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Soviet physics. Doklady

Polarization of fluorescence produced by transitions from upper excited levels

I. E. Zalesskii, V. N. Kotlo, A. N. Sevchenko, К. Н. Соловьев, S. F. Shkirman

Published Mar 1, 1975• 0 citations
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The resonant excitation of the sodium D2 transition by laser radiation was investigated experimentally in this thesis. Line polarization measurement of the resonance fluorescence was employed to investigate the excitation process. The sodium atoms, which were collimated in a very narrow beam, were excited by a monochromatic laser beam with the frequency tuned to resonance with the 32S 112(F=2) - 32P312 hyperfine transition. The direction of the laser beam was perpendicular to the atomic beam and the fluorescence photons were detected along a direction perpendicular to both the laser and atomic beams. The experimental measurements were performed to determine the effect due to the variation of the laser intensity and frequency on the line polarization. A theoretical expression of the line polarization as a function of density matrix elements of the upper excited hyperfine sub -states was derived. A full quantum electrodynamic theory was used to derive an atomic operator equation of motion which was needed to calculate atomic operator elements. These elements then yielded the corresponding density matrix elements. The experimental results and the theoretical modelling were in a good agreement. The first experimental results for the line polarization of the highly excited states, 42D512 and 42D312, are also presented. The use of two lasers enabled these highly excited states to be excited. The line polarization of the fluorescence for transitions from the 4D level down to lower states is derived in terms of the density matrix elements of the upper excited states. Two limiting cases for the theoretical predictions of the line polarization are considered.
The interaction of a four-level atom consisting of one excited state, two upper levels and one ground state is considered. We use one field to drive the transition between the excited state and the ground state, and simultaneously apply another field to couple two transitions from the upper-level doublet to the ground state. We investigate how to control the central linewidth of resonance fluorescence spectrum of the driven transition via quantum interference between two transitions from the upper doublet to the ground state of the atom. In the case of orthogonal dipole moments for the upper doublet and the ground state the widths of the central line and the sidebands of the resonance fluorescence spectrum are totally controlled by the spontaneous emission rate of the upper doublet when the applying field is sufficiently strong. When the dipole moments are parallel, the central linewidth can be much narrower than the linewidths of spontaneous emission of the excited state and of the upper doublet due to the quantum interference. The smaller the upper doublet splitting, the narrower the central linewidth. We also notice that when the upper levels are degenerate the resonance fluorescence spectrum may depend on the initial condition because of the quantum interference.