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Journal of the Optical Society of America B

Raman–Ramsey electromagnetically induced transparency in the configuration of counterpropagating pump and probe in vacuum Rb cell

I. S. Radojičić, Milan Radonjić, Marina M. Lekić, Z. D. Grujić, Dragan Lukić, Branislav M. Jelenkovic

Published Feb 12, 2015• 7 citations
Publisher

Abstract

Counterpropagating, spatially separated hollow pump and coaxial probe laser beams generate narrow Zeeman electromagnetically induced transparency (EIT) resonances in the vacuum Rb cell. The lasers are locked to D2 line transition Fg=2→Fe=1 of Rb87. For the probe laser beam intensity between 0.1 and 3.0 mW/cm2 this Ramsey-type configuration yields dual-structured resonances having a narrow peak on top of a broader pedestal. Linewidths of the narrow peak are nearly independent of the probe laser beam intensity and of the probe diameter (for diameters 0.8 and 2.7 mm), provided that the dark region between the pump and the probe beams is fixed. At the probe laser beam intensities below 0.1 mW/cm2 Zeeman EIT is a single narrow resonance. With this geometry of laser beams, and at low probe intensity, the presence of the pump enables the probe EIT, i.e., the probe transmission becomes enhanced in a narrow spectral window. Accompanying theoretical model showed good quantitative agreement with the measurements.

