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Physical Chemistry Chemical Physics

The Stern–Gerlach experiment and the effects of spin relaxation

Håkan Wennerström, Per-Olof Westlund

Published Dec 23, 2011• 20 citations
Publisher

Abstract

The classical Stern-Gerlach experiment is analyzed with an emphasis on the spin dynamics. The central question asked is whether there occurs a relaxation of the spin angular momentum during the time the particle passes through the Stern-Gerlach magnet. We examine in particular the transverse relaxation, involving angular momentum exchange between the spin of the particles and the spins of the magnet. A method is presented describing relaxation effects at an individual particle level. This leads to a stochastic equation of motion for the spins. This is coupled to a classical equation of motion for the particle translation. The experimental situation is then modeled through simulations of individual trajectories using two sets of parameter choices and three different sets of initial conditions. The two main conclusions are: (A) if the coupling between the magnet and the spin is solely described by the Zeeman interaction with the average magnetic field the simulations show a clear disagreement with the experimental observation of Stern and Gerlach. (B) If one, on the other hand, also allows for a T(2) relaxation time shorter than the passage time one can obtain a practically quantitative agreement with the experimental observations. These conclusions are at variance with the standard textbook explanation of the Stern-Gerlach experiment.

DOI
10.1039/c2cp22173j

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Physical review. B, Condensed matter•May 1, 1998•1 citation
The classical Stern-Gerlach experiment is analyzed with an emphasis on the spin dynamics. The central question asked is whether there occurs a relaxation of the spin angular momentum during the time the particle passes through the Stern-Gerlach magnet. We examine in particular the transverse relaxation, involving angular momentum exchange between the spin of the particles and the spins of the magnet. A method is presented describing relaxation effects at an individual particle level. This leads to a stochastic equation of motion for the spins. This is coupled to a classical equation of motion for the particle translation. The experimental situation is then modeled through simulations of individual trajectories using two sets of parameter choices and three different sets of initial conditions. The two main conclusions are: (A) if the coupling between the magnet and the spin is solely described by the Zeeman interaction with the average magnetic field the simulations show a clear disagreement with the experimental observation of Stern and Gerlach. (B) If one, on the other hand, also allows for a T(2) relaxation time shorter than the passage time one can obtain a practically quantitative agreement with the experimental observations. These conclusions are at variance with the standard textbook explanation of the Stern-Gerlach experiment.
The Stern-Gerlach experiment is a seminal experiment in quantum physics, involving the interaction between a particle with spin and an applied magnetic field gradient. A recent article [Wennerström et al., Phys. Chem. Chem. Phys., 2012, 14, 1677-1684] claimed that a full understanding of the Stern-Gerlach experiment can only be attained if transverse spin relaxation is taken into account, generated by fluctuating magnetic fields originating in the magnetic materials which generate the field gradient. This interpretation is contrary to the standard quantum description of the Stern-Gerlach experiment, which requires no dissipative effects. We present simulations of conventional quantum dynamics in the Stern-Gerlach experiment, using extended Wigner functions to describe the propagation of the quantum state in space and time. No relaxation effects are required to reproduce the qualitative experimental behaviour. We also present simulations of quantum dynamics in the Rabi experiment, in which an applied radiofrequency field induces spin transitions in the particle wave.
We analyze a coincidence Stern-Gerlach measurement often discussed in connection with the derivation and illustration of Bell's theorem. The treatment is based on our recent analysis of the original Stern-Gerlach experiment (PCCP, 14, 1677‐1684 (2012)), where it is concluded that it is necessary to include a spin relaxation process to account for the experimental observations. We consider two limiting cases of a coincidence measurement using both an analytical and a numerical description. In on limit relaxation effects are neglected. In this case the correlation between the two spins present in the initial state is conserved during the passage through the magnets. However, at exit the z coordinate along the magnetic field gradient is randomly distributed between the two extreme values. In the other limit T2 relaxation is assumed to be fast relative to the time of flight through the magnet. In this case the z coordinate takes one of two possible values as observed in the original Stern‐Gerlach experiment. Due to the presence of a relaxation process involving transfer of angular momentum between particle and magnet the initially entangled spin state changes character leading to a loss of correlation between the two spins. In the original derivations of Bell's theorem based on a coincidence Stern‐Gerlach setup one assumes both a perfect correlation between the spins and only two possible values for the z‐coordinate on exit. According to the present calculations one can satisfy either of these conditions but not both simultaneously.
