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Applied Physics Letters

Decay times of excitons in lattice-matched InGaAs/InP single quantum wells

Igal Brener, D. Gershoni, D. Ritter, Morton B. Panish, Robert A. Hamm

Published Mar 4, 1991• 10 citations
Publisher

Abstract

A study of the photoluminescence decay times in lattice-matched InGaAs/InP single quantum wells grown by two different epitaxial techniques is presented. We show that these decay times can be measured directly using a nonlinear photoluminescence autocorrelation technique. A model based on the saturation of localized exciton states describes the temporal behavior and the optical nonlinearities observed very well.

DOI
10.1063/1.104457

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A study of the photoluminescence decay times in lattice-matched InGaAs/InP single quantum wells grown by two different epitaxial techniques is presented. We show that these decay times can be measured directly using a nonlinear photoluminescence autocorrelation technique. A model based on the saturation of localized exciton states describes the temporal behavior and the optical nonlinearities observed very well.
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Time-resolved photoluminescence (PL) of excitonic molecules in GaAs quantum wells (QW's) reveals an initial transient characterized by a finite rise and an extremely fast nonexponential decay [H. Wang, J. Shah, and T. C. Damen et al., Solid State Commun. 98, 807 (1996)]. The transient is attributed to coherent quantum evolution towards the molecule ground state of two optically correlated excitons, ${\ensuremath{\sigma}}^{+}$ and ${\ensuremath{\sigma}}^{\ensuremath{-}},$ which undergo the Coulombic attraction. In the present paper, we develop a theory of the transient PL and fit the experimental data. The radiative decay of a quasi-two-dimensional (2D) excitonic molecule is analyzed with the giant oscillator strength model adapted to QW's and with the bipolariton model. Within the 2D bipolariton model, the main ``hidden'' channel of the radiative decay of an excitonic molecule is the resonant dissociation into two outgoing interface (surface) polaritons rather than the observable decay into the bulk radiative modes. We conclude that quasi-2D molecules dissociate already within the initial transient of PL, while the following exponential decay of the molecule-mediated PL is due to the escape of secondary interface polaritons into the bulk modes. According to the 2D bipolariton model, the sequence ``two incoming $\mathrm{photons}\ensuremath{\rightarrow}\mathrm{two}$ virtual $\mathrm{excitons}\ensuremath{\rightarrow}2\mathrm{D}$ $\mathrm{molecule}\ensuremath{\rightarrow}\mathrm{two}$ outgoing interface polaritons'' is a completely coherent process. The fit of the time-resolved molecule-mediated PL provides us with numerical estimates of the exciton-photon coupling in GaAs QW's.
Ultrafast absorption saturation in an exciton Bragg reflector, consisting of InGaAs quantum wells embedded in InP/InGaAsP Bragg layers, is characterized by pump-induced transient reflectance spectroscopy at room temperature. Spectral modulation of the reflected probe pulses is caused by ultrafast absorption saturation of excitons in the quantum wells. The spectral modulation leads to an optical phase shift of 1.6 π. The exciton-induced phase shift is more than four times as large as that induced by free carriers in a Bragg reflector.
Abstract : In this paper we describe a detailed study of the complete time evolution of the optical nonlinearities of type-11 GaAs/AlAs quantum wells using nanosecond and femtosecond pump/probe spectroscopy. We explain these nonlinearities by solving the generalized Wannier equation for the case of a type-II quantum-well structure. In contrast to the usual type-I quantum-wells, we observe different shifts and saturations of light- and heavy-hole excitons as well as the absence of gain. The dominant effects are a blue shift and saturation of the heavy-hole (HH) exciton.
Absorption spectra of strained InGaAs/InP quantum wells exhibit a single, unusually large exciton feature. 60% quenching is obtained for 4.3 mW Nd:YAG effective pump power at a wavelength of 1.064 mu m. A simple two-level formula fits well the behaviour at the exciton peak, and absorption spectra are reasonably approximated by a standard two-dimensional exciton model. Saturation intensities calculated with these techniques range around 200 W cm-2. Finally the Kramers-Kronig relations are used to calculate the associated refractive index change.