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Physical Review A

Prediction of Feshbach resonances in collisions of ultracold rubidium atoms

J. M. M. J. Vogels, Chin‐Chun Tsai, R. S. Freeland, S. J. J. M. F. Kokkelmans, BOUDEWIJN J. VERHAAR, Daniel J. Heinzen

Published Aug 1, 1997• 133 citations
Publisher

Abstract

On the basis of recently measured ${\mathrm{Rb}}_{2}$ bound-state energies and continuum properties, we predict magnetically induced Feshbach resonances in collisions of ultracold rubidium atoms. The resonances make it possible to control the sign and magnitude of the effective particle-particle interaction in a Rb Bose-Einstein condensate by tuning a bias magnetic field. For the case of ${}^{85}\mathrm{Rb}$ they occur at field values in the range where these atoms can be magnetostatically trapped. For ${}^{87}\mathrm{Rb}$ they are predicted to occur at negative field values.

DOI
10.1103/physreva.56.r1067

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The research described in this thesis is part of an international effort with the aim of studying ultracold quantum degenerate gas samples like Bose-Einstein condensates and Fermi degenerate systems, consisting of atoms confined in magnetic or optical traps. The behavior of such samples is governed by the inter-atomic interactions and the resulting properties of the atom-atom scattering. At the relevant temperatures of 1nK to 10µK a key property is the atom-atom scattering length a. In chapter 2 a theoretical method is presented which enables one to describe the interaction and scattering of (ultra)cold atoms to unprecedented precision. It is also unparalleled in comprehensiveness: it allows the prediction of a large and varied set of experimental data for all isotopes of the same element. The method relies on the extraction from experiments of a few (phase) parameters which completely summarize the behavior of the atoms in the (ultra)cold regime. In chapter 3 the method is applied to the "workhorses" of cold-atom physics: the atomic species 85Rb and 87Rb. We extract the foregoing parameters to a very high precision from several recent high precision experiments, allowing us to predict e.g. the 87Rb spinor condensate to be ferromagnetic: a prediction for which the scattering length has to be calculated with a precision better than 1%. We also predict Feshbach resonances at experimentally accessible magnetic field strengths; resonances searched for and found by the experimental group of Rempe. In close collaboration with his group we "fine-tune" the interaction parameters found previously, by making use of only one of the observed resonances. We then obtain agreement with 42 out of the observed 43 resonance field strengths and are able to identify bound states inducing the Feshbach resonances at these locations. Chapter 4 describes the results of this research. With a thorough understanding of the rubidium interactions, we then switch to lithium which has a fermionic (6Li) and a bosonic (7Li) isotope. Both are being used in cold-atom experiments. In chapter 5 we evaluate the interaction parameters for lithium allowing us to predict magnetic field strengths for which a sample of fermionic 6Li atoms can be regarded as strongly interacting. Furthermore, a three-level method for measuring mean-field shifts, based on radio-frequency techniques, is introduced. For weak interactions we find proportionality of resonance shifts to interaction strengths. In the strongly interacting regime, however, these shifts become very small reflecting the quantum unitarity limit and many-body effects. Most interesting is the fact that in this regime the shifts are small both for large positive a and for large negative a, likely reflecting the universality of the interaction energy. In chapters 6 and 7 the interactions between lithium atoms are reinvestigated, making use of newly available experimental data and with the updated interaction parameters special attention is paid to locating field strengths at which magnetically tunable Feshbach resonances occur in the scattering of lithium atoms. In chapter 6 scattering events in a gas of (fermionic) 6Li atoms are studied. In chapter 7 we show that a consistent description of the 6Li+6Li system can be given. We discuss theoretical uncertainties for the position of the wide 6Li Feshbach resonance and present an analytic scattering model for this resonance, based on the inclusion of a field-dependent virtual open-channel state. We predict new Feshbach resonances for the 6Li-7Li system, and their importance for different types of crossover superfluidity models is discussed. Molecules created by magnetically sweeping over these resonances will have a fermionic character. One magnetic field strength is predicted at which two different fermionic molecules can be created simultaneously.

