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Low Temperature Physics

To the theory of spin–charge separation in one-dimensional correlated electron systems

Andrei A. Zvyagin

Published Sep 1, 2004• 3 citations
Publisher

Abstract

Spin–charge separation is considered to be one of the key properties that distinguish low-dimensional electron systems from others. Three-dimensional correlated electron systems are described by the Fermi liquid theory. There, low-energy excitations (quasiparticles) are reminiscent of noninteracting electrons: They carry charges −e and spins 1/2. It is believed that for any one-dimensional correlated electron system, low-lying electron excitations carry either only spin and no charge, or only charge without spin. That is why recent experiments looked for such low-lying collective electron excitations, one of which carries only spin, and the other carries only charge. Here we show that despite the fact that for exactly solvable one-dimensional correlated electron models there exist excitations which carry only spin and only charge, in all these models with short-range interactions the low-energy physics is described by low-lying collective excitations, one of which carries both spin and charge.

DOI
10.1063/1.1802958

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Cambridge University Press eBooks•Mar 31, 2005•0 citations
Spin–charge separation is considered to be one of the key properties that distinguish low-dimensional electron systems from others. Three-dimensional correlated electron systems are described by the Fermi liquid theory. There, low-energy excitations (quasiparticles) are reminiscent of noninteracting electrons: They carry charges −e and spins 1/2. It is believed that for any one-dimensional correlated electron system, low-lying electron excitations carry either only spin and no charge, or only charge without spin. That is why recent experiments looked for such low-lying collective electron excitations, one of which carries only spin, and the other carries only charge. Here we show that despite the fact that for exactly solvable one-dimensional correlated electron models there exist excitations which carry only spin and only charge, in all these models with short-range interactions the low-energy physics is described by low-lying collective excitations, one of which carries both spin and charge.
Abstract. I give a brief introduction to Luttinger liquids. Luttinger liquids are paramagnetic one-dimensional metals without Landau quasi-particle excitations. The elementary excitations are collective charge and spin modes, leading to charge-spin separation. Correlation functions exhibit power-law behavior. All physical properties can be calculated, e.g. by bosonization, and depend on three parameters only: the renormalized coupling constant Kρ, and the charge and spin velocities. I also discuss the stability of Luttinger liquids with respect to temperature, interchain coupling, lattice effects and phonons, and list important open problems. WHAT IS A LUTTINGER LIQUID ANYWAY? Ordinary, three-dimensional metals are described by Fermi liquid theory. Fermi liquid theory is about the importance of electron-electron interactions in metals. It states that there is a 1:1-correspondence between the low-energy excitations of a free Fermi gas, and those of an interacting electron liquid which are termed “quasiparticles” [1]. Roughly speaking, the combination of the Pauli principle with low excitation energy (e.g. T ≪ EF) and the large phase space available in 3D, produces
The bosonization procedure works equally well for fermions with spin, thus providing us with an essentially nonperturbative approach to one-dimensional metals. The foundations of this approach were laid in the late 1970s and early 1980s by various authors (see the review article by Brazovsky and Kirova (1984) and references therein). The bosonization approach is based on the fact that coherent excitations in onedimensional interacting systems are not renormalized electrons, but collective excitations – bosons. For spinless fermions there is only one branch of collective excitations – charge density waves. For fermions with spin, another branch appears which represents spin density waves. Elementary excitations in the charge sector carry charge ± e and spin 0; excitations in the spin sector are neutral and carry spin 1/2. Since the different branches have different symmetry properties, one can expect them to have quite different spectra. This can even go to such extremes that one branch has a gap and the other does not. It is only natural under such circumstances that electrons, which carry quantum numbers from both the spin and charge sectors, cannot propagate coherently. Roughly speaking, the parts of the electron containing different degrees try to tear it in pieces; it is customary to call this phenomenon spin-charge separation . Empirically this loss of coherence is revealed as an absence of a quasi-particle pole in the single-electron Green's function, an effect whose existence is supported by experimental observations (see discussion at the end of the chapter). All phenomenona described above (the spin-charge separation and existence of excitations with fractions of quantum numbers) can be described by the model considered below.
