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Nonlinear atom optics

Elena V. Goldstein

Published Jan 1, 1996• 0 citations
OpenAlex

Abstract

In contrast to electromagnetic fields, matter-wave fields are intrinsically interacting due to the presence of atom-atom collisions. Hence, matter-wave optics becomes effectively nonlinear as soon as the atomic densities are high enough that collisions can no longer be ignored. The goal of this dissertation is to study selected aspects of atom optics under such conditions. Specifically, Chapter 2 studies the near-resonant dipole-dipole interaction between two atoms in tailored vacua. In contrast to spontaneous emission, whose rate is known to be influenced by the type of vacuum the atom interacts with, we find that the dipole-dipole potential is determined only by the free space vacuum and is not modified either by thermal or squeezed vacua. In addition in the far off-resonance regime we find that the squeezed vacuum results in an additional contribution to the effective potential governing the evolution of the atomic ground state. In the second part of the dissertation, which comprises Chapter 3, we then study several aspects of the many-body theory of atomic ultracold systems in situations where the nonlinearity arises due to the two-body dipole-dipole interaction. After a formal theoretical development we discuss the possibility of using atomic phase conjugation off Bose condensates as a diagnostic tool to access the spatial coherence properties and to measure the lifetime of the condensate. We argue that phase conjugation provides an attractive alternative to the optical methods of probing condensate proposed in the past. We further study the elementary excitations in a multicomponent Bose condensates and determine the quasi-particle frequency spectrum. We show that in that case interferences resulting from cross-coupling between the condensate components can lead to a reversal of the sign of the effective two-body interaction and to the onset of spatial instabilities.

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Physics of ultra cold atoms and molecules is one of the most rapidly developing areas of the modern atomic, molecular, optical physics and quantum optics.This area covers several sub-areas of diverse importance, but definitely two trends can be easily identifies: i) fundamental research on properties of ultra cold atoms and molecules, and in particular atomic and molecular condensates trapped and lattice gases; here the fundamental questions of nature and form of phase transitions in degenerate systems are being posed and studied; ii) more applications oriented research on ultracold atoms and molecules, involving in particular applications in precision measurements, atomic clocks, frequency standards, atom and molecule interferometry, quantum information, quantum engineering, "super" chemistry etc.This thesis concerns both of these major trends.The applications, or more specifically quantum engineering aspect are discussed in the first four chapters of the thesis, which deal with optical manipulations of ultra cold gases, in particular optical generation of vortices in Bose condensates, quasi-solitons in Fermi gases, and retarded dipole-dipole interactions in Bose, or Fermi gases.This thesis consists of four main chapters.Chapter 2, "Optical generation of vortices in Bose Einstein Condensates".In this chapter we study theoretically the generation of vortices by phase imprinting in trapped Bose-Einstein condensates.Phase imprinting is achieved by passing a short off-resonance laser pulse through an appropriately designed absorption plate, and impinging it on a condensate.We answer the fundamental question of how the circulation and the vortex are introduced into the system, and discuss the creation of vortex arrays.We discuss vortex dynamics and interactions in such configurations.Various methods of vortex detection based on interference combined with Bragg scattering are also analyzed.In Chapter 3, "Fermionic 'Solitons'" we investigate in detail the concept of low energy excitations of ultra cold Fermi gases.This excitations are generated using the same idea of phase imprinting as that employed in the generation of vortices in BEC.We address in this chapter some questions concerning the generation (via phase imprinting) of soliton-like solutions in a single-component Fermi gas of neutral atoms at zero and finite temperatures.By using both numerical and analytical calculations, we find the conditions under which it is possible to find in non-interacting Fermi gases, quasisolitons which resemble the properties of solitons in non-linear integrable equations.We present the results for both spatially homogeneous and trapped cases, and emphasize the importance of Fermi statistics and the absence of interactions for the existence of such solutions.In Chapter 4, "Generating Dipole Condensate" we keep studying the possibilities of optical manipulations of ultracold gases.In particular, we study two different ways to laser-induce dipole-dipole interactions in trapped Bose-Einstein condensates.The first one employs the fact that those atoms in high Rydberg states posses a large dipolar moment.We first analyze the idea of imposing the dipole moment as a time average over short stroboscopic pulses.These pulses are coherently transporting the atoms from the ground atomic state to some high Rydberg state and back.The second idea is based on the observation that in strong static or oscillatory electric fields, atoms polarize and acquire dipole moment.We analyze the possibilities and limitations of inducing such a high electric field using lasers of low frequency.In Chapter 5, "Dipolar BCS", we continue our study of trapped fermionic gases, with the analysis of the BCS transition in trapped dipolar fermionic gases.We find that the critical strength of the dipole-dipole interaction to achieve BCS pairing, depends on the trap geometry.We find the particular form of this dependence, and present the solutions for the order parameter.This first chapter is meant as a general introduction to the thesis.This introduction is by no means exhaustive, and should be rather treated as a collection of basic facts concerning ultra cold gases, without rigorous derivations.The last subsection of the introductory chapter, discusses very briefly the most important achievements and trends in the field and the current state of the art.

