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Optics Express

Mechanism of the metallic metamaterials coupled to the gain material

Zhixiang Huang, Sotiris Droulias, Thomas Koschny, Costas M. Soukoulis

Published Oct 11, 2014• 16 citations
Publisher

Abstract

We present evidence of strong coupling between the gain material and the metallic metamaterials. It is of vital importance to understand the mechanism of the coupling of metamaterials with the gain medium. Using a four-level gain system, the numerical pump-probe experiments are performed in several configurations (split-ring resonators (SRRs), inverse SRRs and fishnets) of metamaterials, demonstrating reduction of the resonator damping in all cases and hence the possibility for loss compensation. We find that the differential transmittance ΔT/T can be negative in different SRR configurations, such as SRRs on the top of the gain substrate, gain in the SRR gap and gain covering the SRR structure, while in the fishnet metamaterial with gain ΔT/T is positive.

DOI
10.1364/oe.22.028596

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We present evidence of strong coupling between the gain material and the metallic metamaterials. It is of vital importance to understand the mechanism of the coupling of metamaterials with the gain medium. Using a four-level gain system, the numerical pump-probe experiments are performed in several configurations (split-ring resonators (SRRs), inverse SRRs and fishnets) of metamaterials, demonstrating reduction of the resonator damping in all cases and hence the possibility for loss compensation. We find that the differential transmittance ΔT/T can be negative in different SRR configurations, such as SRRs on the top of the gain substrate, gain in the SRR gap and gain covering the SRR structure, while in the fishnet metamaterial with gain ΔT/T is positive.
We establish a new approach for pump-probe simulations of metallic metamaterials coupled to the gain materials. It is of vital importance to understand the mechanism of the coupling of metamaterials with the gain medium. Using a four-level gain system, we have studied light amplification of arrays of metallic split-ring resonators with a gain layer underneath. We find that the differential transmittance ΔT/T can be negative for split-ring resonators on the top of the gain substrate, which is not expected, and ΔT/T is positive for the gain substrate alone. These simulations agree with pump-probe experiments and can help to design new experiments to compensate for the losses of metamaterials.
We numerically investigate loss compensation and transmission in pump-probe experiments in resonant metamaterials with gain using an FDTD algorithm coupled to semiclassical rate equations. We observe differential transmittance signals from the coupled system that are a factor of four to five larger than for the bare quantum well. We observe a more rapid temporal decay of the differential transmittance signal for the coupled system compared to the bare quantum well. The effective metamaterial gain beyond the bare quantum-well gain, leading to a significant reduction of the metamaterial’s losses, but no complete compensation of the losses. We explain experimentally observed negative differential transmission by gain-dependent impedance. Article not available.
This study demonstrates a metamaterial with two coupled split-ring resonators (SRR) can exhibit an effect reminiscent of electromagnetically induced transparency (EIT), a coherent process normally observed in three-level atomic media. The coupling between two SRR induces a frequency splitting in the spectral response of the metamaterial, opening up a narrow transmission band in the centre of the absorption line. The obtained reduction in group velocity together with the low absorption is useful for a variety of slow-light applications, without the need for the extreme cooling or the large magnetic fields that are typically required for EIT in atomic systems.
Metamaterials, or artificial materials with optical properties not known for natural materials, have recently been used to demonstrate unusual optical phenomena, such as negative refraction, perfect lenses, subwavelength components, and electromagnetic invisibility cloaks. Most of the metamaterials designed to date are periodic structures containing a single resonating element in each unit cell, such as a split-ring resonator (SRR), a cutwire, or a slab-wire pair [1]. In this contribution, we demonstrate that a metamaterial with two coupled SRRs can exhibit an effect reminiscent of electromagnetically induced transparency (EIT), a coherent process normally observed in three-level atomic media [2]. Due to this process, a small transparency window with low absorption appears in the spectral response of the metamaterial. Simultaneously, extremely steep normal dispersion is observed in the transparency window, which is useful for slow-light applications.
Two independent significant developments have challenged our understanding of light-matter interaction, one, involves the artificially structured materials known as metamaterials, and the other, relates to the coherent control of quantum systems via the quantum interference route. We theoretically demonstrate that one can engineer the electromagnetic response of composite metamaterials using coherent quantum interference effects. In particular, we predict that these composite materials can show a variety of effects ranging from dramatic reduction of losses to switchable ultraslow-to-superluminal pulse propagation. We propose parametric control of the metamaterials by active tuning of the capacitance of the structures, which is most efficiently engineered by embedding the metamaterial structures within a coherent atomic/molecular medium. This leads to dramatic frequency dependent features, such as significantly reduced dissipation accompanied by enhanced filling fraction. For a Split-ring resonator medium with magnetic properties, the associated splitting of the negative permeability band can be exploited for narrow band switching applications at near infrared frequencies involving just a single layer of such composite metamaterials.
Nanoplasmonic metamaterials are an exciting new class of engineered media that promise a range of important applications, such as subwavelength focusing, cloaking, and slowing/stopping of light. At optical frequencies, using gain to overcome potentially not insignificant losses has recently emerged as a viable solution to ultra-low-loss operation that may lead to next-generation active metamaterials. Maxwell-Bloch models for active nanoplasmonic metamaterials are able to describe the coherent spatiotemporal and nonlinear gain-plasmon dynamics. Here, we extend the Maxwell-Bloch theory to a Maxwell-Bloch Langevin approach-a spatially resolved model that describes the light field and noise dynamics in gain-enhanced nanoplasmonic structures. Using the example of an optically pumped nanofishnet metamaterial with an embedded laser dye (four-level) medium exhibiting a negative refractive index, we demonstrate the transition from loss-compensation to amplification and to nanolasing. We observe ultrafast relaxation oscillations of the bright negative-index mode with frequencies just below the THz regime. The influence of noise on mode competition and the onset and magnitude of the relaxation oscillations is elucidated, and the dynamics and spectra of the emitted light indicate that coherent amplification and lasing are maintained even in the presence of noise and amplified spontaneous emission.