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Quantum Optics Journal of the European Optical Society Part B

Coherent transfer of photon momentum by adiabatic following in a dark state

Lori S. Goldner, Christoph Gerz, R. J. C. Spreeuw, S. L. Rolston, Christoph Ira Westbrook, William D. Phillips, P. Marte, P. Zoller

Published Aug 1, 1994• 16 citations
Publisher

Abstract

We demonstrate a new technique for the mechanical manipulation of atoms with light that may be used to deflect or split an atomic beam. This technique depends on the existence of an internal superposition state of the atom that is 'dark' to resonant excitation by a particular light field. An atom in a dark state may adiabatically follow a slowly varying light field in such a way that both the internal state and the atom's momentum are changed. Because the dark state never absorbs or fluoresces, the atomic coherence, necessary for atom interferometry, is preserved. We use laser-cooled Cs atoms to demonstrate the transfer of 8 photon momenta from the slowly varying laser field to the atom.

DOI
10.1088/0954-8998/6/4/016

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We have observed momentum transfer in cesium atoms using the process of adiabatic transfer between dark states. We have investigated the sensitivity of this process to Zeeman shifts and to the differences between the translational energies of the states involved. We have shown that, for a chosen velocity class, the resultant phase shifts of the magnetic substates can be canceled so a dark state is maintained. Two different laser polarization configurations were used to perform the experiments: two circularly polarized beams or a linearly and a circularly polarized beam. Results for each are presented. Finally we discuss the relevance of our results to atomic interferometry and consider methods to minimize the possible phase shifts introduced in an atomic interferometer based upon adiabatic transfer. \textcopyright{} 1996 The American Physical Society.

Physical Review A•Jan 1, 1996•42 citations
We demonstrate a new technique for the mechanical manipulation of atoms with light that may be used to deflect or split an atomic beam. This technique depends on the existence of an internal superposition state of the atom that is 'dark' to resonant excitation by a particular light field. An atom in a dark state may adiabatically follow a slowly varying light field in such a way that both the internal state and the atom's momentum are changed. Because the dark state never absorbs or fluoresces, the atomic coherence, necessary for atom interferometry, is preserved. We use laser-cooled Cs atoms to demonstrate the transfer of 8 photon momenta from the slowly varying laser field to the atom.
We have observed transfer of momentum and ground state population in laser-cooled cesium by adiabatic following of a slowly evolving light field. In this new technique for mechanical manipulation of atoms, spontaneous emission is suppressed since the atoms evolve in a ``dark'' state that follows the light field. This means that the phase coherence of the atom is preserved so that this technique is useful in the realization of coherent atomic beam splitters and mirrors. Our experimental results are in good agreement with optical Bloch equation calculations.
We describe a technique for creating superpositions of degenerate quantum states, such as are needed for beam splitters used in matter-wave optics, by manipulating the timing of three orthogonally polarized laser beams through which moving atoms (or molecules) pass; motion across the laser beams produces pulses in the atomic rest frame. As illustrated with representative simulations for transitions in metastable neon, a single pass through three overlapping laser beams can produce superpositions (with preselected phase) of atomic beams differing by transverse momentum corresponding to the momentum of four photons. Like the two-photon momentum transfer of the tripod linkage pattern which it extends, the method relies on controlled adiabatic time evolution in the Hilbert subspace of two degenerate dark states. It is thus a generalization to multiple dark states (and larger transfers of linear momentum to the atomic beam) of the single dark state occurring with the stimulated Raman adiabatic passage (STIRAP) technique, and therefore it is potentially insensitive to decoherence due to spontaneous emission. By extending the tripod-linkage system to more numerous degenerate states, the technique not only increases the atomic beam deflections but, as we demonstrate, allows control over the superposition phase and amplitudes. LIke other techniques based on adiabatic time evolution, the technique is robust with respect to variations of the intensity, timing, and other characteristics of the laser fields. Unlike STIRAP, the same robust partial population transfer occurs for opposite timings of the pulse sequence, as is needed for such procedures as Hadamard gates.
Two different research teams have taken a big step toward atom interferometry. They have succeeded in splitting atomic beams by using atoms in spin states that neither absorb nor reemit laser light. By proper adjustment of experimental conditions, atoms are changed from one spin state to another, without passing through the intermediary excited state. The atoms in essence absorb momentum from the laser photons, without absorption or emission of photons. The change in momentum deflects atoms in the proper spin state.
Coherent manipulations of atoms using laser light The internal structure of a particle - an atom or other quantum system in which the excitation energies are discrete - undergoes change when exposed to pulses of near-resonant laser light. This tutorial review presents basic concepts of quantum states, of laser radiation and of the Hilbert-space statevector that provides the theoretical portrait of probability amplitudes - the tools for quantifying quantum properties not only of individual atoms and molecules but also of artificial atoms and other quantum systems. It discusses the equations of motion that describe the laser-induced changes (coherent excitation), and gives examples of laser-pulse effects, with particular emphasis on two-state and three-state adiabatic time evolution within the rotating-wave approximation. It provides pictorial descriptions of excitation based on the Bloch equations that allow visualization of two-state excitation as motion of a three-dimensional vector (the Bloch vector). Other visualization techniques allow portrayal of more elaborate systems, particularly the Hilbert-space motion of adiabatic states subject to various pulse sequences. Various more general multilevel systems receive treatment that includes degeneracies, chains and loop linkages. The concluding sections discuss techniques for creating arbitrary pre-assigned quantum states, for manipulating them into alternative coherent superpositions and for analyzing an unknown superposition. Appendices review some basic mathematical concepts and provide further details of the theoretical formalism, including photons, pulse propagation, statistical averages, analytic solutions to the equations of motion, exact solutions of periodic Hamiltonians, and population-trapping "dark" states.
We have observed momentum transfer in cesium atoms using the process of adiabatic transfer between dark states. We have investigated the sensitivity of this process to Zeeman shifts and to the differences between the translational energies of the states involved. We have shown that, for a chosen velocity class, the resultant phase shifts of the magnetic substates can be canceled so a dark state is maintained. Two different laser polarization configurations were used to perform the experiments: two circularly polarized beams or a linearly and a circularly polarized beam. Results for each are presented. Finally we discuss the relevance of our results to atomic interferometry and consider methods to minimize the possible phase shifts introduced in an atomic interferometer based upon adiabatic transfer. \textcopyright{} 1996 The American Physical Society.