DOI
10.1364/josab.32.000426

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Journal of Physics B Atomic Molecular and Optical Physics•Aug 5, 2013•6 citations
Counterpropagating, spatially separated hollow pump and coaxial probe laser beams generate narrow Zeeman electromagnetically induced transparency (EIT) resonances in the vacuum Rb cell. The lasers are locked to D2 line transition Fg=2→Fe=1 of Rb87. For the probe laser beam intensity between 0.1 and 3.0 mW/cm2 this Ramsey-type configuration yields dual-structured resonances having a narrow peak on top of a broader pedestal. Linewidths of the narrow peak are nearly independent of the probe laser beam intensity and of the probe diameter (for diameters 0.8 and 2.7 mm), provided that the dark region between the pump and the probe beams is fixed. At the probe laser beam intensities below 0.1 mW/cm2 Zeeman EIT is a single narrow resonance. With this geometry of laser beams, and at low probe intensity, the presence of the pump enables the probe EIT, i.e., the probe transmission becomes enhanced in a narrow spectral window. Accompanying theoretical model showed good quantitative agreement with the measurements.
Experimental and theoretical investigations show the strong effect of the pump beam, spatially separated from the probe beam, on the probe's electromagnetically induced absorption (EIA) and nonlinear magneto-optical rotation (NMOR). Linearly polarized pump and probe laser beams are locked to the Fg = 2 → Fe = 3 transition of the 87Rb D2 line and pass a vacuum Rb gas cell coaxially. We show that the observed narrowing of EIA and NMOR resonances is due to the Ramsey effect. Linewidths of the resonances decrease when the size of the dark region between pump and probe lasers increases. Variation of the angle between pump and probe linear polarizations strongly influences the phases of atomic coherences generated by the pump beam and consequently the line-shapes of the probe EIA and NMOR resonances. Complete change of the resonance sign is possible if the phases of the ground state coherences, Δmg = 2, are altered by π. The central EIA fringe becomes less pronounced if the probe intensity increases, due to the larger probe contribution to atomic evolution. Ramsey-like interference is a manifestation of the evolution of ground state Zeeman coherences, required for EIA, in the dark region in the presence of a small magnetic field.
Abstract We investigate, experimentally and theoretically, time development of Zeeman electromagnetically induced transparency (EIT) during propagation of two time separated polarization laser pulses, preparatory and probe, through Rb vapour. The pulses were produced by modifying laser intensity and degree of elliptical polarization. The frequency of the single laser beam is locked to the hyperfine transition of the D 1 line in 87 Rb. Transients in the intensity of component of the transmitted light are measured or calculated at different values of the external magnetic field, during both preparatory and probe pulse. Zeeman EIT resonances at particular time instants of the pulse propagation are reconstructed by appropriate sampling of the transients. We observe how laser intensity, Ramsey sequence and the Rb cell temperature affect the time dependence of EIT line shapes, amplitudes and linewidths. We show that at early times of the probe pulse propagation, several Ramsey fringes are present in EIT resonances, while at later moments a single narrow peak prevails. Time development of EIT amplitudes are determined by the transmitted intensity of the component during the pulse propagation.
Electromagnetically induced transparency (EIT) due to Zeeman coherences in the Rb buffer gas cell is studied for different laser beam profiles, laser beam radii and intensities from 0.1 to 10 mW cm −2 . EIT line shapes can be approximated by the Lorentzian for wide Gaussian laser beam (6.5 mm in diameter) if laser intensity is weak and for a Π laser beam profile of the same diameter. Line shapes of EIT become non-Lorentzian for the Gaussian laser beam if it is narrow (1.3 mm in diameter) or if it has a higher intensity. EIT amplitudes and linewidths, for both laser beam profiles of the same diameter, have very similar behaviour regarding laser intensity and Rb cell temperature. EIT amplitudes are maximal at a certain laser beam intensity and this intensity is higher for narrower laser beams. The EIT linewidth estimated at zero laser intensity is about 50 nT or 0.7 kHz, which refers to 1.5 ms relaxation times of Zeeman coherences in 87 Rb atoms in our buffer gas cell. Blocking of the centre of the wide Gaussian laser beam in front of the photo detector yields Lorentzian profiles with a much better contrast to the linewidth ratio for EIT at higher intensities, above ∼2 mW cm −2 .
We investigate the evolution of the atomic coherence between Zeeman sublevels with $\ensuremath{\Delta}{m}_{F}=2$ in the region between pump and probe laser beams, in a Rb vapor cell using the Hanle configuration. The transmission of the probe beam, placed inside the hollow pump beam, shows the narrowing of the Hanle resonance (at external magnetic field B=0B=0B=0) by Ramsey fringes whose separation from the central peak depends on the distance between the beams. The temporal evolution of the pump induced alignment is evident from the changes of the probe transmission spectra with increasing the angle between linear polarizations of each beam. Experimental results are in agreement with the results of the model which calculates probe fluorescence by solving time-dependent optical Bloch equations, from the time when atom enters the pump beam to the time when it leaves the probe beam. The results for total excited state populations were averaged over atomic velocities distribution.
We experimentally studied the effects of laser beam diameter on electromagnetically induced transparency (EIT) due to Zeeman coherences induced by a laser resonant with the hyperfine transition Fg = 2 → Fe = 1 of 87Rb in a rubidium buffer gas cell. We use two laser beams of Gaussian intensity radial profile for laser beam diameters of 6.5 and 1.3 mm, laser intensities in the range of 0.1–35 mW cm−2 and cell temperatures between 60 and 82 °C. The results show that the amplitude of the normalized EIT resonance has a maximum at a laser intensity which depends on laser beam diameter and cell temperature. The laser intensity corresponding to the maximum EIT amplitude is higher for a smaller laser beam and higher cell temperature. The linewidth of Zeeman EIT resonance varies nearly linearly with laser intensity, almost independent of cell temperature and laser beam diameter.
Experimental and theoretical analyses show the effect of laser beam radial intensity distribution on line-shapes and line-widths of the electromagnetically induced transparency (EIT). We used Gaussian and Π (flat top) laser beam profiles, coupling the D1 transition of 87Rb atoms in the vacuum cell in the Hanle experimental configuration. We obtained non-Lorentzian EIT line-shapes for a Gaussian laser beam, while line-shapes for a Π laser beam profile are very well approximated with Lorentzian. EIT line-widths, lower for Gaussian than for Π, show nonlinear dependence on laser intensity for both laser beam profiles. EIT amplitudes have similar values and dependence on laser intensity for both laser beams, showing the maximum at around 0.8 mW cm−2. Differences between the EIT line-shapes for the two profiles are mainly due to distinct physical processes governing atomic evolution in the rim of the laser beam, as suggested from the EIT obtained from the various segments of the laser beam cross-section.