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arXiv:cond-mat/0008395

Theory of Ideal Four-Wave Mixing in Bose-Einstein Condensates

Deng, Wenji, P. M. Hui

Published Aug 28, 2000• 0 citations
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Abstract

Starting from a second-quantized Hamiltonian of many-particle systems, we derive the Gross-Pitaevskii (GP) equation in momentum space, which is suitable for studying the multi-wave mixing processes of coherent matter waves. The coupling equations are then applied to study ideal four-wave mixing (4WM), in which only four waves with definite wavevectors are involved. Some interesting problems of 4WM, such as the phase-matching condition, the collapse and revival behaviour, the effects of relative phase difference, and the conversion efficiency are discussed in detail. We also show that the main characters of recent 4WM experiment [Deng et al, Nature 398, 218 (1999)] can be undersood in the present simplified model.

DOI
10.48550/arxiv.cond-mat/0008395

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Starting from a second-quantized Hamiltonian of many-particle systems, we derive the Gross-Pitaevskii (GP) equation in momentum space, which is suitable for studying the multi-wave mixing processes of coherent matter waves. The coupling equations are then applied to study ideal four-wave mixing (4WM), in which only four waves with definite wavevectors are involved. Some interesting problems of 4WM, such as the phase-matching condition, the collapse and revival behaviour, the effects of relative phase difference, and the conversion efficiency are discussed in detail. We also show that the main characters of recent 4WM experiment [Deng et al, Nature 398, 218 (1999)] can be undersood in the present simplified model.
A recent experiment [Deng et al., Nature (London) 398, 218 (1999)] demonstrated four-wave mixing of matter wave packets created from a Bose-Einstein condensate. The experiment utilized light pulses to create two high-momentum wave packets via Bragg diffraction from a stationary Bose-Einstein condensate. The high-momentum components and the initial low-momentum condensate interact to form a new momentum component due to the nonlinear self-interaction of the bosonic atoms. We develop a three-dimensional quantum- mechanical description, based on the slowly-varying-envelope approximation, for four-wave mixing in Bose-Einstein condensates using the time-dependent Gross-Pitaevskii equation. We apply this formulation to describe the experimental observations and to make predictions. We examine the role of phase-modulation, momentum, and energy conservation (i.e., phase matching), and particle number conservation in four-wave mixing of matter waves, and develop simple models for understanding our numerical results.
The nonlinear coupling term in the Gross-Pitiaevski equation which describes a Bose-Einstein condensate (BEC) can cause four- wave mixing (4WM) if three BEC wavepackets with momenta k1, k2, and k3 interact. The interaction will produce a fourth wavepacket with momentum k4 = k1 + k2. We study this process using numerical models and suggest that experiments are feasible. Conservation of energy and momentum have different consequences for 4WM with massive particles than in the nonlinear optics case because of the different energy-momentum dispersion relations.
Abstract We describe possibilities of spontaneous, degenerate four-wave mixing (FWM) processes in spin–orbit coupled Bose–Einstein condensates. Phase matching conditions (i.e., energy and momentum conservation laws) in such systems allow one to identify four different configurations characterized by involvement of distinct spinor states in which such a process can take place. We derived these conditions from first principles and then illustrated dynamics with direct numerical simulations. We found, among others, the unique configuration, where both probe waves have smaller group velocity than pump wave and proved numerically that it can be observed experimentally under proper choice of the parameters. We also reported the case when two different FWM processes can occur simultaneously. The described resonant interactions of matter waves is expected to play an important role in the experiments of BEC with artificial gauge fields. Beams created by FWM processes are an important source of correlated particles and can be used in the experiments testing quantum properties of atomic ensembles.
A recent experiment demonstrated four-wave mixing of wavepackets in a sodium Bose–Einstein condensate (Deng et al 1999 Nature 398 218). This was followed by a theoretical and numerical treatment of the experiment (Trippenbach et al 2000 Phys. Rev. A 62 02368). In the experiment, a short period of free expansion of the condensate, after release from the magnetic trap, was followed by a set of two Bragg pulses which created moving wavepackets. These wavepackets, due to nonlinear interaction and under phase-matching conditions, created a new momentum component in a four-wave mixing process. We propose simple mathematical models for this process. Next we suggest that, instead of exactly matching the frequencies as in the abovementioned experiments, we introduce a small mismatch in the energies, and therefore the frequencies Δω. We show that such a small mismatch can compensate for the initial phases that are built on the condensate during free expansion. A physical explanation is offered. This compensation can improve the efficiency of four-wave mixing; in some cases even increasing it by a factor of 2. We also deal with the situation where two strong wavepackets are accompanied by a weak input beam applied as a seed both with and without a mismatch. Here the influence of the mismatch is less obviously beneficial. We also comment on recent work by Ketterle's group (Vogels et al 2002 Phys. Rev. Lett. 89 020401).
We investigate the four-wave mixing of matter wave packets created from a Bose–Einstein condensate, realized experimentally by utilizing light pulses to create two high-momentum wave packets via Bragg diffraction from a stationary condensate. Based on the Gross–Pitaevskii equation, a set of nonlinearly coupled envelope equations including self- and cross-phase modulational effects are derived systematically using a method of multiple-scales. The exact and explicit analytical solutions are provided for the coupled envelope equations and the evolution of the wave packets after turning off trapping potential is discussed and compared with experiment.