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At the most fundamental level of quantum electrodynamics, there is no such thing as two-body interactions between atoms. The potentials that describe these interactions are effective potentials resulting from a series of approximations whose validity depends on the precise situation at hand. Considering a one-dimensional geometry for simplicity, we discuss under which conditions the familiar form of the near-resonant dipole-dipole interaction is valid, paying particular attention to the effects of interatomic propagation of light, and to what extent it can be modified in the tailored electromagnetic environments provided by optical resonators. We find that once the atoms have established that they are inside a resonator, the dipole-dipole potential may or may not remain a useful concept, depending upon the strength of the atom-field interaction. In the weak-coupling regime, one finds a two-body dipole-dipole interaction that can be enhanced or inhibited by varying the atom-field detuning. In the strong-coupling regime, by contrast, the two-body dipole-dipole potential ceases to be meaningful.

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•Jan 1, 2010•0 citations
In contrast to electromagnetic fields, matter-wave fields are intrinsically interacting due to the presence of atom-atom collisions. Hence, matter-wave optics becomes effectively nonlinear as soon as the atomic densities are high enough that collisions can no longer be ignored. The goal of this dissertation is to study selected aspects of atom optics under such conditions. Specifically, Chapter 2 studies the near-resonant dipole-dipole interaction between two atoms in tailored vacua. In contrast to spontaneous emission, whose rate is known to be influenced by the type of vacuum the atom interacts with, we find that the dipole-dipole potential is determined only by the free space vacuum and is not modified either by thermal or squeezed vacua. In addition in the far off-resonance regime we find that the squeezed vacuum results in an additional contribution to the effective potential governing the evolution of the atomic ground state. In the second part of the dissertation, which comprises Chapter 3, we then study several aspects of the many-body theory of atomic ultracold systems in situations where the nonlinearity arises due to the two-body dipole-dipole interaction. After a formal theoretical development we discuss the possibility of using atomic phase conjugation off Bose condensates as a diagnostic tool to access the spatial coherence properties and to measure the lifetime of the condensate. We argue that phase conjugation provides an attractive alternative to the optical methods of probing condensate proposed in the past. We further study the elementary excitations in a multicomponent Bose condensates and determine the quasi-particle frequency spectrum. We show that in that case interferences resulting from cross-coupling between the condensate components can lead to a reversal of the sign of the effective two-body interaction and to the onset of spatial instabilities.
In the present thesis we study several schemes where the detection of the emitted light from an atomic ensemble gives information about the state of the atoms. In chapter 1 we review the basic theory for the light matter interaction in second quantized form. In chapter 2 we show how conservative potentials for the atoms, such as dispersive optical lattices, can be realized experimentally due to the dispersive interaction with a far detuned laser We then review some basic properties of the physics of a particle in a periodic potential. We show that the ground state and the lowest lying excitations of a Bose-Einstein condensate in a dispersive optical lattice can be described by the Bose-Hubbard Hamiltonian. In chapter 3 we study the photonic bandstructure of a chain of fixed pointlike atoms in a biperiodic configuration. We calculate the photonic spectra and the probe transmission if the atoms are in free space and inside a standing wave optical resonator. In chapter 4 we consider light scattering from ultracold atoms in an optical lattice where we calculate the photonic scattering cross section as a function of energy and direction of emission along the Mott-insulator-superfluid phase transition. We take into account the finite tunneling rate for the atoms, when evaluating the scattering cross section of the photons and the effect of photon recoil onto the atoms. In chapter 5 we consider a gas of ultracold atoms trapped at two spatially separated regions in space. Using a two Raman lasers to couple atoms out of the systems we show that it is possible to measure the mean value of the atomic field operator of the two systems by measuring the scattered light intensity of one of the Raman lasers. We show how this setup might be used to measure the temperature of a Bose-Einstein condensate and to monitor the superfluid to Mott-insulator phase transition for a gas of ultracold atoms in an optical lattice.
