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Physical Chemistry Chemical Physics

Visualisation of quantum evolution in the Stern–Gerlach and Rabi experiments

Marcel Utz, Malcolm H. Levitt, Nathan Cooper, Hendrik Ulbricht

Published Dec 19, 2014• 23 citations
Publisher

Abstract

The Stern-Gerlach experiment is a seminal experiment in quantum physics, involving the interaction between a particle with spin and an applied magnetic field gradient. A recent article [Wennerström et al., Phys. Chem. Chem. Phys., 2012, 14, 1677-1684] claimed that a full understanding of the Stern-Gerlach experiment can only be attained if transverse spin relaxation is taken into account, generated by fluctuating magnetic fields originating in the magnetic materials which generate the field gradient. This interpretation is contrary to the standard quantum description of the Stern-Gerlach experiment, which requires no dissipative effects. We present simulations of conventional quantum dynamics in the Stern-Gerlach experiment, using extended Wigner functions to describe the propagation of the quantum state in space and time. No relaxation effects are required to reproduce the qualitative experimental behaviour. We also present simulations of quantum dynamics in the Rabi experiment, in which an applied radiofrequency field induces spin transitions in the particle wave.

DOI
10.1039/c4cp05606j

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The Stern-Gerlach experiment is a seminal experiment in quantum physics, involving the interaction between a particle with spin and an applied magnetic field gradient. A recent article [Wennerström et al., Phys. Chem. Chem. Phys., 2012, 14, 1677-1684] claimed that a full understanding of the Stern-Gerlach experiment can only be attained if transverse spin relaxation is taken into account, generated by fluctuating magnetic fields originating in the magnetic materials which generate the field gradient. This interpretation is contrary to the standard quantum description of the Stern-Gerlach experiment, which requires no dissipative effects. We present simulations of conventional quantum dynamics in the Stern-Gerlach experiment, using extended Wigner functions to describe the propagation of the quantum state in space and time. No relaxation effects are required to reproduce the qualitative experimental behaviour. We also present simulations of quantum dynamics in the Rabi experiment, in which an applied radiofrequency field induces spin transitions in the particle wave.
The classical Stern-Gerlach experiment is analyzed with an emphasis on the spin dynamics. The central question asked is whether there occurs a relaxation of the spin angular momentum during the time the particle passes through the Stern-Gerlach magnet. We examine in particular the transverse relaxation, involving angular momentum exchange between the spin of the particles and the spins of the magnet. A method is presented describing relaxation effects at an individual particle level. This leads to a stochastic equation of motion for the spins. This is coupled to a classical equation of motion for the particle translation. The experimental situation is then modeled through simulations of individual trajectories using two sets of parameter choices and three different sets of initial conditions. The two main conclusions are: (A) if the coupling between the magnet and the spin is solely described by the Zeeman interaction with the average magnetic field the simulations show a clear disagreement with the experimental observation of Stern and Gerlach. (B) If one, on the other hand, also allows for a T(2) relaxation time shorter than the passage time one can obtain a practically quantitative agreement with the experimental observations. These conclusions are at variance with the standard textbook explanation of the Stern-Gerlach experiment.
The Stern-Gerlach experiment is the fundamental experiment in order to exhibit the quantization of spin and understand the measurement problem in quantum mechanics. However, although the Stern-Gerlach experiment plays an essential role in the teaching of quantum mechanics, no complete analysis of this experiment using Pauli spinors is presented in the pedagogical literature. This paper presents such an analysis and develops implications for the theory of quantum measurement. We first propose an analytic expression of both the wave function and the probability density in the Stern-Gerlach experiment. Our explicit solution is obtained via a complete integration of the Pauli equation over time and space. The probability density evolution describes a slipping of the wave packet into two separate packets due to the measurement device, but it cannot account for impacts. We therefore calculate the de Broglie-Bohm trajectories, which not only explain impacts naturally, but also accounts for the spin quantization following the magnetic field gradient. It is then possible to propose a clear explanation of measurement effects in the Stern-Gerlach experiment.
A detailed analysis of the classic Stern–Gerlach experiment is presented. An analytical simple solution is presented for the quantum description of the translational and spin dynamics of a silver atom in a magnetic field with a gradient along a single z-direction. This description is then used to obtain an approximate quantum description of the more realistic case with a magnetic field gradient also in a second y-direction. An explicit relation is derived for how an initial off center deviation in the y-direction affects the final result observed at the detector. This shows that the “mouth shape” pattern at the detector observed in the original Stern–Gerlach experiment is a generic consequence of the gradient in the y-direction. This is followed by a discussion of the spin dynamics during the entry of the silver atom into the magnet. An analytical relation is derived for a simplified case of a field only along the z-direction. A central question for the conceptual understanding of the Stern–Gerlach experiment has been how an initially unpolarized spin ends up in a polarized state at the detector. It is argued that this can be understood with the use of the adiabatic approximation. When the atoms first experience the magnetic field outside the magnet, there is in general a change in the spin state, which transforms from a degenerate eigenstate in the absence of a field into one of two possible non-degenerate states in the field. If the direction of the field changes during the passage through the device, there is a corresponding adiabatic change of the spin state. It is shown that an application of the adiabatic approximation in this way is consistent with the previously derived exact relations.
Originally conceived as a thought experiment, an apparatus consisting of two Stern–Gerlach apparatuses joined in an inverted manner touched on the fundamental question of the reversibility of evolution in quantum mechanics. Theoretical analysis showed that uniting the two partial beams requires an extreme level of experimental control, making the proposal in its original form unrealizable in practice. In this work, we revisit the above question in a numerical study concerning the possibility of partial-beam recombination in a spin-coherent manner. Using the Suzuki–Trotter numerical method of wave propagation and a configurable, approximation-free magnetic field, a simulation of a transversal Stern–Gerlach interferometer under ideal conditions is performed. The result confirms what has long been hinted at by theoretical analyses: the transversal Stern–Gerlach interferometer quantum dynamics is fundamentally irreversible even when perfect control of the associated magnetic fields and beams is assumed.
Abstract The Stern–Gerlach experiment reveals the quantum mechanical nature of spin through the force experienced by a non-relativistic neutral atom in a static magnetic field gradient. A key open question concerns when, along the atom’s trajectory, the spin state collapses into an eigenstate and by what mechanism. We analyze the influence of quantum electrodynamic (QED) vacuum fluctuations on spin dynamics and show that they induce spin self-interactions, leading to decoherence and memory effects. However, the magnitude of these effects is shown to be too small to account for the deterministic collapse of the spin wavefunction.