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Physical Review Letters

Nonlinear atom optics

Georg Lenz, Pierre Meystre, Ewan M. Wright

Published Nov 15, 1993• 166 citations
Publisher

Abstract

We study an ensemble of N bosonic atoms coupled by dipole-dipole interaction and also interacting with an electromagnetic field. Effective single-atom nonlinear Schr\"odinger equations are derived. The implications of these equations are discussed in the context of some standard atom optics geometries, illustrating in particular how many-body effects modify the Pendell\"osung of Bragg scattering. In another regime, the problem is reduced to a classical massive Thirring model, with the possibility of generating atomic Thirring solitons.

DOI
10.1103/physrevlett.71.3271

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We study an ensemble of N bosonic atoms coupled by dipole-dipole interaction and also interacting with an electromagnetic field. Effective single-atom nonlinear Schr"odinger equations are derived. The implications of these equations are discussed in the context of some standard atom optics geometries, illustrating in particular how many-body effects modify the Pendell"osung of Bragg scattering. In another regime, the problem is reduced to a classical massive Thirring model, with the possibility of generating atomic Thirring solitons.
We present a many-body theory of nonlinear atom optics, and discuss some of its physical implications in the coherent regime. Considering a system of N identical two-level atoms interacting with classical and quantum-mechanical electromagnetic fields, we derive a Fock-space many-particle master equation. Introducting a Bogoliubov-Born-Green-Kirkwood-Yvon hierarchy and a Hartree-Fock factorization to truncate this hierarchy, we obtain an effective nonlinear single-particle master equation that forms the basis of nonlinear atom optics. In the second part of the paper, we concentrate on the coherent part of that master equation, and derive an effective single-atom nonlinear Schr\"odinger equation. This equation leads to the prediction of a number of effects, and, in particular, several kinds of atomic solitons. We discuss and numerically study two such kinds of solitons, Thirring solitons and gap solitons. Finally, the axial containment of an atomic gap soliton is illustrated.
In contrast to electromagnetic fields, matter-wave fields are intrinsically interacting due to the presence of atom-atom collisions. Hence, matter-wave optics becomes effectively nonlinear as soon as the atomic densities are high enough that collisions can no longer be ignored. The goal of this dissertation is to study selected aspects of atom optics under such conditions. Specifically, Chapter 2 studies the near-resonant dipole-dipole interaction between two atoms in tailored vacua. In contrast to spontaneous emission, whose rate is known to be influenced by the type of vacuum the atom interacts with, we find that the dipole-dipole potential is determined only by the free space vacuum and is not modified either by thermal or squeezed vacua. In addition in the far off-resonance regime we find that the squeezed vacuum results in an additional contribution to the effective potential governing the evolution of the atomic ground state. In the second part of the dissertation, which comprises Chapter 3, we then study several aspects of the many-body theory of atomic ultracold systems in situations where the nonlinearity arises due to the two-body dipole-dipole interaction. After a formal theoretical development we discuss the possibility of using atomic phase conjugation off Bose condensates as a diagnostic tool to access the spatial coherence properties and to measure the lifetime of the condensate. We argue that phase conjugation provides an attractive alternative to the optical methods of probing condensate proposed in the past. We further study the elementary excitations in a multicomponent Bose condensates and determine the quasi-particle frequency spectrum. We show that in that case interferences resulting from cross-coupling between the condensate components can lead to a reversal of the sign of the effective two-body interaction and to the onset of spatial instabilities.
A vector quantum field theory is developed to describe the interaction of an ultracold atomic ensemble with a laser field. The ultracold atomic ensemble is composed of either bosonic atoms or fermionic atoms. The photon exchanges between different ultracold atoms result in a long-range interatom interaction. Under appropriate conditions, such a many-body interaction leads to an effective ``Kerr-type'' nonlinearity of atomic waves. In terms of the nonlinearity, we construct a general formalism of nonlinear atom optics for an ultracold atomic beam. Applying the formalism to the diffraction of an ultracold atomic beam composed of bosonic atoms by a standing-wave laser field, we find that the many-body nonlinearity induces self-phase and cross-phase modulation of diffracted atomic waves. As a result, a standing-wave laser acts as a nonlinear atomic grating which diffracts atoms in the same way as a nonlinear periodic medium diffracts photons.
The interaction of copropagating electromagnetic and matter waves is described with a set of coupled higher-order nonlinear Schr\"odinger equations. Optical self-focusing modulates an initially planar wave leading to the generation of dipole forces on the atoms. Atomic channeling due to the dipole forces leads, in the nonlinear regime, to filamentation of the atomic beam. Instability growth rates are calculated for atomic beams with both low and high phase space densities. In one transverse dimension an exact solution is found that describes a coupled optical and atomic soliton.
We review recent developments in quantum and classical soliton theory, leading to the possibility of observing both classical and quantum parametric solitons in higher-dimensional environments. In particular, we consider the theory of three bosonic fields interacting via both parametric (cubic) and quartic couplings. In the case of photonic fields in a nonlinear optical medium this corresponds to the process of sum frequency generation (via (2) nonlinearity) modified by the (3) nonlinearity. Potential applications include an ultrafast photonic AND-gate. The simplest quantum solitons or energy eigenstates (bound-state solutions) of the interacting field Hamiltonian are obtained exactly in three space dimensions. They have a point-like structure - even though the corresponding classical theory is nonsingular. We show that the solutions can be regularized with the imposition of a momentum cut-off on the nonlinear couplings. The case of three-dimensional matter-wave solitons in coupled atomic/molecular Bose-Einstein condensates is discussed.
At the most fundamental level of quantum electrodynamics, there is no such thing as two-body interactions between atoms. The potentials that describe these interactions are effective potentials resulting from a series of approximations whose validity depends on the precise situation at hand. Considering a one-dimensional geometry for simplicity, we discuss under which conditions the familiar form of the near-resonant dipole-dipole interaction is valid, paying particular attention to the effects of interatomic propagation of light, and to what extent it can be modified in the tailored electromagnetic environments provided by optical resonators. We find that once the atoms have established that they are inside a resonator, the dipole-dipole potential may or may not remain a useful concept, depending upon the strength of the atom-field interaction. In the weak-coupling regime, one finds a two-body dipole-dipole interaction that can be enhanced or inhibited by varying the atom-field detuning. In the strong-coupling regime, by contrast, the two-body dipole-dipole potential ceases to be meaningful.