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Journal of Physics B Atomic Molecular and Optical Physics

Exponential pulse steepening in degenerate two-photon propagation

Heinz Steudel, David J. Kaup

Published Jul 4, 2012• 0 citations
Publisher

Abstract

The resonant propagation of an optical pulse in a two-photon absorber with a coherent initial excitation of the medium may lead to a pulse steepening growing exponentially in space. In addition another example is given wherein the steepening is followed by flattening. These results are new although, principally, they could be obtained from the general solution of the respective Goursat problem of an amplitude-modulated initial wave (H Steudel and D J Kaup 1996 J. Mod. Opt. 43 1851). In addition, we also give a simple theorem whereby it is demonstrated that the spatial derivative of the phase of the electric field will always be bounded. Furthermore, it is also shown that there can be certain critical points at which the atomic state, as well as the electric field, can become stationary in time and the spatial direction. © 2012 IOP Publishing Ltd.

DOI
10.1088/0953-4075/45/14/145502

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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•May 5, 1999•0 citations
The resonant propagation of an optical pulse in a two-photon absorber with a coherent initial excitation of the medium may lead to a pulse steepening growing exponentially in space. In addition another example is given wherein the steepening is followed by flattening. These results are new although, principally, they could be obtained from the general solution of the respective Goursat problem of an amplitude-modulated initial wave (H Steudel and D J Kaup 1996 J. Mod. Opt. 43 1851). In addition, we also give a simple theorem whereby it is demonstrated that the spatial derivative of the phase of the electric field will always be bounded. Furthermore, it is also shown that there can be certain critical points at which the atomic state, as well as the electric field, can become stationary in time and the spatial direction. © 2012 IOP Publishing Ltd.
Coherent propagation of an optical pulse in a medium with a second-order resonance is investigated when we include both the dynamical Stark effect and a population-dependent refraction index. We show how to obtain the general solution when the incident pulse has no phase-modulation. The amplitude-modulation of the incident pulse can be arbitrary as can be the initial state of the medium. This general solution is reduced to obtaining the solution of an ordinary differential equation and quadratures. For an initially de-excited medium, the solution reduces to that given by Poluektov et al. {I. A. Poluektov, Yu. M. Popov and V. S. Roitberg, 1975, Kvant. Elektron. (Moscow), 2, 1147 [1975, Sov. J. Quant. Electron., 5, 620]}. We give some illustrative examples of solutions for various initial profiles. It is also shown that the oscillating two-stream instability (OTSI) from plasma physics is equivalent to the Maxwell-Bloch equations for degenerate two-photon propagation. We give a solution for the OTSI which contains five arbitrary real functions.
The initial value problem for the propagation of a pulse through a resonant two-level optical medium is solved by the inverse scattering method. In general, an incident pulse decomposes not only into a special class of pulses to which the medium is transparent but also yields radiation which is absorbed by the medium. In this respect ``this problem'' has properties markedly different from other dispersive and reversible wave phenomena some of which are tractable by the inverse scattering method. Indeed, it is remarkable that in the present case the method still applies. In particular, we show that, while there are an infinite number of local conservation laws, the integrated densities, and in particular the energy, are only conserved for a very special class of initial conditions. The theoretical results obtained are in close agreement with all the qualitative features observed in the experiments on coherent pulse propagation. Finally, we also show that causality is preserved. Two new and novel features are introduced and briefly discussed. First, we show that if the homogeneous broadening effect is a function of position in the medium, the pulses may speed up and slow down accordingly, without losing their permanent identities. Second, we have found a new kind of solution mode corresponding to a proper eigenvalue of the scattering problem which is not a bound state.