Physics of ultra cold atoms and molecules is one of the most rapidly developing areas of the modern atomic, molecular, optical physics and quantum optics.This area covers several sub-areas of diverse importance, but definitely two trends can be easily identifies: i) fundamental research on properties of ultra cold atoms and molecules, and in particular atomic and molecular condensates trapped and lattice gases; here the fundamental questions of nature and form of phase transitions in degenerate systems are being posed and studied; ii) more applications oriented research on ultracold atoms and molecules, involving in particular applications in precision measurements, atomic clocks, frequency standards, atom and molecule interferometry, quantum information, quantum engineering, "super" chemistry etc.This thesis concerns both of these major trends.The applications, or more specifically quantum engineering aspect are discussed in the first four chapters of the thesis, which deal with optical manipulations of ultra cold gases, in particular optical generation of vortices in Bose condensates, quasi-solitons in Fermi gases, and retarded dipole-dipole interactions in Bose, or Fermi gases.This thesis consists of four main chapters.Chapter 2, "Optical generation of vortices in Bose Einstein Condensates".In this chapter we study theoretically the generation of vortices by phase imprinting in trapped Bose-Einstein condensates.Phase imprinting is achieved by passing a short off-resonance laser pulse through an appropriately designed absorption plate, and impinging it on a condensate.We answer the fundamental question of how the circulation and the vortex are introduced into the system, and discuss the creation of vortex arrays.We discuss vortex dynamics and interactions in such configurations.Various methods of vortex detection based on interference combined with Bragg scattering are also analyzed.In Chapter 3, "Fermionic 'Solitons'" we investigate in detail the concept of low energy excitations of ultra cold Fermi gases.This excitations are generated using the same idea of phase imprinting as that employed in the generation of vortices in BEC.We address in this chapter some questions concerning the generation (via phase imprinting) of soliton-like solutions in a single-component Fermi gas of neutral atoms at zero and finite temperatures.By using both numerical and analytical calculations, we find the conditions under which it is possible to find in non-interacting Fermi gases, quasisolitons which resemble the properties of solitons in non-linear integrable equations.We present the results for both spatially homogeneous and trapped cases, and emphasize the importance of Fermi statistics and the absence of interactions for the existence of such solutions.In Chapter 4, "Generating Dipole Condensate" we keep studying the possibilities of optical manipulations of ultracold gases.In particular, we study two different ways to laser-induce dipole-dipole interactions in trapped Bose-Einstein condensates.The first one employs the fact that those atoms in high Rydberg states posses a large dipolar moment.We first analyze the idea of imposing the dipole moment as a time average over short stroboscopic pulses.These pulses are coherently transporting the atoms from the ground atomic state to some high Rydberg state and back.The second idea is based on the observation that in strong static or oscillatory electric fields, atoms polarize and acquire dipole moment.We analyze the possibilities and limitations of inducing such a high electric field using lasers of low frequency.In Chapter 5, "Dipolar BCS", we continue our study of trapped fermionic gases, with the analysis of the BCS transition in trapped dipolar fermionic gases.We find that the critical strength of the dipole-dipole interaction to achieve BCS pairing, depends on the trap geometry.We find the particular form of this dependence, and present the solutions for the order parameter.This first chapter is meant as a general introduction to the thesis.This introduction is by no means exhaustive, and should be rather treated as a collection of basic facts concerning ultra cold gases, without rigorous derivations.The last subsection of the introductory chapter, discusses very briefly the most important achievements and trends in the field and the current state of the art.
In this thesis I report on experiments that enter a new regime in the many body physics of ultracold atomic gases. A Bose-Einstein condensate is loaded into a three-dimensional optical lattice potential formed by a standing wave laser light field. In this novel quantum system we have been able to both realize a quantum phase transition from a superfluid to a Mott insulator, and to observe the collapse and revival of a macroscopic matter wave field. Quantum phase transitions are driven by quantum fluctuations and occur, even at zero temperature, as the relative strength of two competing energy terms in the underlying Hamiltonian is varied across a critical value. In the first part of this work I report on the observation of such a quantum phase transition in a Bose-Einstein condensate with repulsive interactions, held in a three-dimensional optical lattice potential. In the superfluid ground state, each atom is spread-out over the entire lattice, whereas in the Mott insulating state, exact numbers of atoms are localized at individual lattice sites. We observed the reversible transition between those states and detected the gap in the excitation spectrum of the Mott insulator. A Bose-Einstein condensate is usually described by a macroscopic matter wave field. However, a quantized field underlies such a "classical" matter wave field of a Bose-Einstein condensate. The striking behavior of ultracold matter due to the field quantization and the nonlinear interactions between the atoms is the focus of the second part of this work. The matter wave field of a Bose-Einstein condensate is observed to undergo a series of collapses and revivals as time evolves. Furthermore, we show that the collisions between individual pairs of atoms lead to a fully coherent collisional phase shift in the corresponding many-particle state, which is a crucial cornerstone of proposed novel quantum computation schemes with neutral atoms. With these experiments we enter a new field of physics with ultracold quantum gases. In this strongly correlated regime, interactions between atoms dominate the behavior of the many-body system such that it can no longer be described by the usual theories for weakly interacting Bose gases. This novel quantum system offers the unique possibility to experimentally address fundamental questions of modern solid state physics, atomic physics, quantum optics, and quantum information.
