Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Progress of Theoretical Physics

Nonlinear Excitations in a Matter-Photon System

Sachio Takeno

Published Dec 1, 1975• 1 citation
Publisher

Abstract

A quantum theory of nonlinear excitations in a matter-photon system is developed by generalizing the conventional two-level-atom model of a matter in several directions, on the assumption that the overlapping of atomic wave functions on different atomic sites is negligible.The model matter Hamiltonian is shown to be expressible in a generalized form' of the Heisenberg model Hamiltonian with anisotropic long-range exchange interactions with spin operators replaced by quasi-Pauli operators.From approxirpate formal solutions of a set of nonlinear equations satisfied by the quasi-Pauli operators ~nd photon operators, brief discussion is given on nonlinear Frenkel excitons and nonlinear exciton-photon coupled modes.An attempt is made to formulate a theory of higher-order nonlinear physical properties of the matter-photon system by including interactions of magnetic as •well as electric dipoles of atoms with photons.A brief discussion is also given on the coherence properties. of the matter-photon system which are characterized by the simultaneo~s existence of •a photon coherent state and an atomic-polarization coherent state.*> Throughout this paper, we will often use a simplified .notation l, rather than l 1, whenever appropriate, to avoid the use of complicated symbols.Also, the complex conjugate of a quantity• A is denoted by A*.

DOI
10.1143/ptp.54.1616

Related papers

A Theory of Frenkel Excitons Using a Two-Level-Atom Model

Shôzô Takeno, Mahito Mabuchi

A formal, regorous theory of Frenkel excitons interacting with an external electromagnetic field is doveloped within the framework of a two-level-atom model in which the dipole approximation is employed in describing the atom-field (taken as a c-number) interaction. The model exciton Hamiltonian is shown to be identical in form with the Heisenberg model Hamiltonian for S=1/2 spins with anisotropic long-range exchange interactions. Instead of treating excitons as a non-ideal Bose gas, atomic polarization operators and level population defference are taken up as two fundamental quantities to describe Frenkel excitons. A pair of equations satisfied by these two quantities are derived. It is shown that Frenkel excitons are generally expressed as quantum-mechanical nonlinear polarization waves, the nonlinearity being characterized by the level population. A discussion is given on the interrelationship between such polarization waves and those derivable from the classical Drude-Lorentz model. With the aid of several approximation procedures similar to those employed in nonlinear optics, a set of equations describing nonlinear exciton-photon coupled modes are derived. Brief discussion is given on the eigenfrequencies of nonlinear Frenkel excitons and nonlinear polaritons. The existence of nonlinear exciton-photon coupled modes whose properties are different from those of polariton modes is suggested.

Progress of Theoretical Physics•Dec 1, 1973•27 citations

A2 Term, Renormalization of Matter-Photon Interaction and Coherent States in Matter-Photon Systems

Sachio Takeno, Michiyoshi Nagashima

A non-relativistic quantum theory of matter-photon interaction is formulated, within the framework of the dipole approximation, by employing a canonical transformation to diago­ nalize the A' term plus the free photon Hamiltonian. The matter-photon interaction is there­ by expressed rigorously in a renormalized A·p form. Using this form for the Dicke model of two-level atoms interacting with a single-mode radiation field, we examine a possibility of the occurrence of stationary coherent states which could arise for a photon and atomic polarization as the ground state of the system, deducing a condition for such coherent states. The condition, expressed as an inequality which imposes a stable nontrivial Bloch angle of the uniform atomic polarization, is identical with that for the occurrence of a second order phase transition, and indicates that the non-existence of a second order phase transition pointed out by Rza2ewski et al. io; in fact a consequence of the present treatment of the A'­ term renormalization. However, a fulfillment of the condition is recovered, if exchange­ type atom-atom interaction is taken into account in the matter system. We also present a method to construct an effective Hamiltonian of atom-atom interaction which is equivalent to the above Dicke model in the thermodynamic limit.

Progress of Theoretical Physics•May 1, 1977•5 citations

Coherent States and Envelope Kinklike Exciton-Photon Coupled Modes in Nonlinear Frenkel Excitons Interacting with Radiation Fields

Shôzô Takeno

Interactions of nonlinear Frenkel excitons with an intense external radiation field (rf) are studied by taking the atomic polarization, the atomic population difference and the electric field as a set of variables to study the coherence and nonlinearity properties of the exciton-rf system. To equations for these quantities, terms are added phenomenologicaly to take care of pumping and dissipative effects. Two kinds of solutions are obtained under certain conditions, one representing the existence of the stationary coherent polarization and the macroscopic number of photons with wave number equal to that of the excitons and another envelope-kink-like, steady exciton-rf coupled modes around the stationary coherent states

Journal of the Physical Society of Japan•Aug 15, 1993•3 citations

Nonlinear Excitations and Coherent States in the Ising Model in a Transverse Field

Shôzô Takeno

Nonlinear excitations in the Ising model in a transverse field or an equivalent Frenkel-exciton model for a system of two-level atoms are studied by using a method of diagonal coherent-state representation. It is shown that if the ratio of the Ising interaction to a transverse-field strength exceeds a certain critical value, stationary coherent states giving the ground state and excited states of the model Hamiltonian are characterized by two degenerate structures resulting from spatially uniform coherent states and static domain-wall type excitations, respectively. Particular solutions for the time evolution of spin operators corresponding to atomic polarization are then studied. It is shown that moving domain-wall solutions or moving solitary-wave solutions can exist under certain conditions.

