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Nature Photonics

Controlling the dipole force

Juan Ortigoso, Mirta Rodríguez

Published Nov 30, 2009• 4 citations
Publisher
DOI
10.1038/nphoton.2009.228

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We measure the role of field-induced alignment on the dipole force for molecules using a single focused nonresonant laser beam. We show that through the alignment process we can modify the effective polarizability by field polarization and thus control the center-of-mass motion of the molecule. We observe a maximum change of 2020%20 in the dipole force on CS2{}_{2}2​ molecules when changing from linearly to circularly polarized light. Additionally, the effect of the dipole force on different vibrational states is also studied.
We describe simulations that illustrate the possibility for manipulating the position correlation of atoms in a magneto-optical trap (MOT) using the dipole–dipole interaction. The control scheme utilizes a narrow band laser that is detuned to the high-frequency side of a single-photon Rydberg transition in an isolated atom. As two atoms move near each other, they can be laser excited to repelling diatomic Rydberg–Rydberg potential energy curves which halt their approach. By chirping the laser from large to small detunings, atoms in a MOT can be pushed apart by dipole–dipole forces, thereby controlling nearest-neighbor interactions. Alternatively, by holding the frequency of the Rydberg excitation laser fixed as the MOT is loaded, it should be possible to limit the minimum distance between atoms to a prescribed value.