An investigation is made of optical pulse propagation in a two-photon-absorbing medium in the incoherent regime. Simple analytic expressions describing the initial stage of evolution of arbitrarily shaped radiation pulses are derived in the long-wavelength approximation. The steady-state pulse shape is determined. In cases of self-modulation instability, the steady-state pulse is a harmonic wave whose period is governed by the properties of the medium and does not depend on the intensity of the propagating radiation. A qualitative investigation is made of the formation of steady-state pulses.
The three-pulse stimulated photon echo has been considered as one of the most fundamental transient four wave mixing processes1, where each of the three excitation pulses induces a single elementary interaction process between a laser field and an inhomogeneously broadened two-level system., resulting in a burst of the fourth wave, i.e., echo. Now if four or more optical pulses are applied to a medium, a number of photon echoes should be expected, in general. At low excitation intensities where the perturbation theory is applicable, however, the dominant nonlinear process is still the three-pulse stimulated echo and consequently each echo signal is generated only by three of the preceding pulses. It is rather a remarkable result that the echo intensity is unaffected by the presence of all the rest of the pulses other than its three generators. With this in mind, it is theoretically and experimentally shown that by applying a single optical pulse (#1) propagating along k1 followed by N pairs of counter-propagating pulses (#2j (k2j) and #3j− (k3j = −k2j); j=1,…N) in various directions, it is possible to obtain N photon echoes along the direction -k1 opposite to the first pulse #1. We will call this degenerate photon echoes, degenerate in. the sense that the echoes are spatially overlapping and temporally simultaneous. When N=l, this scheme is reduced to the ordinary backward photon echo2,3. The doubly degenerate case (N=2) is illustrated in Fig. 1. The j-th echo will be generated by the set of pulses (#1, #2j, #3j) and appear at t = t3j + t2j − t1 where t1, i2j and t3j are the arrival times of the pulses #1, #2j and #3j, respectively.
Quantum coherence and interference in atomic systems can lead to interesting optical phenomena such as nonabsorbing resonances, lasing without inversion, generating an ultrahigh index of refraction without absorption, propagation of light pulses without losses. In the last-named is given the title transparency. Up to now it is known some types of transparency in multi-level resonant media. One of them is electromagnetically induced transparency (EIT). The phenomenon of EIT in the propagation of laser radiation through an absorbing medium has been recently investigated and explained in terms of quantum coherence and interference for multi-level atomic system. For instance in the (Lambda) -system, if the atomic medium is prepared in a quantum superposition of states, matched pulses, i.e., a pair of optical pulses whose amplitude and phase have a well defined relation, propagate without absorption. The mechanism of coherent population trapping is responsible for EIT in a (Lambda) -system. There is another, well known mechanism for creating transparency in a two-state atom: self-induced transparency, or SIT. Here, a single pulse whose area (the integral of its Rabi frequency over time) is 2(pi) is applied to the medium. Such a pulse causes the atoms to cycle smoothly from the ground to the excited state and then back again. In principle, such a pulse can propagate over long distances. SIT can be generalized to multi-level systems and multiple quasi-monochromatic fields. Generalization of SIT in a (Lambda) -system was obtained in reference 2. In this report we present a new type of transparency (combined transparency). This type describes propagation of laser pulse through a (Lambda) -type medium where the initial atomic state is prepared in the form of spatially varying coherent superposition of low-energetic states (initial coherency gradient). The common envelope behaves as usual 2(pi) hyperbolic secant pulse, but the ratio between the components of frequencies transitions 1> yields 3> and 2> yields 3> changes due to coherent Raman scattering so (phi) equals atan(E1/E2) equals (pi) /2-Gz, where z is the coordinate, G is the constant determined by both the incident pulse parameters and the initial coherence between the atomic states. Our solution demonstrates a direct connection of EIT in adiabatic regime to the SIT effects. This type of a transparency is given the title screw-type transparency, because for the given form of incident pulse (pitch of screw) medium is transparent, if medium's the initial coherence gradient is correspondingly prepared (thread on a engine nut). Besides a transparency, this phenomenon contains a transformation of the incident pulse frequency during the process of the propagation. This property of the phenomena can be result in a complete conversion of the frequency.