We describe an atom-optical technique for producing large changes in the momentum of cold atoms using a pulsed standing wave of off-resonant light. Experimental results are presented showing how the efficiency and the amount of momentum transfer depend on the parameters of the light field. We also present a theoretical analysis and derive a closed formula which is in excellent agreement with the experimental data.
We describe an atom-optical technique for producing large changes in the momentum of cold atoms using a pulsed standing wave of off-resonant light. Experimental results are presented showing how the efficiency and the amount of momentum transfer depend on the parameters of the light field. We also present a theoretical analysis and derive a closed formula which is in excellent agreement with the experimental data.
In this thesis, the use of pulsed laser fields to control the center-of-mass motion of neutral atoms and molecules is studied both numerically and experimentally. In particular, we consider the use of a pulsed standing wave for the deflection of atomic beams, and develop novel types of mirrors for applications in atom and molecule optics. The research work shows that pulsed laser fields can be applied to form efficient mirrors for neutral particles regardless of the details of their internal energy-level structure. Moreover, it is shown that pulsed standing waves can also be utilized to efficiently deflect atomic beams. In the first part of the thesis, we study the effects of phase fluctuations of the laser field on the momentum distribution of atoms after interaction with a standing wave. Our numerical simulations show that the coherence properties of the laser field play a major role in diffraction of atoms, especially when using pulsed lasers. It turns out that the effects caused by the limited coherence time of the optical field are clearly observable as a transfer of atoms in momentum space to the region around zero momentum rather than to high momentum states. The numerical analysis of the pulsed standing-wave diffraction was complemented by experimental measurements of the deflection profiles of a beam of thermal sodium atoms. The experimental distributions were measured for a value of the coherence time intermediate between the Rabi period and the interaction time. A comparison of the results with an expected distribution calculated for a fully coherent interaction shows that the phase fluctuations of the light field drastically affect the achievable transverse momentum values. Based on our theoretical and experimental analysis of the diffraction profiles, we conclude that large deflection angles can be reached only when laser pulses with a Fourier-limited bandwidth are applied. The second part of the thesis concentrates on the development of pulsed mirrors for neutral atoms and molecules. In particular, we consider the use of an evanescent wave, formed in total internal reflection of light on a vacuum-dielectric interface, and of a standing wave as possible mirror configurations. Our numerical simulations of the pulsed evanescent-wave mirror show that atoms with initial velocities up to several tens of meters per second can be reflected already at the moderate field intensities of a few tens of MW/cm2. This allows pulsed evanescent waves to be applied in a compact setup to control the motion of thermal atomic beams, for which the traditional atom mirrors are suited only at grazing incidence. However, since the effective interaction volume of the atomic beam and the laser field is limited by the short decay length of the evanescent wave, only a relatively small number of atoms can be reflected with a single laser pulse. Furthermore, the reflection is always inelastic, since the force exerted on the atoms varies as a function of the initial position of the particles. To solve the above problem we consider the use of a standing wave as a pulsed mirror for atoms. Our numerical simulations show that with a proper choice of the pulse duration and field intensity, each period of the standing-wave pattern functions as an elastic mirror for particles with an initial kinetic energy below the depth of the standing-wave potential. Hence, the standing-wave pattern acts as a long row of independent atom mirrors, which provides a novel route to controlling large volumes of fast atoms even with a single laser pulse. As a second application for the pulsed standing-wave mirror we consider the reflection of slow molecules, for which no efficient mirror configuration previously has been available. It is shown that pulsed standing waves of nonresonant frequencies can be used to efficiently manipulate large volumes of rotationally cold molecules. With a suitable choice of the parameter values, the molecules can be reflected nearly elastically, or with a tailored momentum distribution. This opens up a possibility to use the pulsed standing-wave mirror to control the motion of particles in various applications of atomic and molecular physics. Such a mirror could be applied, for example, to steer and image molecular beams, separate molecular species, and to form pulsed molecular beams.
Summary form only given. The study of quantum systems that are chaotic in their classical limit has been the subject of intense research in recent years. Atom optics is an ideal experimental testing ground for this field given the combination of well-defined initial conditions, controlled nonlinear potentials, and absence of dissipative processes. To study nonlinear effects in the simplest setting, we measure momentum transferred from a single pulse of a standing wave of light to a sample of ultracold Na atoms, and observe a sharp increase in the momentum transfer when the pulse duration exceeds a critical value.
