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Frontiers in Optics

Laser Spectroscopy of Ultracold Metastable Helium Atoms

L. J. Byron, Oscar Turazza, R. G. Dall, Andrew G. Truscott, K. G. H. Baldwin

Published Jan 1, 2006• 0 citations
Publisher

Abstract

A Bose-Einstein condensation experiment is used to create ultracold metastable helium (23S1) atoms which are probed by a 389nm laser connecting with the 33P state to study photoassociation in the short-lived molecular states thus created.
DOI
10.1364/fio.2006.fthq7

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This article first provides guide lines for the understanding of laser cooling and Bose Einstein Condensation, with a general bibliography of the domain. Some details are given about the case of an ultracold gas of helium atoms in the 23S1 metastable state. Obtention of BEC will be recalled, with discussion of the inhibition of Penning ionization collisions. Recent studies at ENS with photoassociation methods will be summarized, including the formation of giant dimers providing another example of ionization inhibition.
During the last decades the study of cold atoms has grown in a great measure. Research in this field has been made possible due to the development of laser cooling and trapping techniques. We use laser cooling to cool helium atoms down to a temperature of 1 mK and we are able to trap 106 atoms in our magneto-optical trap. The helium atoms are in a metastable state, the He 23S1 state, which has a lifetime of more than 2 hours. With cold atoms phenomena can be studied that are not accessible using thermal atoms, such as high resolution spectroscopy. Furthermore cold atoms are the first step towards Bose-Einstein condensation. Cold alkali-metal atoms have been extensively studied, using photoassociation spectroscopy. In this thesis the first photoassociation results for rare gas atoms, namely metastable helium atoms will be discussed. Various experiments are described and an analysis of the results is given.
Photoassociation of metastable He (2/sup 3/S/sub 1/) atoms at ultra low temperatures close to the BEC phase transition is studied, which was achieved previously in an Ioffe-Pritchard magnetic trap and detected optically through absorption imaging of the optical density profile. In the present experiment, the cloud is brought close to the BEC transition by evaporation and then illuminated by laser pulse tunable around the three (2/sup 3/S/sub 1/-2/sup 3/P/sub 0,1,2/) resonance lines at 1083 nm. A subsequent optical density measurement is used to detect any increases in the trap loss rate that may have been caused by the pulse. The experiment is particularly interested in detecting losses due to the production of ultracold molecules by photoassociation (PA), and in finding several weakly bound S-P states that have not previously been detected.
We produce giant, purely long-range helium dimers by photoassociation of metastable helium atoms in a magnetically trapped, ultracold cloud. The photoassociation laser is detuned close to the atomic 2(3)S1-2(3)P0 line and produces strong heating of the sample when resonant with molecular bound states. The temperature of the cloud serves as an indicator of the molecular spectrum. We report good agreement between our spectroscopic measurements and our calculations of the five bound states belonging to a 0(+)(u) purely long-range potential well. These previously unobserved states have classical inner turning points of about 150a(0) and outer turning points as large as 1150a(0).