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Physical Review A

Quantum theory of a two-photon micromaser

L. Davidovich, J. M. Raimond, M. Brune, S. Haroche

Published Oct 1, 1987• 203 citations
Publisher

Abstract

We present the quantum theory of a microscopic maser operating on a degenerate two-photon transition between levels of the same parity. We derive both a master equation and a Fokker-Planck equation for this system, and show that quantum effects may have a substantial influence on the behavior of the maser. They modify the oscillation threshold and make external triggering of this maser unnecessary, whereas, according to semiclassical theory, such a triggering is required to start up the maser oscillation. We derive the phase-diffusion properties of the field and show that the diffusion coefficient is complex in this case, its imaginary part being associated with a frequency shift of the field inside the cavity. We show that, in steady state, the photon-number statistics is sub-Poissonian for a wide range of pumping rates.

DOI
10.1103/physreva.36.3771

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arXiv:quant-ph/0307226•Jul 30, 2003•0 citations
We present the quantum theory of a microscopic maser operating on a degenerate two-photon transition between levels of the same parity. We derive both a master equation and a Fokker-Planck equation for this system, and show that quantum effects may have a substantial influence on the behavior of the maser. They modify the oscillation threshold and make external triggering of this maser unnecessary, whereas, according to semiclassical theory, such a triggering is required to start up the maser oscillation. We derive the phase-diffusion properties of the field and show that the diffusion coefficient is complex in this case, its imaginary part being associated with a frequency shift of the field inside the cavity. We show that, in steady state, the photon-number statistics is sub-Poissonian for a wide range of pumping rates.
We present the theory of a truly microscopic maser consisting of a single-mode high-Q resonator in which a monoenergetic beam of excited two-level atoms is injected at such a low flux that at most one atom at a time is present inside the cavity. Both a microscopic theory and a heuristic Fokker-Planck approach are presented. We show that the micromaser exhibits a number of novel features that are averaged out in usual masers and lasers. First, the field is in general sub-Poissonian, which reflects the quantization of both the field and its sources. Second, the onset of maser oscillations may be followed by a succession of abrupt transitions in the state of the field. Finally, as the atomic flux through the resonator is increased, the maser threshold acquires characteristics of a continuous phase transition, whereas the subsequent changes in the field distribution become analogous to first-order phase transitions.
We present the theory of a microscopic maser operating on a nondegenerate two-photon transition between two states of same parity. We start from a three-level Hamiltonian, and discuss both the one-photon resonant cascade and the two-photon regime, when the intermediate state is far off resonance. In the semiclassical limit, we derive rate equations for the field intensities and get the corresponding steady-state values. The vacuum is stable in the two-photon regime but becomes unstable for zero detuning (a clear signature of a one-photon process). Solutions displaying true two-photon operation (intermediate state unpopulated) even with zero detuning are displayed. Using the full quantum density-matrix approach, we derive a master equation for the field and discuss both operating regimes, showing that the spontaneous emission may turn the vacuum unstable in the two-photon case. In the off-resonance two-photon regime, there is a strong correlation between the fluctuations of the intensities of the two modes. We find a squeezing factor of 50% for the fluctuations in the difference of intensities.
We discuss the quantum theory of a simple model of a maser oscillator, consisting of one radiation-field mode interacting with a large number of stationary three-level atoms. The field and the atoms also interact with separate heat reservoirs which represent dissipation mechanisms and an incoherent pumping mechanism. The model is sufficiently simple that some analytical progress can be made with the nonlinear quantal equations before further approximation is necessary. We start from the quantal equation of motion of the field-atom density operator. We make immediate use of a diagonal coherent-state expansion for the field part of the density operator and a somewhat similar expansion for the atom part. This yields an exact equation of the Fokker-Planck form for a ccc-number weight distribution, which retains all the significance of the original operator equation, and which has the semiclassical equation for the same model as a first, fluctuation-free approximation. We make use of our basic Fokker-Planck equation in a variety of ways. We discuss the reduction of the equation under conditions that the atomic decay constants are large (large atomic linewidth), arriving finally at an equation of motion for a field-only weight function which serves to demonstrate the basic coherence properties of a maser. We derive and discuss the equation of motion of the generalized Wigner density for the maser model. The generalized Wigner density is a smoothed version (a convolution) of our basic weight distribution, and from it we derive an equivalent classical model including noise sources. Finally, we discuss other useful weight distributions and the number representation for the field. The equations we derive in these discussions make contact with the rate equations of Shimoda, Takahasi, and Townes, as well as with the more recent work of Lax and Louisell, Lax, and of Scully and Lamb.
We formulate the theory of a micromaser operating simultaneously on a one- and a two-photon atomic transition. Departing from the complete microscopic Hamiltonian for this composite `atom plus field' system, we derive the equations governing its behaviour in the semiclassical approximation and also the fully quantum mechanical master equation. Using parameters corresponding to existing realizations of the one- and two-photon micromaser, we obtain illustrative examples of some novel aspects of this system in the steady state as well as in dynamical evolution.
We investigate the quantum dynamics of a two-photon micromaser pumped by atoms injected in the superposition state of the upper and intermediate levels. We simulate a master equation governing the system by the Monte Carlo wavefunction approach and analyse the steady-state behaviour as a function of the atomic transit time. The atomic coherence can effectively enhance the intensity and sub-Poissonian of the cavity field as compared with the atomic mixture. It is also discovered that the phase of the cavity field can be shifted by adjusting the detuning between the atom and field. This result shows that it is possible to manipulate the phase of the cavity field by detuning, due to atomic coherence.
We present a theory which can explain the micromaser as well as its optical counterpart, the microlaser, for appropriate values of dissipative parameters. We show that, in both the the cases, the cavity radiation fields can have sub-Poissonian photon statistics. We further analyse if it is possible to attain a Fock state of the radiation field. The microlaser is precluded for such analysics due to the damping of its lasing levels making transitions at optical frequencies. Hence, we focus our attention on the micromaser and our exact simulation of the dynamics shows that it is not possible to generate a Fock state of the cavity radiation field.