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On the basis of recently measured Rb2{\mathrm{Rb}}_{2}Rb2​ bound-state energies and continuum properties, we predict magnetically induced Feshbach resonances in collisions of ultracold rubidium atoms. The resonances make it possible to control the sign and magnitude of the effective particle-particle interaction in a Rb Bose-Einstein condensate by tuning a bias magnetic field. For the case of 85Rb{}^{85}\mathrm{Rb}85Rb they occur at field values in the range where these atoms can be magnetostatically trapped. For 87Rb{}^{87}\mathrm{Rb}87Rb they are predicted to occur at negative field values.
We present an analysis of experimentally accessible magnetic Feshbach resonances in ultracold heteronuclear $^{85}\mathrm{Rb}\text{\ensuremath{-}}^{87}\mathrm{Rb}$ and $^{6}\mathrm{Li}\text{\ensuremath{-}}^{87}\mathrm{Rb}$ mixtures. Using recent experimental measurements of the triplet scattering lengths for $^{6}\mathrm{Li}\text{\ensuremath{-}}^{87}\mathrm{Rb}$ and $^{7}\mathrm{Li}\text{\ensuremath{-}}^{87}\mathrm{Rb}$ mixtures and Feshbach resonances for one combination of atomic states, we create model potential curves and fine-tune them to reproduce the measured resonances and to predict the location of several experimentally relevant resonances in Li-Rb collisions. To model $^{85}\mathrm{Rb}\text{\ensuremath{-}}^{87}\mathrm{Rb}$ collisions, we use accurate Rb2{\mathrm{Rb}}_{2}Rb2​ potentials obtained previously from the analysis of experiments on $^{87}\mathrm{Rb}\text{\ensuremath{-}}^{87}\mathrm{Rb}$ collisions. We find resonances that occur at very low magnetic fields, below 10G10\phantom{\rule{0.3em}{0ex}}\mathrm{G}10G, which may be useful for entanglement generation in optical lattices or atom chip magnetic traps.
A rigorous quantum theory of atomic collisions in the presence of radio frequency (rf) magnetic fields is developed and applied to elucidate the effects of combined dc and rf magnetic fields on ultracold collisions of Rb atoms. We show that rf fields can be used to induce Feshbach resonances, which can be tuned by varying the amplitude and frequency of the rf field. The rf-induced Feshbach resonances occur also in collisions of atoms in low-field-seeking states at moderate rf field strengths easily available in atom chip experiments, which opens up the world of tunable interactions to magnetically trappable atomic quantum gases.
Ultracold Cs2_22​ Feshbach Spectroscopy
We have observed and located more than 60 magnetic field-induced Feshbach resonances in ultracold collisions of ground-state 133^{133}133Cs atoms. These resonances are associated with molecular states with up to four units of rotational angular momentum, and are detected through variations in the elastic, inelastic, and radiative collision cross sections. These observations allow us to greatly improve upon the interaction potentials between two cesium atoms and to reproduce the positions of most resonances to accuracies better than 0.5%. Based on the relevant coupling scheme between the electron spin, nuclear spin, and orbital angular momenta of the nuclei, quantum numbers and energy structure of the molecular states beneath the dissociation continuum are revealed. Finally, we predict the relevant collision properties for cesium Bose-Einstein condensation experiments.
The research described in this thesis is part of an international effort with the aim of studying ultracold quantum degenerate gas samples like Bose-Einstein condensates and Fermi degenerate systems, consisting of atoms confined in magnetic or optical traps. The behavior of such samples is governed by the inter-atomic interactions and the resulting properties of the atom-atom scattering. At the relevant temperatures of 1nK to 10µK a key property is the atom-atom scattering length a. In chapter 2 a theoretical method is presented which enables one to describe the interaction and scattering of (ultra)cold atoms to unprecedented precision. It is also unparalleled in comprehensiveness: it allows the prediction of a large and varied set of experimental data for all isotopes of the same element. The method relies on the extraction from experiments of a few (phase) parameters which completely summarize the behavior of the atoms in the (ultra)cold regime. In chapter 3 the method is applied