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Journal of Modern Optics

The role of coherent effects in mode bistability of a gas laser in inhomogeneous medium

Gabriela Wa̧sik, Gerd Leuchs

Published Mar 1, 2001• 0 citations
Publisher

Abstract

We have studied microscopic effects leading to mode competition in an inhomogeneously broadened medium of a gas laser with a weakly anisotropic cavity. The polarization bistability observed in some lasers, which is believed to be caused by hole burning, we attribute to microscopic coherent effects induced by two light fields. Due to these effects one field can be coupled with another. Hole burning is found to be important, but not crucial. The exact solution of the equation of motion for field amplitudes is compared with the third order approximation of perturbation theory. The role of four wave mixing, important for bistability of axial modes in a homogeneously broadened medium, is discussed.

DOI
10.1080/09500340108230939

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We have studied microscopic effects leading to mode competition in an inhomogeneously broadened medium of a gas laser with a weakly anisotropic cavity. The polarization bistability observed in some lasers, which is believed to be caused by hole burning, we attribute to microscopic coherent effects induced by two light fields. Due to these effects one field can be coupled with another. Hole burning is found to be important, but not crucial. The exact solution of the equation of motion for field amplitudes is compared with the third order approximation of perturbation theory. The role of four wave mixing, important for bistability of axial modes in a homogeneously broadened medium, is discussed.
The instabilities in homogeneously broadened lasers, which we described in the previous chapter, have a paradigmatic importance because they arise in models which allow one to perform the linear-stability analysis in a simple analytic form. The treatment of the corresponding instabilities in the case of in homogeneously broadened lasers is substantially more complex in general. However, it is very interesting because, as we shall see, the instabilities arise in parametric domains that are much more accessible from the experimental viewpoint. A related issue is that of the possibility of multimodal emission in a laser. It is common knowledge that in order to attain multimode emission it is necessary to have a sort of in homogeneity in the gain medium, because in a completely homogeneous configuration all modes interact with all atoms, and the arising competition among modes implies that only one of them survives. There are basically two main kinds of in homogeneity, the first is of spatial nature and the other is of spectral nature. The first kind is realized in Fabry–Perot lasers, because different cavity modes interact with atoms at different spatial positions in the cavity thanks to the standing-wave configuration of the field and to the consequent phenomenon of spatial hole- burning (see Section 14.2 and Fig. 14.1). This circumstance is capable of weakening the mode–mode competition and allowing multimode operation. In unidirectional ring lasers, on the other hand, there is an “inhomogeneous” configuration in the case of inhomogeneous broadening, because different groups of atoms have different transition frequencies and therefore interact with different modes thanks to the spectral hole-burning (see Section 15.2 and Fig. 15.3). Again, this weakens the mode–mode competition and allows multimode operation. However, these are qualitative considerations, and the only reliable and quantitative method to determine the possibility of multimodal operation is the linear-stability analysis of the single-mode stationary solutions.
The effects of inhomogeneous broadening, spatial hole burning, and Gaussian beams are calculated for the four coefficients derived in previous papers in this series [Phys. Rev. A 31, 3112 (1985); 31, 3124 (1985)] on the quantum theory of multiwave mixing. These coefficients uniformly describe how one or two strong classical-field modes and one or two weak quantum-field modes interact in a two-level medium. The phenomena for which this theory is applicable includes resonance fluorescence, Rayleigh scattering, laser and/or optical bistability instabilities, and phase conjugation. The averaged formulas are illustrated by resonance-fluorescence spectra. We find the sidepeaks can be ``washed out'' and that asymmetries can occur.
Unstable and bistable behavior has been predicted recently in multimode homogeneously broadened lasers as a function of the detuning between the cavity and the atomic frequencies. As an example of a device for which most required physical conditions for the appearance of this instability are satisfied, we have analyzed the behavior of a low-pressure (10–20 Torr) CO2 laser. The operating parameters (relaxation rates for the population inversion, 104s−1, and for the polarization, 108s−1) restrict the accessible range of theoretically expected phenomena to a stable intensity output without evidence of stable self-pulsing. However, mode–mode competition is responsible for bistability in both the intensity and the operating frequency on varying the detuning parameter. This behavior is confirmed by additional observations of the transient that accompanies the jump between the two stable branches. We have also studied the effect of varying the cavity losses and discovered bistability also in the vicinity of the threshold for laser action. This kind of behavior is not predicted by the plane wave Maxwell-Bloch equations but can be explained in terms of a radial gain profile. Both effects—mode–mode competition and transverse—lead to a variety of bistable behaviors depending on gas pressure and discharge current.
A new semiclassical model of the active medium of a gas laser and a description of its interaction with a classical electromagnetic field are reported. The model is based upon an exact microscopic formulation of the density of the active medium in a suitably defined semiclassical state space. Field-medium interaction mechanisms are studied by coupling the equation describing the dynamics of this density with Maxwell's field equations and the Schr\"odinger wave equation. Coupled stochastic nonlinear equations are formulated and quasilinear techniques are employed to effect their solutions. Wave-dipole correlations, the dominant nonlinearity, is shown to effect stability, produce the phenomena of hole burning, mode coupling, and frequency conversion, and to provide the mechanism whereby nonresonant pump field energy is converted into resonant laser oscillations.
Using classical fields and the density-matrix formalism, we analyze the nonlinear characteristics of a gas laser amplifier subject to an axial magnetic field, operating with two optical-frequency signals of arbitrary polarization. Perturbational solutions, valid for relatively weak intensities, are obtained which describe the saturation interaction of the signals and the generation of combination tones. An arbitrary amount of Doppler broadening is considered throughout. The simple $J=1\ensuremath{\rightarrow}J=0$ model is found convenient to describe the physical processes taking place. In general, however, the interactions are found to depend on the JJJ values of the levels. We find that only saturation and no combination-tone generation occurs for two opposite circularly polarized signals, while both effects are, in general, present for two linearly or elliptically polarized fields. The limiting case of zero magnetic field is examined separately. It is also found that in many cases the medium is made effectively anisotropic by the nonlinear interactions. Applications to measurements of atomic parameters such as JJJ values, ggg values, and lifetimes are discussed.