At the most fundamental level of quantum electrodynamics, there is no such thing as two-body interactions between atoms. The potentials that describe these interactions are effective potentials resulting from a series of approximations whose validity depends on the precise situation at hand. Considering a one-dimensional geometry for simplicity, we discuss under which conditions the familiar form of the near-resonant dipole-dipole interaction is valid, paying particular attention to the effects of interatomic propagation of light, and to what extent it can be modified in the tailored electromagnetic environments provided by optical resonators. We find that once the atoms have established that they are inside a resonator, the dipole-dipole potential may or may not remain a useful concept, depending upon the strength of the atom-field interaction. In the weak-coupling regime, one finds a two-body dipole-dipole interaction that can be enhanced or inhibited by varying the atom-field detuning. In the strong-coupling regime, by contrast, the two-body dipole-dipole potential ceases to be meaningful.
This thesis covers most of my work in the field of ultracold atoms loaded in optical lattices. It makes a route through the physics of cold atoms in periodic potentials starting from the simple noninteracting system and going into the many-body physics that describes the strongly correlated Mott insulator regime. Even though this thesis is a theoretical work all the chapters are linked either with experiments already done or with ongoing experimental efforts. This thesis can be divided into four different parts. The first part comprises chapters 1 to 3. In these chapters, after a brief introduction to the field of optical lattices I review the fundamental aspects pertaining to the physics of systems in periodic potentials. The second part deals with the superfluid weakly interacting regime where standard mean field techniques can be applied. This is covered in chapters 4 and 5. Specifically, chapter 4 introduces the discrete nonlinear Schroedinger equation (DNLSE) and uses it to model some experiments. In chapter 5 I go one step further and include the small quantum fluctuations neglected in the DNLSE by studying quadratic approximations of the Bose-Hubbard Hamiltonian. Chapters 6 to 8 can be grouped as the third part of the thesis. In them I adopt an effective action formalism, the so called two particle irreducible effective action (2PI) together with the closed time path (CTP) formalism to study far-from-equilibrium dynamics. The many-body techniques discussed in these chapters systematically include higher order quantum corrections, not included in the quadratic approximations of the Hamiltonian, which we show are crucial for a correct description of the quantum dynamics outside the very weakly interacting regime. Finally, chapter 9 to 11 are devoted to study the Mott insulator phase. In these chapters using perturbation theory I study the Mott insulator ground state and its excitation spectrum, the response of the system to Bragg spectroscopy, and propose a mechanism to correct for the residual quantum coherences inherent to the Mott insulator ground state. Even though small these are not ideal for the use of neutral atoms in optical lattice as a tool for quantum computation.
This dissertation contains a study of ultracold atoms in optical cavities. We particularly focus on two aspects of the coupled atom-cavity systems. In the first aspect, we implement the quantum nature of the light field to probe the quantum state of the atoms. This is interesting due to the nondestructive nature of the characterization of many-body atomic states. In the second aspect we study the cavity optomechanics that investigates the coupling of mechanical and optical degrees of freedom via radiation pressure. The optomechanical cavity provides an interesting nonlinear system to study the coupling between atoms and the intracavity field.In the context of cavity quantum electrodynamics we study the reflection of two counter-propagating modes of the light field in a high-Q ring cavity by ultracold atoms either in the Mott insulator state or in the superfluid state of an optical lattice. We find that the dynamics of the reflected light strongly depends on both the lattice spacing and the state of the matter-wave field. By using the Monte Carlo wave-function method to account for the cavity damping we also determine the two-time correlation function and the time-dependent physical spectrum of theretroreflected field. We find that the light field and the atoms become entangled if the latter are in a superfluid state. We also analyze quantitatively the entanglement between the atoms and the light.In cavity optomechanics the mechanical effect can either comes from a vibrating macroscopic oscillator or a collective density excitation of a Bose-Einstein condensate. First we use a Fabry-Perot-type cavity to study the opto-mechanically-induced bistable quantum phase transitions between superfluid and a Mott insulator states of an ultracold bosonic gases trapped inside the cavity. Secondly, we study the symmetricand antisymmetric collective density side modes of the BEC which results from the optomechanical effects of the light fields in a ring cavity.