Abstract Coherent manipulation of atoms with atom-optic light pulses is central to atom interferometry. Achieving high pulse efficiency is essential for enhancing fringe contrast and sensitivity, in particular for large-momentum transfer interferometers which use an increased number of pulses. We perform an investigation of optimizing the frequency domain of pulses by using tailored polychromatic light fields, and demonstrate the possibility to deliver high-efficiency and resilient atom-optic pulses even in the situation of inhomogeneous atomic clouds and laser beams. We find that this approach is able to operate over long interrogation times despite spontaneous emission and to achieve experimentally relevant pulse efficiencies for clouds up to 100μK 100 μ K . This overcomes some of the most stringent barriers for large-momentum transfer and has the potential to reduce the complexity of atom interferometers. We show that polychromatic light pulses could enhance single-photon-based large-momentum transfer atom interferometry—achieving 850ℏk 850 ħ k of momentum splitting with experimentally accessible parameters, which represents a significant improvement over the state-of-the art. The benefits of the method extend beyond atom interferometry and could enable groundbreaking advances in quantum state manipulation.
This thesis is devoted to the study of some theoretical aspects of the problem of Quantum Accelerator Modes (QAMs), which has received considerable interest in recent years both by experimentalists and theorists in the fields of Quantum Chaos, Quantum Optics and cold-ultracold atomic physics.\nQAMs, recently observed in cold atom optics, are formed by exposing cold alkali atoms to periodic kicks in the direction of the gravitational field. The kicks are generated by a pulsed standing wave of light. A QAM is characterized by a momentum transfer, which increases linearly with the number of pulses, to a substantial fraction of the atoms. QAMs arise for values of the pulse period close to a integer multiple of half of a characteristic time TB (the Talbot time), typical of the kind of atoms used.\nA detailed theoretical explanation of this quantum effect is presented. The system can be modelled by a variant of the well-known quantum Kicked Rotator, in which the effects of a static force, produced by the earth gravitational field, are taken into account. A pseudo-classical theory has been formulated, in which the role of Planck constant is played by the detuning of the kicking period from the resonant value: in the asymptotic limit for a vanishing detuning, QAMs are described by the stable periodic orbit of a “formally” classical map on the 2-torus. An analysis of parametric dependence of the map is performed perturbatively; the parameter regions where the motion is stable and periodic exhibit Arnol’d tongues-like structures. The ordering of Arnol’d tongues and hence the classification of experimentally observed accelerator modes is provided by a number-theoretic construction known as the Farey Tree.\nQuantum decay of the modes from classical stable islands immersed in a chaotic sea is analysed and its relations to the famous Wannier-Stark problem are investigated. Theoretical estimates for the lifetimes of the metastable states as a function of the effective Planck constant are obtained.\nQAM dynamics in a Bose-Einstein condensate is then considered. Modifications on transport phenomena, imposed by nonlinearities of Gross-Pitaevskii type, which describe the atomic interactions in a mean-field approach, are examined by computer-assisted analysis.\nFinally, the problem of QAMs in the vicinity of a generic quantum resonance, namely for kicking period sufficiently close to any rational multiple of the Talbot time, is studied.\nThe theoretical framework is nontrivially generalized in terms of spinor dynamics: an ansatz of the Born-Oppenheimer type allows to decouple the dynamics of spinor and orbital degrees of freedom and a description of the orbital motion by means of “formally” classical equations is achieved. New rich families of experimental observable QAMs are predicted.
A near-resonant standing laser light field is used to focus a diverging beam of sodium atoms onto the atomic-beam axis. The investigations presented here distinguish between channeling of atoms with trajectories close to the axis and imaging of the atomic source. For laser detunings close to resonance, acceleration of the atoms in the transverse direction occurs. The amount of acceleration changes as either the intensity or the detuning of the standing wave is varied, thereby altering the position at which the atoms are imaged. This results in a variable focal-length lens for atoms. The experimental results are in good agreement with a theoretical model based on a continued-fraction solution for the standing-wave light forces.