Journal of Applied Spectroscopy

Concentration depolarization of fluorescence in systems with nonuniformly broadened electronic levels

V. T. Koyava, Владимир Иванович Попечиц, A. M. Sarzhevskii

Published Jun 1, 1980• 1 citation

Publisher

DOI: 10.1007/bf00604284

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Journal of Applied Spectroscopy

Concentration depolarization of fluorescence in systems with nonuniformly broadened electronic levels

V. T. Koyava, Владимир Иванович Попечиц, A. M. Sarzhevskii

Published Jun 1, 1980• 1 citation

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DOI: 10.1007/bf00604284

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Laser-induced fluorescence line narrowing has been observed for the first time in a nonresonantly excited rare-earth system. Excitation with the 4727-\AA{} ${A}^{+}$ line into the $^{4}G_{\frac{11}{2}}$ level of ${\mathrm{Nd}}^{3+}$ in glass results in narrowing of transitions from the $^{4}F_{\frac{3}{2}}$ to both the $^{4}I_{\frac{9}{2}}$ ground manifold and the $^{4}I_{\frac{11}{2}}$ excited manifold. The concentration dependence of the line narrowing provides information regarding resonant ion-ion energy transfer within the inhomogeneously broadened system.Laser-induced fluorescence line narrowing has been observed for the first time in a nonresonantly excited rare-earth system. Excitation with the 4727-\AA{} ${A}^{+}$ line into the $^{4}G_{\frac{11}{2}}$ level of ${\mathrm{Nd}}^{3+}$ in glass results in narrowing of transitions from the $^{4}F_{\frac{3}{2}}$ to both the $^{4}I_{\frac{9}{2}}$ ground manifold and the $^{4}I_{\frac{11}{2}}$ excited manifold. The concentration dependence of the line narrowing provides information regarding resonant ion-ion energy transfer within the inhomogeneously broadened system.

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Laser-induced fluorescence line narrowing has been observed for the first time in a nonresonantly excited rare-earth system. Excitation with the 4727-\AA{}

{A}^{+}

line into the

^{4}G_{\frac{11}{2}}

level of

{\mathrm{Nd}}^{3+}

in glass results in narrowing of transitions from the

^{4}F_{\frac{3}{2}}

to both the

^{4}I_{\frac{9}{2}}

ground manifold and the

^{4}I_{\frac{11}{2}}

excited manifold. The concentration dependence of the line narrowing provides information regarding resonant ion-ion energy transfer within the inhomogeneously broadened system.