Journal of the Physical Society of Japan•Apr 1, 1980•9 citations

Few- and many-body photon bound states in quantum nonlinear media: a spin-model approach

Giuseppe Calajò, Darrick E. Chang

The emergence of multi-photon bound states in quantum nonlinear media is an intriguing phenomenon that has attracted significant theoretical and experimental interest. Such bound states can emerge in quite different settings, such as arrays of quantum emitters coupled to photonic waveguides and Rydberg nonlinear media. The theoretical tools to characterize the bound states are equally diverse, ranging from Bethe ansatz to effective field theories. Here, we propose and utilize a spin-model formulation of quantum atom-light interactions as a general, unified framework to study bound states, and apply this formalism to several distinct systems. We show how to obtain the bound-state dispersion relation within the two-excitation subspace, and also numerically investigate how the properties of higher multi-photon bound states manifest themselves in the propagation of large photon number pulses and spatio-temporal correlations at the output. Interestingly, for all the specific systems studied (chiral and bi-directional waveguides, and Rydberg media), we find that the large-photon number limit always coincides with the well-known semi-classical soliton phenomenon of self-induced transparency or immediate generalizations thereof.

•Sep 30, 2021•1 citation

Photon Exchange Between a Pair of Nonidentical Atoms with Two Forms of Interactions

Shahram Mohammad-Mehdi Golshan

A pair of nonidentical two-level atoms, separated by a fixed distance R, interact through photon exchange. The system is described by a state vector which is assumed to be a superposition of four "essential states": (1) the first atom is excited, the second one is in the ground state, and no photon is present, (2) the first atom is in its ground state, the second one is excited, and no photon is present, (3) both atoms are in their ground states and a photon is present, and (4) both atoms are excited and a photon is also present. The system is initially in state (1). The probabilities of each atom being excited are calculated for both the minimally-coupled interaction and the multipolar interaction in the electric dipole approximation. For the minimally-coupled interaction Hamiltonian, the second atom has a probability of being instantaneously excited, so the interaction is not retarded. For the multipolar interaction Hamiltonian, the second atom is not excited before the retardation time, which agrees with special relativity. For the minimally-coupled interaction the nonphysical result occurs because the unperturbed Hamiltonian is not the energy operator in the Coulomb gauge. For the multipolar Hamiltonian in the electric dipole approximation the unperturbed Hamiltonian is the energy operator. An active view of unitary transformations in nonrelativistic quantum electrodynamics is used to derive transformation laws for the potentials of the electromagnetic field and the static Coulomb potential. For a specific choice of unitary transformation the transformation laws for the potentials are used in the minimally-coupled second-quantized Hamiltonian to obtain the multipolar Hamiltonian, which is expressed in terms of the quantized electric and magnetic fields.

