelope approximation, for four-wave mixing in Bose-Einstein condensates using the time-dependent Gross-Pitaevskii equation. We apply this formulation to describe the experimental observations and to make predictions. We examine the role of phase-modulation, momentum, and energy conservation (i.e., phase matching), and particle number conservation in four-wave mixing of matter waves, and develop simple models for understanding our numerical results.
Starting from a second-quantized Hamiltonian of many-particle systems, we derive the Gross-Pitaevskii (GP) equation in momentum space, which is suitable for studying the multi-wave mixing processes of coherent matter waves. The coupling equations are then applied to study ideal four-wave mixing (4WM), in which only four waves with definite wavevectors are involved. Some interesting problems of 4WM, such as the phase-matching condition, the collapse and revival behaviour, the effects of relative phase difference, and the conversion efficiency are discussed in detail. We also show that the main characters of recent 4WM experiment [Deng et al, Nature 398, 218 (1999)] can be undersood in the present simplified model.
The advent of the laser as an intense, coherent light source gave birth to nonlinear optics, which now plays an important role in many areas of science and technology. One of the first applications of nonlinear optics was the production of coherent light of a new frequency by multi-wave mixing of several optical fields in a nonlinear medium. Until the experimental realization of Bose-Einstein Condensation (BEC) there had been no intense coherent source of matter-waves analogous to the optical laser. FEC has already been exploited to produce a matter-wave `laser' leading to the threshold of a new field of physics: nonlinear atom optics. Recently the first experiment in nonlinear atom optics was reported: the observation of coherent four wave mixing in which three sodium matter waves mix to produce a fourth. The experiment utilized light pulses to create two high-momentum wavepackets via Bragg diffraction from a stationary Bose- Einstein condensate. The high-momentum components and the remaining zero momentum condensate component interact to form a new momentum component due to the nonlinear self- interaction of the bosonic atoms. We develop a quantum mechanical description, based on the slowly-varying-envelope approximation to the time-dependent nonlinear Schrodinger equation (also called the Gross-Pitaevskii equation), to describe four-wave mixing in Bose-Einstein condensates and apply this description to understand the experimental observations and to make new predictions. We examine the role of phase-modulation, momentum and energy conservation (i.e., phase-matching), and particle number conservation in four-wave mixing of matter waves.