to the "workhorses" of cold-atom physics: the atomic species 85Rb and 87Rb. We extract the foregoing parameters to a very high precision from several recent high precision experiments, allowing us to predict e.g. the 87Rb spinor condensate to be ferromagnetic: a prediction for which the scattering length has to be calculated with a precision better than 1%. We also predict Feshbach resonances at experimentally accessible magnetic field strengths; resonances searched for and found by the experimental group of Rempe. In close collaboration with his group we "fine-tune" the interaction parameters found previously, by making use of only one of the observed resonances. We then obtain agreement with 42 out of the observed 43 resonance field strengths and are able to identify bound states inducing the Feshbach resonances at these locations. Chapter 4 describes the results of this research. With a thorough understanding of the rubidium interactions, we then switch to lithium which has a fermionic (6Li) and a bosonic (7Li) isotope. Both are being used in cold-atom experiments. In chapter 5 we evaluate the interaction parameters for lithium allowing us to predict magnetic field strengths for which a sample of fermionic 6Li atoms can be regarded as strongly interacting. Furthermore, a three-level method for measuring mean-field shifts, based on radio-frequency techniques, is introduced. For weak interactions we find proportionality of resonance shifts to interaction strengths. In the strongly interacting regime, however, these shifts become very small reflecting the quantum unitarity limit and many-body effects. Most interesting is the fact that in this regime the shifts are small both for large positive a and for large negative a, likely reflecting the universality of the interaction energy. In chapters 6 and 7 the interactions between lithium atoms are reinvestigated, making use of newly available experimental data and with the updated interaction parameters special attention is paid to locating field strengths at which magnetically tunable Feshbach resonances occur in the scattering of lithium atoms. In chapter 6 scattering events in a gas of (fermionic) 6Li atoms are studied. In chapter 7 we show that a consistent description of the 6Li+6Li system can be given. We discuss theoretical uncertainties for the position of the wide 6Li Feshbach resonance and present an analytic scattering model for this resonance, based on the inclusion of a field-dependent virtual open-channel state. We predict new Feshbach resonances for the 6Li-7Li system, and their importance for different types of crossover superfluidity models is discussed. Molecules created by magnetically sweeping over these resonances will have a fermionic character. One magnetic field strength is predicted at which two different fermionic molecules can be created simultaneously.
Due to atomic interactions, a dilute gas Bose-Einstein condensate acquires a self- energy proportional to the two-body scattering length a. This self-energy strongly influences the stability, formation rate, size and shape, collective excitations, and other properties of a condensate. For a given atomic species at zero magnetic field, the scattering length is fixed, and this had led to a rather limited range of interaction strengths in experiments. However, it has been predicted that a magnetically tunable Feshbach resonance could be used to strongly modify scattering lengths [1]. We have observed such a Feshbach resonance in collisions of ultracold 85Rb(f =2, mf=−2) atoms in a magnetic field B. From our measured resonance position and width, we infer that the scattering length a2,−2 for collisions of these atoms has the dispersive resonance form.
We investigate the interactions between ultracold alkali-metal atoms and closed-shell atoms using electronic structure calculations on the prototype system Rb+Sr. There are molecular bound states that can be tuned across atomic thresholds with a magnetic field and previously neglected terms in the collision Hamiltonian that can produce zero-energy Feshbach resonances with significant widths. The largest effect comes from the interaction-induced variation of the Rb hyperfine coupling. The resonances may be used to form paramagnetic polar molecules if the magnetic field can be controlled precisely enough.