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Journal of Experimental and Theoretical Physics Letters

Dark solitons in the condensate of exciton polaritons in semiconductor microcavities under nonresonant optical excitation

A. A. Demenev, Sergei S. Gavrilov, Andrey S. Brichkin, A. V. Larionov, V. D. Kulakovskiĭ

Published Dec 1, 2014• 3 citations
Publisher

Abstract

The first-order spatial correlation function g (1)(r 12) and the polariton density distribution in the condensate of quasi-two-dimensional exciton polaritons formed in a high-Q semiconductor microcavity pillar under nonresonant optical pumping are investigated. It is found that the correlation function in certain regions of the micropillar decreases abruptly with increasing condensate density. It is shown that this behavior of the correlation function is caused by the formation of a localized dark soliton in these regions. A deep minimum of the polariton density and a shift in the phase of the condensate wavefunction by π occur within the soliton localization area.

DOI
10.1134/s002136401420003x

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We show experimentally optical bistability and the existence of bright and dark resonator solitons in the strong coupling regime between quantum-well excitons and the optical field in a semiconductor microcavity. The strong coupling results in a quasi-particle exciton-polariton, which gives access to positive and negative reactive and dissipative optical nonlinearities, as opposed to the usual room temperature semiconductor nonlinearities possessing essentially only one sign. The existence range and the properties of solitons can be varied widely by the detuning between polariton states and light frequency.
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A bosonic condensate of exciton polaritons in a semiconductor microcavity is a macroscopic quantum state subject to pumping and decay. The fundamental nature of this driven-dissipative condensate is still under debate. Here, we gain an insight into spontaneous condensation by imaging long-lifetime exciton polaritons in a high-quality inorganic microcavity in a single-shot optical excitation regime, without averaging over multiple condensate realisations. We demonstrate that condensation is strongly influenced by an incoherent reservoir and that the reservoir depletion, the so-called spatial hole burning, is critical for the transition to the ground state. Condensates of photon-like polaritons exhibit strong shot-to-shot fluctuations and density filamentation due to the effective self-focusing associated with the reservoir depletion. In contrast, condensates of exciton-like polaritons display smoother spatial density distributions and are second-order coherent. Our observations show that the single-shot measurements offer a unique opportunity to study fundamental properties of non-equilibrium condensation in the presence of a reservoir.
A transient spectroscopy technique for studying near-condensate modes of exciton polaritons in high-quality-factor planar semiconductor microcavities is proposed. It is demonstrated that, under the conditions of coherent external pumping, the transition to the upper steady state of an optically bistable condensate is accompanied by the excitation of near-condensate modes. They manifest themselves in the appearance of transient oscillations of the polariton intensity as the system switches to the upper branch of the S-shaped bistable pump dependence of the intensity. Analysis of the time-resolved spectra of these oscillations provides information on interactions in the system and the evolution of the exciton-polariton condensate density.
Dynamics of stimulated scattering of quasi-two-dimensional exciton polaritons in a semiconductor microcavity is considered theoretically. A system possessing a bistable response to coherent excitation is studied. Being a system of weakly interacting Bose particles under strongly nonequilibrium conditions, it exhibits a complex dynamics of the development of condensate modes. It is shown that multimode instability can arise in a threshold way in the system under a smooth increase in pump intensity. In this case, rapid populating of a multitude of unstable modes leads to stochastization of scattering, and evolution to a quasi-steady macrostate is performed as self-organization in an open nonequilibrium system. Arising fluctuations lead to the occurrence of a spatial nonuniformity of the distribution of scattered states.