One of the central issues in the study of high-temperature superconducting cuprates which are composed of two-dimensional (2D) CuO 2 planes is whether the 2D systems with strong electron correlation behave as a Fermi liquid or a non-Fermi-liquid-like one-dimensional (1D) system with electron correlation. In this article, we start with the detailed examination of the electronic structure in cuprates and study theoretically the spin and charge dynamics in 1D and 2D cuprates. The theoretical background of spin-charge separation in the 1D model systems including the Hubbard and t - J models is presented. The first direct observation of collective modes of spin and charge excitations in a 1D cuprate, which are called spinons and holons respectively, in angle-resolved photoemission spectroscopy (ARPES) experiments is reviewed in the light of the theoretical results based on the numerically exact-diagonalization method. The charge and spin dynamics in 1D insulating cuprates is also discussed in connection with the spin-charge separation. The arguments are extended to the 2D cuprates, and the unique aspects of the electronic properties of high-temperature superconductors are discussed. Special emphasis is placed on the d-wave-like excitations in insulating 2D cuprates observed in ARPES experiments. We explain how the excitations are caused by the spin-charge separation. The charge stripes observed in the underdoped cuprates are examined in connection with spin-charge separation in real space.
In contrast to the well-known Fermi-liquid theory of three dimensions, interacting one-dimensional and quasi-one-dimensional systems of fermions are described at low energy by an effective theory known as Luttinger liquid theory. This theory is expressed in terms of collective many-body excitations that show exotic behavior such as spin-charge separation. Luttinger liquid theory is commonly applied on the premise that ``low energy'' describes both the spin and charge sectors. However, when the interactions in the system are very strong, as they typically are at low particle densities, the ratio of spin to charge energy may become exponentially small. It is then possible at very low temperatures for the single-spin excitation energy to be low compared to the characteristic single excitation charge energy, but still high compared to the characteristic spin energy. This energy window of near ground-state charge degrees of freedom but highly thermally excited spin degrees of freedom is called a spin-incoherent Luttinger liquid. The spin-incoherent Luttinger liquid exhibits a higher degree of universality than the Luttinger liquid and its properties are qualitatively distinct. In this Colloquium some recent theoretical developments in the field are detailed and experimental indications of such a regime in gated semiconductor quantum wires are described.
The problem of spin-charge separation is addressed by considering current carrying states in a one-dimensional system of interacting electrons. Exact results for the Hubbard model and the bosonization method are exploited. We find that away from half filling both spin and charge excitations carry charge currents which are proportional to their momenta for most cases. Being in a qualitative agreement with the noninteracting ld Fermi gas picture, this result contradicts the spin-charge separation concept as it is usually derived e.g. from the bosonization approach or in a strong repulsion picture. For weak coupling the paradox is resolved by taking into account the Fermi velocity dispersion and by reexamining the structure of the current operator within the bosonization approach. For strong coupling we recover an effect of hale drag by a spinon as reflected in their momentum shifts.
Non-Fermi liquid behavior In this chapter we begin the study of electronic systems that are not Landau Fermi liquids. These systems are like totalitarian societies in which the behavior of the individual is subordinated to the needs of the organization: their low-energy excitations are collective, rather than single-particle-like. A strongly collective behavior is not at all unusual in condensed matter. For example, the low energy excitations of a crystal lattice are acoustic phonons, which are collective oscillations of the atoms about their equilibrium positions. However, such examples are usually associated with a broken symmetry (translational symmetry in this case): when it comes to homogeneous electron liquids, the familiar picture of Landau's quasiparticles is so ingrained that we tend to regard any departure from it as a surprising phenomenon. Nevertheless, departures from the normal Fermi liquid pattern can and do occur in two typical scenarios: In three- and two-dimensional systems in which the electron liquid is strongly correlated , i.e., when the order of magnitude of the coulomb interaction greatly exceeds the kinetic bandwidth, In quasi-one-dimensional systems, for any strength of the interaction. A trivial example of the first scenario is offered by the three-dimensional electron liquid at very low-density. In this case the electrons form a Wigner crystal and their collective behavior arises immediately from the loss of translational symmetry. Amuch more complex example is offered by the two-dimensional electron liquid at high magnetic field. Because the kinetic energy is effectively suppressed by the magnetic field, the structure of the groundstate and the low-lying excitations is entirely controlled by the coulomb interaction.