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Optics Communications

Lifetime measurement of the (5d6p)3D3 state of barium by dye-laser spectroscopy

Gilbert O. Brink, A. Glassman, R. Gupta

Published Apr 1, 1980• 6 citations
Publisher
DOI
10.1016/0030-4018(80)90084-x

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Whether the transitions between 6s5d 3D and 5d6p 3F can be used for laser cooling of barium heavily depends upon the transition probabilities of 5d6p 3F-5d2 3F. Taking the transition 6s5d 3D3-5d6p 3F4 as a scale, the leakage rate of 5d6p 3F4-5d2 3F was used to evaluate the transition probabilities. 706 nm laser pulses with different durations were applied to a barium atomic beam for 6s5d 3D3-5d2 3F4 optical pumping, and the remaining percentages in 6s5d 3D3 were measured. After exponential fitting, the transition probability of 5d6p 3F4-5d2 3F3,4 was determined to be 2.1(4)×104 s−1, which is in agreement with theoretical calculations using the scaled Thomas-Fermi-Dirac method.

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Whether the transitions between 6s5d 3D and 5d6p 3F can be used for laser cooling of barium heavily depends upon the transition probabilities of 5d6p 3F-5d2 3F. Taking the transition 6s5d 3D3-5d6p 3F4 as a scale, the leakage rate of 5d6p 3F4-5d2 3F was used to evaluate the transition probabilities. 706 nm laser pulses with different durations were applied to a barium atomic beam for 6s5d 3D3-5d2 3F4 optical pumping, and the remaining percentages in 6s5d 3D3 were measured. After exponential fitting, the transition probability of 5d6p 3F4-5d2 3F3,4 was determined to be 2.1(4)×104 s−1, which is in agreement with theoretical calculations using the scaled Thomas-Fermi-Dirac method.