•May 1, 1987•0 citations
A quantum theory of nonlinear excitations in a matter-photon system is developed by generalizing the conventional two-level-atom model of a matter in several directions, on the assumption that the overlapping of atomic wave functions on different atomic sites is negligible.The model matter Hamiltonian is shown to be expressible in a generalized form' of the Heisenberg model Hamiltonian with anisotropic long-range exchange interactions with spin operators replaced by quasi-Pauli operators.From approxirpate formal solutions of a set of nonlinear equations satisfied by the quasi-Pauli operators nd photon operators, brief discussion is given on nonlinear Frenkel excitons and nonlinear exciton-photon coupled modes.An attempt is made to formulate a theory of higher-order nonlinear physical properties of the matter-photon system by including interactions of magnetic as •well as electric dipoles of atoms with photons.A brief discussion is also given on the coherence properties. of the matter-photon system which are characterized by the simultaneos existence of •a photon coherent state and an atomic-polarization coherent state.> Throughout this paper, we will often use a simplified .notation l, rather than l 1, whenever appropriate, to avoid the use of complicated symbols.Also, the complex conjugate of a quantity• A is denoted by A.
A formal, regorous theory of Frenkel excitons interacting with an external electromagnetic field is doveloped within the framework of a two-level-atom model in which the dipole approximation is employed in describing the atom-field (taken as a c-number) interaction. The model exciton Hamiltonian is shown to be identical in form with the Heisenberg model Hamiltonian for S=1/2 spins with anisotropic long-range exchange interactions. Instead of treating excitons as a non-ideal Bose gas, atomic polarization operators and level population defference are taken up as two fundamental quantities to describe Frenkel excitons. A pair of equations satisfied by these two quantities are derived. It is shown that Frenkel excitons are generally expressed as quantum-mechanical nonlinear polarization waves, the nonlinearity being characterized by the level population. A discussion is given on the interrelationship between such polarization waves and those derivable from the classical Drude-Lorentz model. With the aid of several approximation procedures similar to those employed in nonlinear optics, a set of equations describing nonlinear exciton-photon coupled modes are derived. Brief discussion is given on the eigenfrequencies of nonlinear Frenkel excitons and nonlinear polaritons. The existence of nonlinear exciton-photon coupled modes whose properties are different from those of polariton modes is suggested.
A non-relativistic quantum theory of matter-photon interaction is formulated, within the framework of the dipole approximation, by employing a canonical transformation to diago­ nalize the A' term plus the free photon Hamiltonian. The matter-photon interaction is there­ by expressed rigorously in a renormalized A·p form. Using this form for the Dicke model of two-level atoms interacting with a single-mode radiation field, we examine a possibility of the occurrence of stationary coherent states which could arise for a photon and atomic polarization as the ground state of the system, deducing a condition for such coherent states. The condition, expressed as an inequality which imposes a stable nontrivial Bloch angle of the uniform atomic polarization, is identical with that for the occurrence of a second order phase transition, and indicates that the non-existence of a second order phase transition pointed out by Rza2ewski et al. io; in fact a consequence of the present treatment of the A'­ term renormalization. However, a fulfillment of the condition is recovered, if exchange­ type atom-atom interaction is taken into account in the matter system. We also present a method to construct an effective Hamiltonian of atom-atom interaction which is equivalent to the above Dicke model in the thermodynamic limit.
Interactions of nonlinear Frenkel excitons with an intense external radiation field (rf) are studied by taking the atomic polarization, the atomic population difference and the electric field as a set of variables to study the coherence and nonlinearity properties of the exciton-rf system. To equations for these quantities, terms are added phenomenologicaly to take care of pumping and dissipative effects. Two kinds of solutions are obtained under certain conditions, one representing the existence of the stationary coherent polarization and the macroscopic number of photons with wave number equal to that of the excitons and another envelope-kink-like, steady exciton-rf coupled modes around the stationary coherent states
Nonlinear excitations in the Ising model in a transverse field or an equivalent Frenkel-exciton model for a system of two-level atoms are studied by using a method of diagonal coherent-state representation. It is shown that if the ratio of the Ising interaction to a transverse-field strength exceeds a certain critical value, stationary coherent states giving the ground state and excited states of the model Hamiltonian are characterized by two degenerate structures resulting from spatially uniform coherent states and static domain-wall type excitations, respectively. Particular solutions for the time evolution of spin operators corresponding to atomic polarization are then studied. It is shown that moving domain-wall solutions or moving solitary-wave solutions can exist under certain conditions.
The emergence of multi-photon bound states in quantum nonlinear media is an intriguing phenomenon that has attracted significant theoretical and experimental interest. Such bound states can emerge in quite different settings, such as arrays of quantum emitters coupled to photonic waveguides and Rydberg nonlinear media. The theoretical tools to characterize the bound states are equally diverse, ranging from Bethe ansatz to effective field theories. Here, we propose and utilize a spin-model formulation of quantum atom-light interactions as a general, unified framework to study bound states, and apply this formalism to several distinct systems. We show how to obtain the bound-state dispersion relation within the two-excitation subspace, and also numerically investigate how the properties of higher multi-photon bound states manifest themselves in the propagation of large photon number pulses and spatio-temporal correlations at the output. Interestingly, for all the specific systems studied (chiral and bi-directional waveguides, and Rydberg media), we find that the large-photon number limit always coincides with the well-known semi-classical soliton phenomenon of self-induced transparency or immediate generalizations thereof.
A pair of nonidentical two-level atoms, separated by a fixed distance R, interact through photon exchange. The system is described by a state vector which is assumed to be a superposition of four "essential states": (1) the first atom is excited, the second one is in the ground state, and no photon is present, (2) the first atom is in its ground state, the second one is excited, and no photon is present, (3) both atoms are in their ground states and a photon is present, and (4) both atoms are excited and a photon is also present. The system is initially in state (1). The probabilities of each atom being excited are calculated for both the minimally-coupled interaction and the multipolar interaction in the electric dipole approximation. For the minimally-coupled interaction Hamiltonian, the second atom has a probability of being instantaneously excited, so the interaction is not retarded. For the multipolar interaction Hamiltonian, the second atom is not excited before the retardation time, which agrees with special relativity. For the minimally-coupled interaction the nonphysical result occurs because the unperturbed Hamiltonian is not the energy operator in the Coulomb gauge. For the multipolar Hamiltonian in the electric dipole approximation the unperturbed Hamiltonian is the energy operator. An active view of unitary transformations in nonrelativistic quantum electrodynamics is used to derive transformation laws for the potentials of the electromagnetic field and the static Coulomb potential. For a specific choice of unitary transformation the transformation laws for the potentials are used in the minimally-coupled second-quantized Hamiltonian to obtain the multipolar Hamiltonian, which is expressed in terms of the quantized electric and magnetic fields.