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Journal of Modern Optics

Three-photon electromagnetically induced absorption and transparency in an inhomogeneously broadened atomic vapour

C. Y. Ye, Alexander S. Zibrov, Yuri V. Rostovtsev, Andrey B. Matsko, Marlan O. Scully

Published Nov 1, 2002• 14 citations
Publisher

Abstract

We study both theoretically and experimentally three-photon electromagnetically induced transparency and electromagnetically induced absorption resonances in inhomogeneously broadened 85 Rb atomic vapour driven by probe and drive laser radiations. We observe narrow Doppler-free absorption as well as transmission resonances for the probe field when the driving laser field is redshifted from the D1 or D2 lines of 85Rb; the frequency difference between the drive and probe fields is equal to the hyperfine splitting of the ground state of the atoms, and the probe field is tuned to the centre of the Doppler broadened atomic transition. We theoretically study the spectroscopic effect in both homogeneously and inhomogeneously broadened media. Our numerical simulations are in good agreement with the experimental results.

DOI
10.1080/0950034021000011266

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We study both theoretically and experimentally three-photon electromagnetically induced transparency and electromagnetically induced absorption resonances in inhomogeneously broadened 85 Rb atomic vapour driven by probe and drive laser radiations. We observe narrow Doppler-free absorption as well as transmission resonances for the probe field when the driving laser field is redshifted from the D1 or D2 lines of 85Rb; the frequency difference between the drive and probe fields is equal to the hyperfine splitting of the ground state of the atoms, and the probe field is tuned to the centre of the Doppler broadened atomic transition. We theoretically study the spectroscopic effect in both homogeneously and inhomogeneously broadened media. Our numerical simulations are in good agreement with the experimental results.
We study the phenomenon of electromagnetically induced transparency (EIT) in room-temperature Rb vapour under conditions of a strong probe laser. The atoms form a ladder system with the lower transition coupled by the probe laser and the upper transition coupled by the control laser. Density-matrix analysis of the system shows that, for zero-velocity atoms, the strong probe beam causes a reduction in absorption and broadening of the profile. But the lineshape after thermal averaging shows a splitting of the EIT resonance and enhanced absorption near line centre. The experimental observations in 85Rb^{85}Rb85Rb agree qualitatively with the predicted lineshapes.
An electromagnetically induced transparency is observed at one arm of a three-level \ensuremath{\Lambda}-type system in a rubidium D1 line (794.8 nm) with an 85% reduction in absorption, when a pumping field is present at the other arm. This reduction in absorption for the weak probe field is due to the atomic coherence produced by the strong pumping field. This experiment is done in a Rb vapor cell at room temperature with cw diode lasers for both pumping and probe beams in a Doppler-free configuration. A simple theoretical treatment including Doppler broadening is in good qualitative agreement with the experimental measurement.
Atomic coherence resonances such as electromagnetically induced transparency (EIT) and electromagnetically induced absorption (EIA) signals are observed in a Doppler broadened multi-level system for the D 2 line of 85 Rb atoms in a vapour cell considering different types of atom–laser coupling schemes. Besides the coherence resonances, the nonlinear resonances like velocity selective optical pumping (VSOP) dips and velocity selective resonances (VSR) are also observed for the non-zero velocity selective groups of atoms. In the presence of pump, control and probe laser fields, we observe two EIT signals in a double Λ-type system and two EIA signals in a double V -type system. We are able to see the EIA signal for the non-zero velocity group of atoms when the pump laser is locked with an open transition by a small red detuning. We also report the experimental observation of simultaneous EIT and EIA signals in a (Λ+ V )-type system. The effect of frequency tuning of the control laser is also studied in the presence of the frequency locked pump laser. A simple theoretical analysis explains the experimental results.
We demonstrate experimentally the effect of a three-photon electromagnetically induced transparency in hot 85Rb{}^{85}\mathrm{Rb}85Rb atomic vapor driven by two coherent electromagnetic fields. The narrow transparency window is observed on the background of high-contrast Doppler-free subnatural absorption resonance. Our analytical calculations and numerical simulations are in good agreement with the experimental data. Both the transparency and the absorption resonances can find applications in high-precision metrology.
We develop a theory of electromagnetically induced transparency in a three-level, ladder-type Doppler-broadened medium, paying special attention to the case where the coupling and probe beams are counterpropagating and have similar frequencies, so as to reduce the total Doppler width of the two-photon process. The theory is easily generalized to deal with the \ensuremath{\Lambda} configuration, where the ideal arrangement involves two copropagating beams. We discuss different possible regimes, depending on the relative importance of the various broadening mechanisms, and identify ways to optimize the absorption-reduction effect. The theory is compared to the results of a recent experiment (on a ladder-type system), using the Rb D2 line, with generally very good agreement. The maximum absorption reduction observed (64.4%) appears to be mostly limited by the relatively large (\ensuremath{\sim}5 MHz) linewidth of the diode lasers used in our experiment.