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Physical Review Letters

Momentum transfer in laser-cooled cesium by adiabatic passage in a light field

Lori S. Goldner, Christoph Gerz, R. J. C. Spreeuw, S. L. Rolston, Christoph Ira Westbrook, William D. Phillips, P. Marte, P. Zoller

Published Feb 14, 1994• 158 citations
Publisher

Abstract

We have observed transfer of momentum and ground state population in laser-cooled cesium by adiabatic following of a slowly evolving light field. In this new technique for mechanical manipulation of atoms, spontaneous emission is suppressed since the atoms evolve in a ``dark'' state that follows the light field. This means that the phase coherence of the atom is preserved so that this technique is useful in the realization of coherent atomic beam splitters and mirrors. Our experimental results are in good agreement with optical Bloch equation calculations.

DOI
10.1103/physrevlett.72.997

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We have observed transfer of momentum and ground state population in laser-cooled cesium by adiabatic following of a slowly evolving light field. In this new technique for mechanical manipulation of atoms, spontaneous emission is suppressed since the atoms evolve in a ``dark'' state that follows the light field. This means that the phase coherence of the atom is preserved so that this technique is useful in the realization of coherent atomic beam splitters and mirrors. Our experimental results are in good agreement with optical Bloch equation calculations.
We demonstrate a new technique for the mechanical manipulation of atoms with light that may be used to deflect or split an atomic beam. This technique depends on the existence of an internal superposition state of the atom that is 'dark' to resonant excitation by a particular light field. An atom in a dark state may adiabatically follow a slowly varying light field in such a way that both the internal state and the atom's momentum are changed. Because the dark state never absorbs or fluoresces, the atomic coherence, necessary for atom interferometry, is preserved. We use laser-cooled Cs atoms to demonstrate the transfer of 8 photon momenta from the slowly varying laser field to the atom.
We study atomic-beam deflection by adiabatic passage between Zeeman ground levels via Raman transitions induced by counterpropagating ${\mathrm{\ensuremath{\sigma}}}^{\ifmmode\pm\else\textpm\fi{}}$-polarized lasers. We show that complete population transfer between the ground states can be achieved, which corresponds to the scattering of the atomic wave packet into a single final momentum state by absorption and induced emission of laser photons. Although the lasers can be resonant, the excited state(s) are never populated during the adiabatic transfer, which suppresses the effects of spontaneous emission and preserves the coherence of the atomic wave function. This scheme has attractive features as a beam splitter and mirror for atomic interferometry.
We have demonstrated a coherent beam splitter for metastable helium based on adiabatic passage. Light from a homemade LNA laser at 1.083 {mu} is used to excite the {sup 3}S{sub 1}-{sup 3}P{sub 0} transition in a highly collimated beam of metastable helium. The atoms are first optically pumped into the m=0 and m=-1 sublevels. These sublevels are two independent {open_quotes}dark{close_quotes} states from which no further absorption is possible. Population is transferred adiabatically from the m = -1 level to the m =+1 level by means of two partially overlapping laser beams. As well as absorbing 2{h_bar} of angular momentum from the radiation field, the atoms initially in the m = -1 sublevel acquire 2{h_bar}k of linear momentum via an absorption/stimulated emission process. The process can be repeated back to m = -1, and we have demonstrated 4{h_bar}k and 6{h_bar}k coherent momentum transfer using successive interactions regions. The population initially in the m = 0 sublevel is undeflected by the light.
We describe a technique for creating superpositions of degenerate quantum states, such as are needed for beam splitters used in matter-wave optics, by manipulating the timing of three orthogonally polarized laser beams through which moving atoms (or molecules) pass; motion across the laser beams produces pulses in the atomic rest frame. As illustrated with representative simulations for transitions in metastable neon, a single pass through three overlapping laser beams can produce superpositions (with preselected phase) of atomic beams differing by transverse momentum corresponding to the momentum of four photons. Like the two-photon momentum transfer of the tripod linkage pattern which it extends, the method relies on controlled adiabatic time evolution in the Hilbert subspace of two degenerate dark states. It is thus a generalization to multiple dark states (and larger transfers of linear momentum to the atomic beam) of the single dark state occurring with the stimulated Raman adiabatic passage (STIRAP) technique, and therefore it is potentially insensitive to decoherence due to spontaneous emission. By extending the tripod-linkage system to more numerous degenerate states, the technique not only increases the atomic beam deflections but, as we demonstrate, allows control over the superposition phase and amplitudes. LIke other techniques based on adiabatic time evolution, the technique is robust with respect to variations of the intensity, timing, and other characteristics of the laser fields. Unlike STIRAP, the same robust partial population transfer occurs for opposite timings of the pulse sequence, as is needed for such procedures as Hadamard gates.
We propose and demonstrate a novel laser cooling mechanism applicable to particles with narrow-linewidth optical transitions. By sweeping the frequency of counter-propagating laser beams in a sawtooth manner, we cause adiabatic transfer back and forth between the ground state and a long-lived optically excited state. The time-ordering of these adiabatic transfers is determined by Doppler shifts, which ensures that the associated photon recoils are in the opposite direction to the particle's motion. This ultimately leads to a robust cooling mechanism capable of exerting large forces via a weak transition and with reduced reliance on spontaneous emission. We present a simple intuitive model for the resulting frictional force, and directly demonstrate its efficacy for increasing the total phase-space density of an atomic ensemble. We rely on both simulation and experimental studies using the 7.5 kHz linewidth 1 S 0 to 3 P 1 transition in 88 Sr. The reduced reliance on spontaneous emission may allow this adiabatic sweep method to be a useful tool for cooling particles that lack closed cycling transitions, such as molecules.
We propose a relatively robust scheme to implement quantum information transfer via adiabatic passage.When a Λ-type atom interacts with laser and cavity fields adiabatically,the state of the system evolves in a dark state.By the adiabatic passage,we can implement quantum information transfer of all the atomic states.Similarly,the scheme can be used to transfer a cavity mode state.The proposal is robust to restrain the atomic spontaneous emission noise,and transfers quantum information successfully.