The century-old Stern–Gerlach setup is paradigmatic for a quantum measurement. We visualize the electron trajectories following the Bohmian zig-zag dynamics. This dynamics was developed in order to deal with the fundamentally massless nature of particles (with mass emerging from the Brout–Englert–Higgs mechanism). The corresponding trajectories exhibit a stochastic zig-zagging, as the result of the coupling between left- and right-handed chiral Weyl states. This zig-zagging persists in the non-relativistic limit, which will be considered here, and which is described by the Pauli equation for a non-uniform external magnetic field. Our results clarify the different meanings of ‘spin’ as a property of the wave function and as a random variable in the Stern–Gerlach setup, and they illustrate the notion of effective collapse. We also examine the case of an EPR-pair. By letting one of the entangled particles pass through a Stern–Gerlach device, the non-local influence (action-at-a-distance) on the other particle is manifest in its trajectory, e.g. by initiating its zig-zagging.
A thorough motion investigation and analysis was conducted again for the original Stern-Gerlach Experiment(SGE). The analysis is still based on the assumption that the atom passing the SG apparatus is a micromagnet due to the spin of its electron, the atoms in the source beam are with an orientation distribution of its angular momentum vectors, while the spin micromagnet is in the precession induced by an inhomogeneous magnetic field. It is the precession that keeps the silver beam with narrower orientation distribution of its angular momentum vectors after passing through the inhomogeneous magnetic field. The motion relativity was introduced in the SGE between the SG apparatus and the silver source beam, which interpreted all the detection phenomena in the multi-stage SGE. The research provided a new and convincing interpretation to the SGE with full satisfaction based on the classical physics without any mysterious or counter intuitive concepts introduced compared to quantum physics.
A detailed analysis of the classic Stern–Gerlach experiment is presented. An analytical simple solution is presented for the quantum description of the translational and spin dynamics of a silver atom in a magnetic field with a gradient along a single z-direction. This description is then used to obtain an approximate quantum description of the more realistic case with a magnetic field gradient also in a second y-direction. An explicit relation is derived for how an initial off center deviation in the y-direction affects the final result observed at the detector. This shows that the “mouth shape” pattern at the detector observed in the original Stern–Gerlach experiment is a generic consequence of the gradient in the y-direction. This is followed by a discussion of the spin dynamics during the entry of the silver atom into the magnet. An analytical relation is derived for a simplified case of a field only along the z-direction. A central question for the conceptual understanding of the Stern–Gerlach experiment has been how an initially unpolarized spin ends up in a polarized state at the detector. It is argued that this can be understood with the use of the adiabatic approximation. When the atoms first experience the magnetic field outside the magnet, there is in general a change in the spin state, which transforms from a degenerate eigenstate in the absence of a field into one of two possible non-degenerate states in the field. If the direction of the field changes during the passage through the device, there is a corresponding adiabatic change of the spin state. It is shown that an application of the adiabatic approximation in this way is consistent with the previously derived exact relations.
We use a stochastic theory approach to discuss different scenarios such as ``locked moment'' and ``superparamagnetic'' behavior of magnetic clusters seen in Stern-Gerlach (SG) experiments. A dimensionless parameter $\ensuremath{\lambda}{\ensuremath{\tau}}_{E}$ (where \ensuremath{\lambda} is an internal spin relaxation rate and ${\ensuremath{\tau}}_{E}$ is the time spent by the cluster in the field gradient region) and the initial polarization of the cluster moment are shown to determine sensitively the position of the cluster beam on the SG screen.