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Physical Review A

Theory of the nondegenerate two-photon micromaser

Paulo A. Maia Neto, L. Davidovich, J. M. Raimond

Published May 1, 1991• 49 citations
Publisher

Abstract

We present the theory of a microscopic maser operating on a nondegenerate two-photon transition between two states of same parity. We start from a three-level Hamiltonian, and discuss both the one-photon resonant cascade and the two-photon regime, when the intermediate state is far off resonance. In the semiclassical limit, we derive rate equations for the field intensities and get the corresponding steady-state values. The vacuum is stable in the two-photon regime but becomes unstable for zero detuning (a clear signature of a one-photon process). Solutions displaying true two-photon operation (intermediate state unpopulated) even with zero detuning are displayed. Using the full quantum density-matrix approach, we derive a master equation for the field and discuss both operating regimes, showing that the spontaneous emission may turn the vacuum unstable in the two-photon case. In the off-resonance two-photon regime, there is a strong correlation between the fluctuations of the intensities of the two modes. We find a squeezing factor of 50% for the fluctuations in the difference of intensities.

DOI
10.1103/physreva.43.5073

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We present the theory of a microscopic maser operating on a nondegenerate two-photon transition between two states of same parity. We start from a three-level Hamiltonian, and discuss both the one-photon resonant cascade and the two-photon regime, when the intermediate state is far off resonance. In the semiclassical limit, we derive rate equations for the field intensities and get the corresponding steady-state values. The vacuum is stable in the two-photon regime but becomes unstable for zero detuning (a clear signature of a one-photon process). Solutions displaying true two-photon operation (intermediate state unpopulated) even with zero detuning are displayed. Using the full quantum density-matrix approach, we derive a master equation for the field and discuss both operating regimes, showing that the spontaneous emission may turn the vacuum unstable in the two-photon case. In the off-resonance two-photon regime, there is a strong correlation between the fluctuations of the intensities of the two modes. We find a squeezing factor of 50% for the fluctuations in the difference of intensities.
We present the quantum theory of a microscopic maser operating on a degenerate two-photon transition between levels of the same parity. We derive both a master equation and a Fokker-Planck equation for this system, and show that quantum effects may have a substantial influence on the behavior of the maser. They modify the oscillation threshold and make external triggering of this maser unnecessary, whereas, according to semiclassical theory, such a triggering is required to start up the maser oscillation. We derive the phase-diffusion properties of the field and show that the diffusion coefficient is complex in this case, its imaginary part being associated with a frequency shift of the field inside the cavity. We show that, in steady state, the photon-number statistics is sub-Poissonian for a wide range of pumping rates.
We present the theory of a micromaser operating on a cascade three-level atomic transition, which is coupled to two cavity modes satisfying the resonance condition. A numerical approach is employed to integrate the master equation describing the microwave field, allowing us to obtain the semiclassical regime in the limit of large mean photon numbers. We show that the transfer rate from the excited atomic state is very close to 100% over a large interval of variation of the interaction time. The atom - field interaction time may be chosen so as to avoid transitions to the intermediate atomic state when in steady-state operation. In this case, the two cavity modes have nearly the same photon statistics, and the fluctuations in the difference of intensities may be reduced by up to 50% below the classical limit. The intensity correlation between the two cavity modes originates from the possibility of controlling the interaction time, rather than from the simultaneous generation of `twin' photons in a two-photon transition.
The authors develop the theory of the degenerate and nondegenerate two-photon micromaser using the full, three-level Hamiltonian under conditions of overall two-photon resonance. Subject to this condition, their results are valid for arbitrary one-photon detunings, but they consider in particular the large detuning and zero detuning limits, where some simplification is possible. For the case of zero detuning, they obtain semianalytic solutions, and find that, depending upon the interaction time, the system lases as either a single-mode or a two-mode system. They have compared their results with the degenerate two-photon micromaser, and find qualitative differences. Their results are valid for arbitrary one-photon detunings, provided the interaction times are not too long. The solution to the Fokker-Planck equation is found using a detailed balance, linearization procedure, and the photon statistics is investigated. Markedly sub-Poissonian behaviour is possible under certain conditions. They find that the behaviour in the zero detuning, nondegenerate situation is quite distinct to that of all other cases.
We derive the equation of motion for the field density matrix of the degenerate two-photon laser under conditions of two-photon resonance starting from the full microscopic Hamiltonian. Our results are compared with the corresponding quantities obtained from the standard effective Hamiltonian. As we have shown for the nondegenerate case, the full diagonal density-matrix equations tend to the effective Hamiltonian density-matrix equations in an appropriate limit, but the equations of motion for the off-diagonal elements do not coincide. The equations obtained using a more accurate form of the effective Hamiltonian, in which Stark shifts are included, do agree. In this paper we concentrate on the photon-number distribution and the nature of the phase transition that takes place in the neighborhood of the two-photon lasing transition threshold. We determine the steady-state mean photon numbers and consider the stability of the solutions. A solution is found where the mean photon number is zero, but this is found to be a stable solution only for sufficiently weak pumping, whereas in the standard effective Hamiltonian approach it is always stable. As the pumping strength is increased, a range of detunings is reached in which there are two stable solutions. The amplitude of the zero-photon peak diminishes very rapidly as the pumping strength increases. Finally, for sufficiently large detunings, a single, stable, steady-state solution is obtained. The nature of the phase transition is illustrated by presenting plots of the photon-number distribution against detuning and pumping rate. The photon-number fluctuations about the mean are also discussed.
We formulate the theory of a micromaser operating simultaneously on a one- and a two-photon atomic transition. Departing from the complete microscopic Hamiltonian for this composite `atom plus field' system, we derive the equations governing its behaviour in the semiclassical approximation and also the fully quantum mechanical master equation. Using parameters corresponding to existing realizations of the one- and two-photon micromaser, we obtain illustrative examples of some novel aspects of this system in the steady state as well as in dynamical evolution.
A quantum theory of two-photon correlated-spontaneous-emission lasers (CEL's) is developed, starting from the exact atom-field interaction Hamiltonian for cascade three-level atoms interacting with a single-mode radiation field. We consider the situation where the active atoms are prepared initially in a coherent superposition of three atomic levels and derive a master equation for the field-density operator by using a quantum theory for coherently pumped lasers. The master equation is transformed into a Fokker-Planck equation for the antinormal-ordering Q function. The drift coefficients of the Fokker-Planck equation enable us to study the steady-state operation of the two-photon CEL's analytically. We have studied both resonant two-photon CEL for which there is no threshold, and off-resonant two-photon CEL for which there exists a threshold. In both cases the initial atomic coherences provide phase locking, and squeezing in the phase quadrature of the field is found. The off-resonant two-photon CEL can build up from a vacuum when its linear gain is larger than the cavity loss (even without population inversion). Maximum squeezing is found in the no-population-inversion region with the laser intensities far below saturation in both cases, which are more than 90% for the resonant two-photon CEL and nearly 50% for the off-resonant one. Approximate steady-state Q functions are obtained for the resonant two-photon CEL and, in certain circumstances, for the off-resonant one.